Low‐temperature sinterable BaCe2(MoO4)4 ceramics were prepared through solid‐state ceramic route. X‐ray diffraction, laser Raman spectroscopy and scanning electron microscopy techniques have been used to investigate the structure and microstructure of BaCe2(MoO4)4 ceramics. The laser Raman study reveals distorted MoO42− tetrahedral networks in the unit cell of the BaCe2(MoO4)4 ceramics. The BaCe2(MoO4)4 exhibits a dielectric constant of 12.3, an unloaded quality factor of 3320, and a temperature coefficient of resonant frequency of −37 ppm/°C.
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