The ability to tune magnetic orders, such as magnetic anisotropy and topological spin texture, is desired in order to achieve high-performance spintronic devices. A recent strategy has been to employ interfacial engineering techniques, such as the introduction of spin-correlated interfacial coupling, to tailor magnetic orders and achieve novel magnetic properties. We chose a unique polar-nonpolar LaMnO3/SrIrO3 superlattice because Mn (3d)/Ir (5d) oxides exhibit rich magnetic behaviors and strong spin-orbit coupling through the entanglement of their 3d and 5d electrons. Through magnetization and 3 magnetotransport measurements, we found that the magnetic order is interface-dominated as the superlattice period is decreased. We were able to then effectively modify the magnetization, tilt of the ferromagnetic easy axis, and symmetry transition of the anisotropic magnetoresistance of the LaMnO3/SrIrO3 superlattice by introducing additional Mn (3d) and Ir (5d) interfaces. Further investigations using in-depth first-principles calculations and numerical simulations revealed that these magnetic behaviors could be understood by the 3d/5d electron correlation and Rashba spin-orbit coupling.The results reported here demonstrate a new route to synchronously engineer magnetic properties through the atomic stacking of different electrons, contributing to future applications.
The pyrochlore lattice involves corner sharing tetrahedra and the resulting geometric frustration is believed to suppress any antiferromagnetic order for Mott insulators on this structure. There are nevertheless short-range correlations which could be vital near the Mott-Hubbard insulator-metal transition. We use a static auxiliaryfield-based Monte Carlo to study this problem in real space on reasonably large lattices. The method reduces to unrestricted Hartree-Fock at zero temperature but captures the key magnetic fluctuations at finite temperature. Our results reveal that increasing interaction drives the non magnetic (semi) metal to a 'spin disordered' metal with small local moments, at some critical coupling, and then, through a small pseudogap window, to a large moment, gapped, Mott insulating phase at a larger coupling. The spin disordered metal has a finite residual resistivity which grows with interaction strength, diverging at the upper coupling. We present the resistivity, optical conductivity, and density of states across the metal-insulator transition and for varying temperature. These results set the stage for the more complex cases of Mott transition in the pyrochlore iridates and molybdates.
The Shastry-Sutherland model and its generalizations have been shown to capture emergent complex magnetic properties from geometric frustration in several quasi-two-dimensional quantum magnets. Using an sd exchange model, we show here that metallic Shastry-Sutherland magnets can exhibit a topological Hall effect driven by magnetic skyrmions under realistic conditions. The magnetic properties are modeled with competing symmetric Heisenberg and asymmetric Dzyaloshinskii-Moriya exchange interactions, while a coupling between the spins of the itinerant electrons and the localized moments describes the magnetotransport behavior. Our results, employing complementary Monte Carlo simulations and a novel machine learning analysis to investigate the magnetic phases, provide evidence for field-driven skyrmion crystal formation for an extended range of Hamiltonian parameters. By constructing an effective tight-binding model of conduction electrons coupled to the skyrmion lattice, we clearly demonstrate the appearance of the topological Hall effect. We further elaborate on the effects of finite temperatures on both magnetic and magnetotransport properties.
We report the numerical investigation of strain induced superconductor-insulator quantum phase transition on a Lieb lattice. Based on a non perturbative Monte Carlo technique we show that in two dimensions an s-wave superconductor undergoes transition to a highly correlated Bosonic insulator under the influence of strain, applied as staggered hopping amplitudes. To the best of our knowledge, this is the first work to report theoretical investigation of "disorder free" superconductor-insulator phase transition in systems with Lieb lattice structure. With the recent experimental realization of the Lieb lattice in ultracold atomic gases, photonic lattices as well as in solid state systems, we believe that the results presented in this paper would be of importance to initiate experimental investigation of such novel quantum phase transitions. We further discuss the fate of such systems at finite temperature, highlighting the effect of fluctuations on the superconducting pair formations, thermal scales and quasiparticle behavior. The high temperature quasiparticle signatures discussed in this paper are expected to serve as benchmarks for experiments such as radio frequency and momentum resolved radio frequency spectroscopy measurements carried out on systems such as ultracold atomic gases.
-Strongly correlated electron systems; heavy fermions PACS 71.30.+h -Metal-insulator transitions and other electronic transitions PACS 75.10.-b -General theory and models of magnetic ordering Abstract -The rare-earth based pyrochlore molybdates involve orbitally degenerate electrons Hund's coupled to local moments. The large Hund's coupling promotes ferromagnetism, the superexchange between the local moments prefers antiferromagnetism, and Hubbard repulsion tries to open a Mott gap. The phase competition is tuned by the rare-earth ionic radius, decreasing which leads to change from a ferromagnetic metal to a spin disordered highly resistive ground state, and ultimately an 'Anderson-Mott' insulator. We attempt a quantitative theory of the molybdates by studying their minimal model on a pyrochlore geometry, using a static auxiliary field based Monte Carlo. We establish a thermal phase diagram that closely corresponds to the experiments, predict the hitherto unexplored orbital correlations, quantify and explain the origin of the anomalous resistivity, and present dynamical properties across the metal-insulator transition.Introduction. -Traditional Mott materials involve a strong on-site Coulomb interaction that, beyond a critical value, and at integer filling, inhibits electron motion [1]. This, in a clean material, leads to an abrupt change in the zero temperature state from perfectly conducting to non conducting. The non conducting state typically has strong antiferromagnetic (AF) correlations, if not long range order, since that lowers the kinetic energy.The Mott transition on a frustrated structure brings in a novelty since the AF ordered state in the Mott phase cannot be realised and one may have the signatures of a 'spin liquid' [2,3]. Such phases are realised in some triangular lattice organics [4][5][6]. The pyrochlores [7] are also highly frustrated structures, much studied for possible spin liquid phases, but the rare earth molybdates, R 2 Mo 2 O 7 , add additional twists to the Mott problem: (i) the Mott transition in these materials occur in the background of overall ferromagnetic correlation [7][8][9], and (ii) the zero temperature resistivity seems to grow continuously with the control parameter [10] (see next) rather than having an abrupt zero to infinity transition. These features owe their origin to the additional degrees of freedom, and couplings, involved in these materials.The R 2 Mo 2 O 7 family exhibit ground states that vary from a ferromagnetic metal (FM) to a spin glass metal (SG-M) and then a spin glass insulator (SG-I) as the rare earth radius r R is reduced [11]. Materials with R = Nd and Sm are metallic, R = Tb, Dy, Ho, Er, and Y are insulating, and R=Gd is on the verge
We study the classical Heisenberg model on the geometrically frustrated Shastry-Sutherland (SS) lattice with additional Dzyaloshinskii-Moriya (DM) interaction in the presence of an external magnetic field. We show that several noncollinear and noncoplanar magnetic phases, such as the flux, all-in/all-out, 3-in-1-out/3-out-1-in, and canted-flux phases are stabilized over wide ranges of parameters in the presence of the DM interaction. We discuss the role of DM interaction in stabilizing these complex magnetic phases. When coupled to these noncoplanar magnetic phases, itinerant electrons experience a finite Berry phase, which manifests in the form of topological Hall effect, whereby a nonzero transverse conductivity is observed even in the absence of a magnetic field. We study this anomalous magnetotransport by calculating the electron band structure and transverse conductivity for a wide range of parameter values, and demonstrate the existence of topological Hall effect in the SS lattice. We explore the role of the strength of itinerant electron-local moment coupling on electron transport and show that the topological Hall features evolve significantly from strong to intermediate values of the coupling strength, and are accompanied by the appearance of a finite spin Hall conductivity.
The checkerboard lattice, with alternating 'crossed' plaquettes, serves as the two dimensional analog of the pyrochlore lattice. The corner sharing plaquette structure leads to a hugely degenerate ground state, and no magnetic order, for classical spins with short range antiferromagnetic interaction. For the half-filled Hubbard model on this structure, however, we find that the Mott insulating phase involves virtual electronic processes that generate longer range and multispin couplings. These couplings lift the degeneracy, selecting a 'flux like' state in the Mott insulator. Increasing temperature leads, strangely, to a sharp crossover from this state to a '120 degree' correlated state and then a paramagnet. Decrease in the Hubbard repulsion drives the system towards an insulator-metal transition-the moments reduce, and a spin disordered state wins over the flux state. Near the insulator-metal transition the electron system displays a pseudogap extending over a large temperature window.
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