The Chisana Formation consists of Lower Cretaceous volcanic rocks that occur in the Nutzotin Mountains of eastern Alaska. New stratigraphic analysis indicates that the volcanic succession is >2 km thick at the Bonanza Creek type section. We present stratigraphic, geochemical, Sr‐Nd‐Pb isotope, and U‐Pb age data from samples collected from various stratigraphic levels of the Chisana Formation. We demonstrate that the Chisana Formation can be divided into a lower subaqueous unit, a middle transitional unit, and an upper subaerial unit. Chisana Formation lavas range from transitional to subalkaline basalts through andesites. Trace element geochemistry shows high field strength element depletions relative to large ion lithophile elements and hydrous mineral assemblages with calc‐alkaline to tholeiitic chemistries, all consistent with a magmatic arc origin. Chisana lavas yield geochemical compositions and isotope characteristics that overlap with magmas from volcanic suites formed within juvenile continental crust and immature island arcs. Volcanism occurred between ~131 and 117 Ma judging from previously reported lava ages and new U‐Pb ages of detrital zircons recovered from sandstones that conformably underlie the lowermost Chisana Formation lavas. Our results support existing tectonic models in which an east dipping subduction zone existed beneath Wrangellia during Early Cretaceous time. The upsection shift from marine to terrestrial depositional conditions in the Chisana Formation and the overlying ~117–93 Ma Beaver Lake Formation was coincident with regional shortening. Together, the geologic evidence for shortening and terrestrial deposition are interpreted to reflect accretion/suturing of Wrangellia against inboard terranes.

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