The present study provides a detailed investigation of the neck-configuration and Q-values on the cluster decay of proton-rich even-even 124-128Ba isotopes using the relativistic mean-field (RMF) formalism with the NL3* parameter set. The densities of the interacting nuclei from the RMF approach are folded with the R3Y and M3Y interactions to obtain the nuclear potential via the double-folding technique. The preformed cluster model (PCM) based on the quantum mechanical fragmentation theory is employed for the calculation of the decay half-lives. The preformation probability P0 and the penetration probabilities are estimated by the phenomenological scaling factor of Blendowske & Walliser and the WKB approximation respectively. The present investigation reveals that the M3Y and R3Y are associated with different barrier characteristics which are significantly modified with a little variation in the neck-length parameter ΔR. From the Q-value analysis, we have demonstrated that α-decay may not be a favourable decay mode for proton-rich barium isotopes with A > 122.
A new α-emitting has been observed experimentally for neutron deficient 214U which opens the window to theoretically investigate the ground state properties of 214,216,218U isotopes and to examine α-particle clustering around the shell closure. The decay half-lives are calculated within the preformed cluster-decay model (PCM). To obtain the α-daughter interaction potential, the RMF densities are folded with the newly developed R3Y and the well-known M3Y NN potentials for comparison. The alpha preformation probability (Pα) is calculated from the analytic formula of Deng and Zhang. The WKB approximation is employed for the calculation of the transmission probability. The individual binding energies (BE) for the participating nuclei are estimated from the relativistic mean-field (RMF) formalism and those from the finite range droplet model (FRDM) as well as WS3 mass tables. In addition to Z=84, the so-called abnormal enhancement region, i.e., 84≤Z≤90 and N<126, is normalised by an appropriately fitted neck-parameter ΔR. On the other hand, the discrepancy sets in due to the shell effect at (and around) the proton magic number Z=82 and 84, and thus a higher scaling factor ranging from 10−5–10−8 is required. Additionally, in contrast with the experimental binding energy data, large deviations of about 5–10 MeV are evident in the RMF formalism despite the use of different parameter sets. An accurate prediction of α-decay half-lives requires a Q-value that is in proximity with the experimental data. In addition, other microscopic frameworks besides RMF could be more reliable for the mass region under study. α-particle clustering is largely influenced by the shell effect.
An extensive study of [Formula: see text]-decay half-lives for various decay chains of isotopes of [Formula: see text] is performed within the axially deformed relativistic mean-field (RMF) formalism by employing the NL3, NL3[Formula: see text], and DD-ME2 parameter set. The structural properties of the nuclei appearing in the decay chains are explored. The binding energy, quadrupole deformation parameter, root-mean-square charge radius, and pairing energy are calculated for the even–even isotopes of [Formula: see text], which are produced in five different [Formula: see text]-decay chains, namely, [Formula: see text], [Formula: see text], [Formula: see text], [Formula: see text], and [Formula: see text]. A superdeformed prolate ground state is observed for the heavier nuclei, and gradually the deformation decreases towards the lighter nuclei in the considered decay chains. The RMF results are compared with various theoretical predictions and experimental data. The [Formula: see text]-decay energies are calculated for each decay chain. To determine the relative numerical dependency of the half-life for a specific [Formula: see text]-decay energy, the decay half-lives are calculated using four different formulas, namely, Viola–Seaborg, Alex–Brown, Parkhomenko–Sobiczewski and Royer for the above said five [Formula: see text]-decay chain. We notice a firm dependency of the half-life on the [Formula: see text]-decay formula in terms of [Formula: see text]-values for all decay chains. Further, this study also strengthens the prediction for the island of stability in terms of magic number at the superheavy valley in the laboratories.
The fusion dynamics of 16O + 154Sm and 18O+148Nd reactions has been investigated to observe the effect of shape degree of freedom on the fusion cross-section using the coupled channel (CC) calculations. The one dimentional barrier penetration model (1-D BPM) is observed to underestimate the experimental data mainly at below barrier energies. The coupled channel calculations, including target projectile excitations with 1 phonon of vibrational state and 2+ rotational state of target, reproduce the experimental fusion cross-section for 16O + 154Sm reaction at below barrier energies, while show some discrepancy for 18O+148Nd reaction. This discrepancy for 18O+148Nd reaction can be addressed with the inclusion of low-lying states with neutron transfer channels and the neck-formation.
Background: The theoretical and experimental investigations of decay properties of heavy and superheavy nuclei are crucial to explore the nuclear structure and reaction dynamics. Purpose: The aim of this study is to probe the α-decay properties of 243Fm and 245Fm isotopic chains using relativistic mean-field (RMF) approach within the framework of preformed cluster-decay model (PCM). Methods: The RMF densities are folded with the relativistic R3Y NN potential to deduce the nuclear interaction potential between the α particle and daughter nucleus. The penetration probability is calculated within the WKB approximation. Results: The α-decay half-lives of even-odd 243Fm and 245Fm isotopes and their daughter nuclei are obtained from the preformed cluster-decay model. These theoretically calculated half-lives are found to be in good agreement with the recent experimental measurements. Conclusions: The novel result here is the applicability of the scaling factor within the PCM as a signature for shell/sub-shell closures in α-decay studies. As such, we have also demonstrated that N=137, 139 and Z=94 corresponding to 231,233Pu could be shell/sub-shell closures. The least T1/2 is found at 243,245Fm which indicate their individual stability and α-decay as their most probable decay mode.
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