We demonstrate a versatile tunable and highly stable ultrabroadband Ti:sapphire chirped pulse amplification system with a compressed pulse energy of 20 mJ at 100 Hz repetition rate. High power Ti:Sa systems in principle do not offer wavelength tunability due to gain narrowing. Here we demonstrate transform limited pulse generation from 15 fs to 94 fs with tunable central wavelength (λc from 755 nm to 845 nm) and bandwidth (130 nm<Δλ<16 nm) as well as multi-color, time synchronized, sub-100 fs pulses with user defined central wavelength separation. The unique wavelength tunability capabilities have been expanded into the UV and deep-UV by second and third harmonic generation with excellent energy stability. Enhanced energy stability is achieved by multiplexing six ultrastable diode-based solid state pump lasers.

We demonstrate the first carrier-envelope phase (CEP)-stabilized chirped pulse amplification system with pulse peak-powers in the terawatt regime. The system, which eventually is intended to be used in the generation of isolated attosecond pulses, consists of two consecutive multipass amplification stages. The first amplification stage is a commercial CEP-stable kHz system including a single 13-pass amplifier reaching a pulse energy of 2.3 mJ. Pulses are picked after the first stage at a repetition rate of 50 Hz and are further amplified in a 5-pass power-amplifier to pulse energies that reach up to 80 mJ before compression. After compression the pulse energy is 35mJ at a pulse duration of 32 fs, signifying a peak power of 1.1 terawatt. Peak-powers exceeding 1.5 TW should easily be achievable by improving the efficiency of the grating compressor. The CEP-stability of the terawatt system is demonstrated by single shot measurements of the residual CEP jitter at the full repetition rate and show an excellent root-mean-square value of 315 mrad.

Recompressed pulses from Ti:sapphire chirped-pulse lasers are accompanied by a slowly decaying post-pulse pedestal that is coherent with the main pulse. The pedestal typically consists of numerous pulses with temporal separation in the picosecond range. The source of this artifact lies in the Ti:sapphire active medium itself, both in the Kerr-lens mode-locked oscillator and in subsequent amplifiers. In the presence of substantial self-phase modulation, after recompression the post-pedestal generates a mirror-symmetric pre-pulse pedestal. This pedestal severely degrades the leading edge of the output pulse. This degradation is far more limiting than the original post-pedestal and severely lowers the achievable temporal contrast.

We present a new method to control the Carrier-Envelope Phase of ultra-short laser pulses by using the linear Electro-Optic Effect. Experimental demonstration is carried out on a Chirped Pulse Amplification based laser. Phase shifts greater than π radian can be obtained by applying moderate voltage on a LiNbO3 crystal with practically no changes to all other parameters of the pulse with the exception of its group delay. Time response of the Electro-Optic effect makes possible shaping at a high repetition rate or stabilization of the CEP of ultra short CPA laser systems.

Using an original CEP stabilization technique based on the linear electro-optical effect in a specific crystal, we achieved long term CEP stabilization of a 20 W, 1 kHz laser with residual noise as low as 440 mrad (rms). At 3 W, the CEP shot to shot noise is kept as low as 320 mrad (rms) over half an hour.