International audienceOzone profile trends over the period 2000 to 2016 from several merged satellite ozone data sets and from ground-based data by four techniques at stations of the Network for the Detection of Atmospheric Composition Change indicate significant ozone increases in the upper stratosphere, between 35 and 48 km altitude (5 and 1 hPa). Near 2 hPa (42 km), ozone has been increasing by about 1.5 % per decade in the tropics (20° S to 20° N), and by 2 to 2.5 % per decade in the 35° to 60° latitude bands of both hemispheres. At levels below 35 km (5 hPa), 2000 to 2016 ozone trends are smaller and not statistically significant. The observed trend profiles are consistent with expectations from chemistry climate model simulations. Using three to four more years of observations and updated data sets, this study confirms positive trends of upper stratospheric ozone already reported, e.g., in the WMO/UNEP Ozone Assessment 2014, or by Harris et al. (2015). The additional years, and the fact that nearly all individual data sets indicate these increases, give enhanced confidence. Nevertheless, a thorough analysis of possible drifts and differences between various data sources is still required, as is a detailed attribution of the observed increases to declining ozone depleting substances and to stratospheric cooling. Ongoing quality observations from multiple independent platforms are key for verifying that recovery of the ozone layer continues as expected

[1] In this paper we investigate daily variations in middle atmospheric water vapor and ozone based on data from two ground-based microwave radiometers located in the Alpine region of Europe. Temperature data are obtained from a lidar located near the two stations and from the SABER experiment on the TIMED satellite. This unique set of observations is complemented by three different three-dimensional (3-D) chemistry-climate models (Monitoring of Stratospheric Depletion of the Ozone Layer (MSDOL), Laboratoire de Météorologie Dynamique Reactive Processes Ruling the Ozone Budget in the Stratosphere (LMDz-REPROBUS), and Solar Climate Ozone Links (SOCOL)) and the 2-D atmospheric global-scale wave model (GSWM). The first part of the paper is focused on the first Climate and Weather of the Sun-Earth System (CAWSES) tidal campaign that consisted of a period of intensive measurements during September 2005. Variations in stratospheric water vapor are found to be in the order of 1% depending on altitude. Meridional advection of tidal nature is likely to be the dominant driving factor throughout the whole stratosphere, while vertical advection becomes more important in the mesosphere. Observed ozone variations in the upper stratosphere and lower mesosphere show amplitudes of several percent in accordance with photochemical models. Variations in lower stratospheric ozone are not solely governed by photochemistry but also by dynamics, with the temperature dependence of the photochemistry becoming more important. The second part presents an investigation of the seasonal dependence of daily variations. Models tend to underestimate the H 2 O diurnal amplitudes, especially during summer in the upper stratosphere. Good agreement between models and observations is found for ozone in the upper stratosphere, which reflects the fact that the O 3 daily variations are driven by the photochemistry that is well modeled.

The long‐term evolution of upper stratospheric ozone has been recorded by lidars and microwave radiometers within the ground‐based Network for the Detection of Stratospheric Change (NDSC), and by the space‐borne Solar Backscatter Ultra‐Violet instruments (SBUV), Stratospheric Aerosol and Gas Experiment (SAGE), and Halogen Occultation Experiment (HALOE). Climatological mean differences between these instruments are typically smaller than 5% between 25 and 50 km. Ozone anomaly time series from all instruments, averaged from 35 to 45 km altitude, track each other very well and typically agree within 3 to 5%. SBUV seems to have a slight positive drift against the other instruments. The corresponding 1979 to 1999 period from a transient simulation by the fully coupled MAECHAM4‐CHEM chemistry climate model reproduces many features of the observed anomalies. However, in the upper stratosphere the model shows too low ozone values and too negative ozone trends, probably due to an underestimation of methane and a consequent overestimation of ClO. The combination of all observational data sets provides a very consistent picture, with a long‐term stability of 2% or better. Upper stratospheric ozone shows three main features: (1) a decline by 10 to 15% since 1980, due to chemical destruction by chlorine; (2) two to three year fluctuations by 5 to 10%, due to the Quasi‐Biennial Oscillation (QBO); (3) an 11‐year oscillation by about 5%, due to the 11‐year solar cycle. The 1979 to 1997 ozone trends are larger at the southern mid‐latitude station Lauder (45°S), reaching −8%/decade, compared to only about −6%/decade at Table Mountain (35°N), Haute Provence/Bordeaux (≈45°N), and Hohenpeissenberg/Bern(≈47°N). At Lauder, Hawaii (20°N), Table Mountain, and Haute Provence, ozone residuals after subtraction of QBO‐ and solar cycle effects have levelled off in recent years, or are even increasing. Assuming a turning point in January 1997, the change of trend is largest at southern mid‐latitude Lauder, +11%/decade, compared to +7%/decade at northern mid‐latitudes. This points to a beginning recovery of upper stratospheric ozone. However, chlorine levels are still very high and ozone will remain vulnerable. At this point the most northerly mid‐latitude station, Hohenpeissenberg/Bern differs from the other stations, and shows much less clear evidence for a beginning recovery, with a change of trend in 1997 by only +3%/decade. In fact, record low upper stratospheric ozone values were observed at Hohenpeissenberg/Bern, and to a lesser degree at Table Mountain and Haute Provence, in the winters 2003/2004 and 2004/2005.

Abstract. TEMPERA (TEMPERature RAdiometer) is a new ground-based radiometer which measures in a frequency range from 51-57 GHz radiation emitted by the atmosphere. With this instrument it is possible to measure temperature profiles from ground to about 50 km. This is the first groundbased instrument with the capability to retrieve temperature profiles simultaneously for the troposphere and stratosphere. The measurement is done with a filterbank in combination with a digital fast Fourier transform spectrometer. A hot load and a noise diode are used as stable calibration sources. The optics consist of an off-axis parabolic mirror to collect the sky radiation. Due to the Zeeman effect on the emission lines used, the maximum height for the temperature retrieval is about 50 km. The effect is apparent in the measured spectra. The performance of TEMPERA is validated by comparison with nearby radiosonde and satellite data from the Microwave Limb Sounder on the Aura satellite. In this paper we present the design and measurement method of the instrument followed by a description of the retrieval method, together with a validation of TEMPERA data over its first year, 2012.

International audienceUpper stratospheric ozone anomalies from the satellite-borne Solar Backscatter Ultra-Violet (SBUV), Stratospheric Aerosol and Gas Experiment II (SAGE II), Halogen Occultation Experiment (HALOE), Global Ozone Monitoring by Occultation of Stars (GOMOS), and Scanning Imaging Absorption Spectrometer for Atmospheric Chartography (SCIAMACHY) instruments agree within 5% or better with ground-based data from lidars and microwave radiometers at five stations of the Network for the Detection of Atmospheric Composition Change (NDACC), from 45°S to 48°N. From 1979 until the late 1990s, all available data show a clear decline of ozone near 40 km, by 10%–15%. This decline has not continued in the last 10 years. At some sites, ozone at 40 km appears to have increased since 2000, consistent with the beginning decline of stratospheric chlorine. The phaseout of chlorofluorocarbons after the International Montreal Protocol in 1987 has been successful, and is now showing positive effects on ozone in the upper stratosphere. Temperature anomalies near 40 km altitude from European Centre for Medium Range Weather Forecast reanalyses (ERA-40), from National Centers for Environmental Prediction (NCEP) operational analyses, and from HALOE and lidar measurements show good consistency at the five stations, within about 3 K. Since about 1985, upper stratospheric temperatures have been fluctuating around a constant level at all five NDACC stations. This non-decline of upper stratospheric temperatures is a significant change from the more or less linear cooling of the upper stratosphere up until the mid-1990s, reported in previous trend assessments. It is also at odds with the almost linear 1 K per decade cooling simulated over the entire 1979–2010 period by chemistry–climate models (CCMs). The same CCM simulations, however, track the historical ozone anomalies quite well, including the change of ozone tendency in the late 1990s

Abstract. MIPAS observations of temperature, water vapor, and ozone in October 2009 as derived with the scientific level-2 processor run by Karlsruhe Institute of Technology (KIT), Institute for Meteorology and Climate Research (IMK) and CSIC, Instituto de Astrofísica de Andalucía (IAA) and retrieved from version 4.67 level-1b data have been compared to co-located field campaign observations obtained during the MOHAVE-2009 campaign at the Table Mountain Facility near Pasadena, California in October 2009. The MIPAS measurements were validated regarding any potential biases of the profiles, and with respect to their precision estimates. The MOHAVE-2009 measurement campaign provided measurements of atmospheric profiles of temperature, water vapor/relative humidity, and ozone from the ground to the mesosphere by a suite of instruments including radiosondes, ozonesondes, frost point hygrometers, lidars, microwave radiometers and Fourier transform infrared (FTIR) spectrometers. For MIPAS temperatures (version V4O T 204), no significant bias was detected in the middle stratosphere; between 22 km and the tropopause MIPAS temperatures were found to be biased low by up to 2 K, while below the tropopause, they were found to be too high by the same amount. These findings confirm earlier comparisons of MIPAS temperatures to ECMWF data which revealed similar differences. Above 12 km up to 45 km, MIPAS water vapor (version V4O H2O 203) is well within 10 % of the data of all correlative instruments. The well-known dry bias of MIPAS water vapor above 50 km due to neglect of non-LTE effects in the current retrievals has been confirmed. Some instruments indicate that MIPAS water vapor might be biased high by 20 to 40 % around 10 km (or 5 km below the tropopause), but a consistent picture from all comparisons could not be derived. MIPAS ozone (version V4O O3 202) has a high bias of up to +0.9 ppmv around 37 km which is due to a non-identified continuum like radiance contribution. No further significant biases have been detected. Cross-comparison to co-located observations of other satellite instruments (Aura/MLS, ACE-FTS, AIRS) is provided as well.

Abstract. WIRA is a ground-based microwave Doppler spectroradiometer specifically designed for the measurement of profiles of horizontal wind in the upper stratosphere and lower mesosphere region where no other continuously running measurement technique exists. A proof of principle has been delivered in a previous publication. A technical upgrade including a new high-frequency amplifier and sideband filter has improved the signal to noise ratio by a factor of 2.4. Since this upgrade the full horizontal wind field comprising zonal and meridional wind profiles is continuously measured. A completely new retrieval based on optimal estimation has been set up. Its characteristics are detailed in the present paper.Since the start of the routine operation of the first prototype in September 2010, WIRA has been measuring at four different locations at polar, mid-and tropical latitudes (67 • 22 N/26 • 38 E, 46 • 57 N/7 • 26 E, 43 • 56 N/5 • 43 E and 21 • 04 S/55 • 23 E) for time periods between 5.5 and 11 months. The data presented in this paper are daily average wind profiles with typical uncertainties and resolutions of 10 to 20 m s −1 and 10 to 16 km, respectively. A comparison between the data series from WIRA and European Centre for Medium-Range Weather Forecasts (ECMWF) model data revealed agreement within 10 % in the stratospheric zonal wind. The meridional wind profiles agree within their error bars over the entire sensitive altitude range of WIRA. However, significant differences in the mesospheric zonal wind speed of up to 50 % have been found.

The ground‐based microwave radiometers GROMOS and MIAWARA at Bern (Switzerland) continuously measure ozone and water vapor profiles from 20 to 70 km altitude. A major sudden stratospheric warming occurred around 19 February 2008 with minimal temperatures of 189 K at 40 hPa and maximal temperatures of 300 K at 4 hPa. During the stratospheric warming the Swiss ground‐based radiometers observed a depletion of ozone and an enhancement of water vapor while NASA's CALIPSO satellite instrument measured a large PSC area over Europe. Ozone depletion in the lower stratosphere is explained by transport of ozone poor air from the cold polar vortex. The depletion of upper stratospheric ozone is caused by a sudden temperature increase of about 50 K. A simulation of a chemical box model confirms that a major fraction of the observed decrease of the ozone mixing ratio at 4 hPa can be explained by the effect of the increasing temperature on the ozone chemistry. The chemical ozone destruction is dominated by a catalytic NOx cycle, which is more efficient at higher temperatures. The water vapor enhancement can be explained by transport processes. The rather unusual occurrence of a PSC and a sudden stratospheric warming at midlatitudes suggest that further monitoring of the Earth's middle atmosphere is required for the timely detection of unexpected problems due to ozone loss and climate change.