[1] This paper presents the intercomparison of O 3 , HNO 3 , ClO, N 2 O and CO profiles measured by the two spaceborne microwave instruments MLS (Microwave Limb Sounder) and SMR (Submillimetre Radiometer) on board the Aura and Odin satellites, respectively. We compared version 1.5 level 2 data from MLS with level 2 data produced by the French data processor version 222 and 225 and by the Swedish data processor version 2.0 for several days in September 2004 and in March 2005. For the five gases studied, an overall good agreement is found between both instruments. Most of the observed discrepancies between SMR and MLS are consistent with results from other intercomparison studies involving MLS or SMR. O 3 profiles retrieved from the SMR 501.8 GHz band are noisier than MLS profiles but mean biases between both instruments do not exceed 10%. SMR HNO 3 profiles are biased low relative to MLS's by $30% above the profile peak. In the lower stratosphere, MLS ClO profiles are biased low by up to 0.3 ppbv relative to coincident SMR profiles, except in the Southern Hemisphere polar vortex in the presence of chlorine activation. N 2 O profiles from both instruments are in very good agreement with mean biases not exceeding 15%. Finally, the intercomparison between SMR and MLS CO profiles has shown a good agreement from the middle stratosphere to the middle mesosphere in spite of strong oscillations in the MLS profiles. In the upper mesosphere, MLS CO concentrations are biased high relative to SMR while negative values in the MLS retrievals are responsible for a negative bias in the tropics around 30 hPa.
International audienceThe HAMSTRAD microwave instrument operates at 60 and 183 GHz and measures temperature and water vapor, respectively, from 0- to 10-km altitude with a time resolution of 7 min. The radiometer has been successfully deployed at Dome C (Concordia Station), Antarctica (75°06' S, 123°21' E, 3233 m amsl) during the first summertime campaign for 12 days in January-February 2009. The radiometer has been continuously running since January 2010, hosted within a dedicated shelter. We have used the very first set of HAMSTRAD data, recorded when the instrument was outdoors, to assess its potential to sound the troposphere over Dome C, from the planetary boundary layer (PBL) up to the tropopause ( ~ 6 km above surface, ~ 9 km amsl). We have compared the HAMSTRAD measurements to several sets of measurements performed at the Dome-C station or in its vicinity: meteorological radiosondes, in situ PT100 and Humicap sondes along the vertical extent of a 45-m tower, meteorological sensor attached to the HAMSTRAD instrument, and the spaceborne Infrared Atmospheric Sounding Interferometer (IASI) instrument onboard the EUMETSAT MetOp-A satellite in polar orbit. The variability of integrated water vapor (IWV) observed by HAMSTRAD with extremely low values of 0.5 kg *m-2 was also measured by the radiosondes (very high HAMSTRAD versus radiosonde correlation of 0.98), whereas IASI cloud-free measurements did not reproduce well the HAMSTRAD IWV variation (weak HAMSTRAD versus IASI correlation of 0.58). The measurements of absolute humidity (H2O) from HAMSTRAD at Dome C cover a large vertical extent from the surface to about 6 km above surface with a high sensitivity in the free troposphere. The strong diurnal variation of H2O observed by the in situ sensors in the PBL is not well detected by the radiometer. In the free troposphere, the HAMSTRAD versus radiosonde H2O correlation can reach 0.8-0.9. Around the tropopause, HAMSTR- D shows the same variability as IASI and radiosondes but with a dry bias of 0.01 g *m-3. HAMSTRAD tends to show a wetter atmosphere by 0.1-0.3 g *m-3 compared with radiosondes from the surface to ~ 2-km altitude and a drier atmosphere above by ~ 0.1g *m-3. The sensitivity of the temperature profiles from HAMSTRAD is very high in the PBL and in the free troposphere but degrades around the tropopause. The strong diurnal signal measured above the surface by HAMSTRAD (3-6 K) is consistent with all the other in situ data sets. The temporal evolution over the 12-day period in the PBL is also consistent with all other data sets (radiosondes, IASI, in situ sondes, and meteorological sensors). In the free troposphere and around the tropopause, the HAMSTRAD temporal evolution is consistent with that observed by radiosondes and IASI, although a cold bias exists compared with IASI and radiosondes around the tropopause. For heights less than 4 km above surface, HAMSTRAD correlates very well with radiosondes and in situ sensors (correlation better than 0.8) but less well with IASI (0.4). Below the tropopause, th...
International audienceThe H2O Antarctica Microwave Stratospheric and Tropospheric Radiometers (HAMSTRAD) program aims to develop two ground-based microwave radiometers to sound tropospheric and stratospheric water vapor (H2O) above Dome C (Concordia Station), Antarctica (75??06' S, 123??21'E, 3233 m asml), an extremely cold and dry environment, over decades. By using state-of-the-art technology, the HAMSTRAD-Tropo radiometer uses spectral information in the domains 51-59 GHz (oxygen line) and 169-197 GHz (water vapor line) to derive accurate tropospheric profiles of temperature (with accuracy ranging from 1 to 2 K) and low absolute humidity (with accuracy ranging from 0.02 to 0.05 g ?? m-3), together with integrated water vapor (with accuracy of about 0.008 kg ?? m-2) and liquid water path. Prior to its installation at Dome C in January 2009, the fully automated radiometer has been deployed at the Pic du Midi (PdM, 42??56'N, 0??08'E, 2877 m asml, France) in February 2008 and was in operation for five months. Preliminary comparisons with radio soundings particularly launched in the vicinity of PdM in February 2008 and the outputs from the mesoscale MESO-NH model show a great consistency to within 0.2-0.3 g ?? m-3 between all absolute humidity data sets whatever the atmosphere considered (extremely dry or wet)
We present profile measurements of key constituents relevant to stratospheric chemistry and dynamics such as ozone (O3), nitrous oxide (N2O), and chlorine monoxide (ClO) taken during the 2002–03 northern hemisphere winter by the Odin Sub‐Millimetre Radiometer (SMR), a limb‐sounding satellite sensor launched in February 2001. The observations of the chemically passive tracer N2O show a subsidence of lower stratospheric air masses inside the Arctic vortex in the range of 3–5 km, or 60–100 K in terms of potential temperature, for the period November 2002 to March 2003. Activated chlorine in the form of ClO was observed inside the vortex from the beginning of December until mid‐February. The accumulated chemical ozone loss over this period, derived from the correlation of ozone with N2O, is estimated to be 28 ± 9% on the 50 ppbv level of N2O, i.e., for lower stratospheric air masses subsiding from ∼23 down to 19 km, the lower limit of the Odin/SMR ozone measurement in the 501.8 GHz band.
This paper presents the first algorithm developed to retrieve atmospheric vertical profiles of trace gases from calibrated spectra measured by the sub-millimetre radiometer (SMR) onboard the Odin satellite. An estimation of atmospheric profiles is obtained by means of an inversion of the spectra using the Optimal Estimation Method. Great attention is paid to the study of the simultaneous retrieval of several species and nonlinearity effects. The measurement response is defined to give the altitude domain of a good retrieval. Main sources of measurement and forward model errors are characterized and separated into two categories: the fixed errors and the variable errors. We define a standard retrieval strategy that can be applied to theoretically investigate any frequency band of any observing Odin mode. For each frequency band, two categories of species are defined: the target species, i.e., the main species to be retrieved, and the interfering species, i.e., molecules emitting an interfering radiance in the observed band. The standard code is based upon an inversion of spectra using a linearized forward model and simultaneously estimates target species and interfering species. As an example, inversions of synthetic noise-free spectra of ozone and chlorine monoxide within an autocorrelator band ranging from 501.18 to 501.58 GHz are shown to behave as expected in the middle stratosphere and in the lower mesosphere. The error analysis shows retrieval limitations in the lower stratosphere that are mainly induced by the high sensitivity of the retrieval to parameters such as tangent height, accuracy in the vertical profile of the interfering species, and spectral parameters of both target lines and interfering lines. PACS Nos.: 42.68Ay, 07.07Df, 07.57Kp
Abstract. Ground-based microwave measurements of the diurnal and seasonal variations of ozoneat 42±4.5 and 55±8 km are validated by comparing with results from a zero-dimensional photochemical model and a two-dimensional (2D) chemical/radiative/dynamical model, respectively. O3 diurnal amplitudes measured in Bordeaux are shown to be in agreement with theory to within 5%. For the seasonal analysis of O3 variation, at 42±4.5 km, the 2D model underestimates the yearly averaged ozone concentration compared with the measurements. A double maximum oscillation (~3.5%) is measured in Bordeaux with an extended maximum in September and a maximum in February, whilst the 2D model predicts only a single large maximum (17%) in August and a pronounced minimum in January. Evidence suggests that dynamical transport causes the winter O3 maximum by propagation of planetary waves, phenomena which are not explicitly reproduced by the 2D model. At 55±8 km, the modeled yearly averaged O3 concentration is in very good agreement with the measured yearly average. A strong annual oscillation is both measured and modeled with differences in the amplitude shown to be exclusively linked to temperature fields.
Measurements of mid-stratospheric formaldehyde (H2CO) have been obtained from the limb-viewing sub-millimeter radiometer (SMR) instrument aboard the Odin satellite. The analysis is based upon the only weak (808→707) rotational transition line of H2CO that can be measured by Odin/SMR at 576.7083150 GHz in the band dedicated to the measurement of carbon monoxide (CO). The signal-to-noise ratio is increased by averaging about 1000 spectra within 2-km width vertical layers in the stratosphere over periods from 1 to 7 days and within 3 latitude bands: Southern Hemisphere (90°S–45°S), tropics (30°S–30°N), and Northern Hemisphere (45°N–90°N). The faint H2CO line can then be retrieved using the standard scientific ground-segment developed for the Odin/SMR measurements. The mid-stratospheric H2CO shows maxima in the tropics for every period considered (January 2006, February 2005, March 2005, and September 2005). The spring-time extra-tropical mid-stratospheric H2CO is more intense than the fall-time extra-tropical amounts. The simulations from the three-dimensional chemical-transport model Reprobus satisfactorily show these general features
We present a new compact ground-based microwave radiometer dedicated to the study of middle atmospheric water vapor. The instrument detects the 616 − 523 H2O transition line at 22.235 GHz. This radiometer has been designed to be easily transported and operated during measurement campaigns in remote places. The first retrievals, performed with the MOLIERE inversion and radiative transfer software, show good agreement with MIAWARA, the 22 GHz Radiometer developed at the University of Bern, Switzerland, and the Microwave Limb Sounder instrument onboard the Aura satellite.
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