The article describes the problems of creating a scintillation spectrometer with a CsI:Tl crystal to replace spectrometers with NaI:Tl crystals which are widely used at nuclear power plants (NPPs) to monitor the activity of air, waste water and adjacent territories. The advantages of CsI:Tl-spectrometers are in the best energy resolution; much greater resistance to mechanical and electromagnetic influences due to the use of silicon photomultipliers (SiPM) instead of vacuum photomultiplier tubes (VPMT); much greater durability due to the very low hygroscopicity of the material. The strong mismatch between the emission spectrum of the crystal and the spectral sensitivity of the VPMT photocathodes, the relatively long decay time and the complex, multicomponent form of the light flash made spectrometers with CsI:Tl crystals not competitive. The paper describes the methods of constructing a spectrometer, which made it possible to realize the useful properties inherent in a crystal and to level its disadvantages. As a result of the cycle of research and development work, the Stark-02 intellectual detector has been designed and described. Typical relative energy resolution with crystals of volume 45 cm3 at an energy of 662 keV of the 137Cs source is better than 6.5% in the ambient temperature range Q = +10 ÷ +45 °C and not worse than 7.5% in the extended range Q = –25 ÷ +55 °C.
The article describes an equipment for the complex determination of elements in the so-called «intermediate» solutions of spent nuclear fuel (SNF) WOKER. The equipment combines the functions of a densitometer, X-ray fluorescence analyzer and g-spectrometer, some of them can be performed in parallel. The problems of creating high-quality measuring channels of the WOKER and the results achieved are discussed. Particular attention is paid to the method of analysis implemented with the WOKER, which has been successfully used during several years in the radiochemical production of the «Mayak» Production Association.
The article analyzes the possibilities of using modern scintillators that provide a relative energy resolution along the y-line of 137Cs ER662keV ≤ 5%. Precision gamma spectrometers are relevant for use in technological processes of the nuclear industry, at nuclear power plants for monitoring the activity of air, waste water and adjacent areas, etc. Now 36 scintillation crystals are known that meet the above mentioned requirement. Of these, only 8 are produced by industry. Seven crystals are candidates for development in industrial production. The rest are hardly suitable for practical use due to the low light yield of LY (Cs2NaGdCl6:Ce, Tl2LiYCl6:Ce and TlCaCl3, for example). Eu-activated crystals have a high light output (LY = 60÷100 ph/MeV) and a low light output nonlinearity (NLY = 7÷10%) in a wide range of electron energies, which is extremely important for the spectrometry of “soft” y-radiation (ER662keV ≤ 10%). Due to the high self-absorption of light, these scintillators lose their advantages in the energy range Ey = 200÷3000 keV. The article shows that among the scintillators suitable for the simultaneous detection of gamma and neutron radiation, crystals containing 6Li are more preferable.
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