Solid ferromagnetic materials are rigid in shape and cannot be reconfigured. Ferrofluids, although reconfigurable, are paramagnetic at room temperature and lose their magnetization when the applied magnetic field is removed. Here, we show a reversible paramagnetic-to-ferromagnetic transformation of ferrofluid droplets by the jamming of a monolayer of magnetic nanoparticles assembled at the water-oil interface. These ferromagnetic liquid droplets exhibit a finite coercivity and remanent magnetization. They can be easily reconfigured into different shapes while preserving the magnetic properties of solid ferromagnets with classic north-south dipole interactions. Their translational and rotational motions can be actuated remotely and precisely by an external magnetic field, inspiring studies on active matter, energy-dissipative assemblies, and programmable liquid constructs.

The interesting physics and potential memory technologies resulting from topologically protected spin textures such as skyrmions, has prompted efforts to discover new material systems that can host these kind of magnetic structures. Here we use the highly tunable magnetic properties of amorphous Fe/Gd multilayer films to explore the magnetic properties that lead to dipole-stabilized skyrmions and skyrmion lattices that form from the competition of dipolar field and exchange energy. Using both real space imaging and reciprocal space scattering techniques we determined the range of material properties and magnetic fields where skyrmions form.Micromagnetic modeling closely matches our observation of small skyrmion features (~50 to 70nm) and suggests these class of skyrmions have a rich domain structure that is Bloch like in the center of the film and more Néel like towards each surface. Our results provide a pathway to engineer the formation and controllability of dipole skyrmion phases in a thin film geometry at different temperatures and magnetic fields.

We present direct, real-time observations of emergent magnetic monopole dynamics in highly frustrated artificial spin ice.