Magnetic Weyl semimetals with broken time-reversal symmetry are expected to generate strong intrinsic anomalous Hall effects, due to their large Berry curvature. Here, we report a magnetic Weyl semimetal candidate, Co3Sn2S2, with a quasi-two-dimensional crystal structure consisting of stacked Kagomé lattices. This lattice provides an excellent platform for hosting exotic topological quantum states. We observe a negative magnetoresistance that is consistent with the chiral anomaly expected from the presence of Weyl nodes close to the Fermi level. The anomalous Hall conductivity is robust against both increased temperature and charge conductivity, which corroborates the intrinsic Berry-curvature mechanism in momentum space. Owing to the low carrier density in this material and the significantly enhanced Berry curvature from its band structure, the anomalous Hall conductivity and the anomalous Hall angle simultaneously reach 1130 Ω−1 cm−1 and 20%, respectively, an order of magnitude larger than typical magnetic systems. Combining the Kagomé-lattice structure and the out-of-plane ferromagnetic order of Co3Sn2S2, we expect that this material is an excellent candidate for observation of the quantum anomalous Hall state in the two-dimensional limit.
A large anomalous Hall effect is observed in the triangular antiferromagnet Mn3Ge arising from an intrinsic electronic Berry phase.
Weyl semimetals (WSMs) are topological quantum states wherein the electronic bands disperse linearly around pairs of nodes with fixed chirality, the Weyl points. In WSMs, nonorthogonal electric and magnetic fields induce an exotic phenomenon known as the chiral anomaly, resulting in an unconventional negative longitudinal magnetoresistance, the chiral-magnetic effect. However, it remains an open question to which extent this effect survives when chirality is not well-defined. Here, we establish the detailed Fermi-surface topology of the recently identified WSM TaP via combined angle-resolved quantum-oscillation spectra and band-structure calculations. The Fermi surface forms banana-shaped electron and hole pockets surrounding pairs of Weyl points. Although this means that chirality is ill-defined in TaP, we observe a large negative longitudinal magnetoresistance. We show that the magnetoresistance can be affected by a magnetic field-induced inhomogeneous current distribution inside the sample.
The peculiar band structure of semimetals exhibiting Dirac and Weyl crossings can lead to spectacular electronic properties such as large mobilities accompanied by extremely high magnetoresistance. In particular, two closely neighboring Weyl points of the same chirality are protected from annihilation by structural distortions or defects, thereby significantly reducing the scattering probability between them. Here we present the electronic properties of the transition metal diphosphides, WP2 and MoP2, which are type-II Weyl semimetals with robust Weyl points by transport, angle resolved photoemission spectroscopy and first principles calculations. Our single crystals of WP2 display an extremely low residual low-temperature resistivity of 3 nΩ cm accompanied by an enormous and highly anisotropic magnetoresistance above 200 million % at 63 T and 2.5 K. We observe a large suppression of charge carrier backscattering in WP2 from transport measurements. These properties are likely a consequence of the novel Weyl fermions expressed in this compound.
Applying a temperature gradient in a magnetic material generates a voltage that is perpendicular to both the heat flow and the magnetization. 1,2 This is the anomalous Nernst effect (ANE), 3,4 which was thought to be proportional to the value of the magnetization for a long time. However, more generally, the ANE has been predicted to originate from a net Berry curvature of all bands near the Fermi level (EF. 5,6 Subsequently, a large anomalous Nernst thermopower ( ) has recently been observed in topological materials with no net magnetization but large net Berry curvature [n(k)] around EF. 7-9 These experiments clearly fall outside the scope of the conventional magnetization-model of the ANE, but a significant question remains: Can the value of the ANE in topological ferromagnets exceed the highest values observed in conventional ferromagnets? Here, we report a remarkably high -value of ~6.0 µV K −1 at 1 T in the ferromagnetic topological Heusler compound Co2MnGa at room temperature, which is around 7-times larger than any anomalous Nernst thermopower value ever reported for a conventional ferromagnet. Combined electrical, thermoelectric and first-principles calculations reveal that this high value of the ANE arises from a large net Berry curvature near the Fermi level associated with nodal lines and Weyl points.
In stark contrast to ordinary metals, in materials in which electrons strongly interact with each other or with phonons, electron transport is thought to resemble the flow of viscous fluids. Despite their differences, it is predicted that transport in both conventional and correlated materials is fundamentally limited by the uncertainty principle applied to energy dissipation. Here we report the observation of experimental signatures of hydrodynamic electron flow in the Weyl semimetal tungsten diphosphide. Using thermal and magneto-electric transport experiments, we find indications of the transition from a conventional metallic state at higher temperatures to a hydrodynamic electron fluid below 20 K. The hydrodynamic regime is characterized by a viscosity-induced dependence of the electrical resistivity on the sample width and by a strong violation of the Wiedemann–Franz law. Following the uncertainty principle, both electrical and thermal transport are bound by the quantum indeterminacy, independent of the underlying transport regime.
The search for highly efficient and low-cost catalysts is one of the main driving forces in catalytic chemistry. Current strategies for the catalyst design focus on increasing the number and activity of local catalytic sites, such as the edge sites of molybdenum disulfides in the hydrogen evolution reaction (HER). Here, the study proposes and demonstrates a different principle that goes beyond local site optimization by utilizing topological electronic states to spur catalytic activity. For HER, excellent catalysts have been found among the transition-metal monopnictides-NbP, TaP, NbAs, and TaAs-which are recently discovered to be topological Weyl semimetals. Here the study shows that the combination of robust topological surface states and large room temperature carrier mobility, both of which originate from bulk Dirac bands of the Weyl semimetal, is a recipe for high activity HER catalysts. This approach has the potential to go beyond graphene based composite photocatalysts where graphene simply provides a high mobility medium without any active catalytic sites that have been found in these topological materials. Thus, the work provides a guiding principle for the discovery of novel catalysts from the emerging field of topological materials.
An axion insulator is a correlated topological phase, predicted to arise from the formation of a charge density wave in a Weyl semimetal. The accompanying sliding mode in the charge density wave phase, the phason, is an axion. It is expected to cause anomalous magneto-electric transport effects. However, this axionic charge density wave has so far eluded experimental detection. In this paper, we report the observation of a large, positive contribution to the magneto-conductance in the sliding mode of the charge density wave Weyl semimetal (TaSe4)2I for collinear electric and magnetic fields (E||B).The positive contribution to the magneto-conductance originates from the anomalous axionic contribution of the chiral anomaly to the phason current, and is locked to the parallel alignment of E and B. By rotating B, we show that the angular dependence of the magneto-conductance is consistent with the anomalous transport of an axionic charge density wave. 3 Axions refer to elementary particles that have long been known in quantum field theory, 1,2 but have yet to be observed in nature. However, it has been recently understood that axions can emerge as collective electronic excitations in certain crystals, so-called axion insulators. 3 Despite being fully gapped to single-particle excitations in the bulk and at the surface, an axion insulator is characterized by an effective action, which includes a topological EB-term, where E and B are the electromagnetic fields inside the insulator, and plays the role of the dynamical axion field. Physically, the average value of is determined by the microscopic details of the band structure of the system, and gives rise to unusual magnetoelectric response properties such as quantum anomalous Hall conductivities 4-9 , the quantized circular photo-galvanic 4,10,11 effect, and the chiral magnetic effect. 4,[12][13][14] The prospect of realizing an axion insulator has inspired much theoretical and experimental work. Only very recently, signatures of a dynamic axion field have been found on the surface of magnetically doped topological insulator thin films. [15][16][17] However, the axionic quasi-particle in these systems-the axionic polariton 3 -has so far eluded experimental detection. Alternatively, axion insulators have been predicted to arise in Weyl semimetals that are unstable towards the formation of a charge density wave (CDW). [18][19][20][21][22][23] In their parent state, Weyl semimetals are materials in which the low-energy electronic quasiparticles behave as chiral relativistic fermions without rest mass, known as Weyl fermions. [24][25][26][27] The Weyl fermions exist at isolated crossing points of conductance and valence bands-so called Weyl nodes-and their energy can be approximated with a linear dispersion relation ( Fig. 1 (a)). The Weyl nodes always occur in pairs of opposite "handedness" or chirality. At low energies and in the absence of interactions the chirality is a conserved quantum number, and the two chiral populations do not mix. Parallel electric and mag...
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