Squeezing of quantum fluctuations by means of entanglement is a well-recognized goal in the field of quantum information science and precision measurements. In particular, squeezing the fluctuations via entanglement between 2-level atoms can improve the precision of sensing, clocks, metrology, and spectroscopy. Here, we demonstrate 3.4 dB of metrologically relevant squeezing and entanglement for 10 5 cold caesium atoms via a quantum nondemolition (QND) measurement on the atom clock levels. We show that there is an optimal degree of decoherence induced by the quantum measurement which maximizes the generated entanglement. A 2-color QND scheme used in this paper is shown to have a number of advantages for entanglement generation as compared with a single-color QND measurement. N A for the case of independent atoms also referred to as a coherent spin state (CSS). The CSS minimizes the Heisenberg uncertainty product so that, e.g., (δJ z ) 2 (δJ x ) 2 = 1 4| J y | 2 where J y is the expectation value of the spin projection operator. At the expense of an increase in (δJ x ) 2 , it is possible to reduce (δJ z ) 2 (or vice versa) below the projection noise limit while keeping their product constant. This constitutes an example of a spin squeezed state (SSS), for which the atoms need to be correlated. This correlation is ensured to be nonclassical ifwhere ξ defines the squeezing parameter. Under this condition, the atoms are entangled (3) and the prepared state improves the signal-to-noise ratio in spectroscopical and metrological applications (1). Systems of 2 to 3 ions have successfully been used to demonstrate spectroscopic performance with reduced quantum noise and entanglement (4, 5). The situation is somewhat different with macroscopic atomic ensembles where spin squeezing has been an active area of research in the past decade (6-13). To our knowledge, no results reporting ξ < 1 via interatomic entanglement in such ensembles have been reported so far, with a very recent exception of the paper (14) where entanglement in an external motional degree of freedom of 2 · 10 3 atoms via interactions in a Bose-Einstein condensate is demonstrated. Spin Squeezing by Quantum Nondemolition (QND) MeasurementsIn this article, we report on the generation of an SSS fulfilling Eq. 1 in an ensemble of ≈10 5 atoms via a QND measurement (7, 15-17) of J z . We show how to take advantage of the entanglement in this mesoscopic system by using Ramsey spectroscopy (1)-one of the methods of choice for precision measurements of time and frequency (18) (Fig. 1A). The figure presents the evolution of the pseudospin J whose tip is traveling over the Bloch sphere. The Ramsey method allows using the atomic ensemble as a sensor for external fields where the perturbation of the energy difference between the levels ΔE ↑↓ is measured, or as a clock where the frequency of an oscillator is locked to the transition frequency between the two states Ω = ΔE ↑↓ / . Fig. 1 B illustrates how a suitable SSS can improve the precision of the Ramsey measurement pr...

Abstract. We use a quantum non-demolition measurement to generate a spin squeezed state and to create entanglement in a cloud of 10 5 cold cesium atoms. For the first time we operate an atomic clock improved by spin squeezing beyond the projection noise limit in a proof-of-principle experiment. For a clockinterrogation time of 10 µs, the experiments show an improvement of 1.1 dB in the signal-to-noise ratio, compared to the atomic projection noise limit.

We report on structural properties of two-component Coulomb crystals in a linear Paul trap. The crystals consist of two laser cooled ion species, 24Mg+ and 40Ca+. The lighter 24Mg+ ions form an inner cylindrical crystal structure surprisingly similar to that of an infinitely long single component crystal, while the outermost shell of the surrounding 40Ca+ ions have a spheroidal shape, which is highly insensitive to the presence of the 24Mg+ ions. Observed changes in the radial separation of the two ion species with the radius of the inner cylindrical crystal is explained by a simple model.

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