Two new kinds of the structural in-homogeneities in the polystyrene films were created by the irradiation of the film with nanosecond pulses of the infrared laser with 1064 nm wavelength. At the beginning of the irradiation dark micro-inclusions having unusual close to rectangular geometries appeared. After about 30 seconds of the irradiation one more kind structural distortions appeared having the geometries of the systems of the concentric micro-rings. Simultaneously with the creation of these concentric micro-rings the film started to emit bright blue luminescence all over its area and significant focusing of the laser beam during its propagation through the film was observed resulting in the generation of the bright white flashes at the screen installed behind the film. The creation of the dark rectangular spots as well as of the concentric micro-rings are ascribed to the non-linear interactions between the laser radiation and the structural distortions produced in the film due to photo-thermal processes excited in the film.
Spectral features of cryogenic liquids, especially nitrogen, seem to be clearly investigated due to the wide application in science. On the other hand, material properties can really be different under intensive laser irradiation. During irradiation of liquid nitrogen with pulsed (pulse duration 20 ns) YaG: Nd 1064 nm laser with average power of 0.3 W we have found bright luminescence in the visible region with five narrow spectral lines. This phenomenon can be explained by the multiphoton excitation of nitrogen molecules and ions with infrared photons. Its spatial and spectral characteristics are attributed to Amplified Spontaneous Emission. The main features include super-linear dependence of the emission intensity on the intensity of the excitation radiation, limited amount of narrow spectral bands and conical geometry of the emission with the clear separation of the cones in correspondence with the spectral lines of the emission. This phenomenon manifests liquid nitrogen as the convenient substance of Kerr type for studies of various non-linear optical processes by means of nanosecond lasers instead of femtosecond lasers applied usually for these purposes.
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