This experimental study examines the relationship between transverse jet structural characteristics and the shear layer instabilities forming on the upstream side of the jet column. Jets composed of mixtures of helium and nitrogen were introduced perpendicularly into a low-speed wind tunnel using several alternative injectors: convergent circular nozzles mounted either flush with or elevated above the tunnel floor, and a flush-mounted circular pipe. Both non-intrusive optical diagnostics (planar laser-induced fluorescence (PLIF) and particle image velocimetry (PIV)) and intrusive probe-based (hot-wire anemometry) measurements were used to explore a range of jet-to-crossflow momentum flux ratios and density ratios for which previous studies have identified upstream shear layer transition from convective to absolute instability. Remarkable correspondences were identified between formation of the well-known counter-rotating vortex pair (CVP) associated with the jet cross-section and conditions producing strong upstream shear layer vorticity rollup, arising typically from absolute instability in the shear layer. In contrast, asymmetries in the jet mean cross-sectional shape and/or lack of a clear CVP were observed to correspond to weaker, convectively unstable jet shear layers.
A nozzle-beam-skimmer sampling system is used to measure species concentration profiles for a lean one-dimensional premixed CO-02-Ar flame, into which small amounts of sulfur dioxide are introduced. The net formation rate for sulfur trioxide is obtained from the flux fraction profile for this species. The kinetic schemeis then utilized, along with the measured temperature profiles, to evaluate the rate Coefficients k l and k2 over the temperature range of 1435-1850 K. The most satisfactory agreement between the measured net formation rate for SO3 and that calculated on the basis of reactions (1) and (2) Reactions (1) and (2) are found to be nearly balanced in a substantial region of the flame. Here the data are more sensitive to the difference in activation energies, as opposed to a particular value for either. Implications of this observation on the uncertainty of the deduced temperature dependence for each reaction are discussed, as are some of the procedures used in the data analysis.
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