Stretchable and conformable synapse memristors that can emulate the behaviour of the biological neural system and well adhere onto the curved surfaces simultaneously are desirable for the development of imperceptible wearable and implantable neuromorphic computing systems. Previous synapse memristors have been mainly limited to rigid substrates. Herein, a stretchable and conformable memristor with fundamental synaptic functions including potentiation/depression characteristics, long/short-term plasticity (STP and LTP), "learning-forgetting-relearning" behaviour, and spike-rate-dependent and spike-amplitude-dependent plasticity is demonstrated based on highly elastic Ag nanoparticle-doped thermoplastic polyurethanes (TPU : Ag NPs) and polydimethylsiloxane (PDMS). The memristor can be well operated even at 60% strain and can be well conformed onto the curved surfaces. The formed conductive filament (CF) obtained from the movement of Ag nanoparticle clusters under the locally enhanced electric field gives rise to resistance switching of our memristor. These results indicate a feasible strategy to realize stretchable and conformable synaptic devices for the development of new-generation artificial intelligence computers.
Ultrathin organic thin-film transistors (OTFTs) have received extensive attention due to their outstanding advantages, such as extreme flexibility, good conformability, ultralight weight, and compatibility with low-cost and large-area solution-processed techniques. However, compared with the rigid substrates, it still remains a challenge to fabricate high-performance ultrathin OTFTs. In this study, a high-performance ultrathin 2,7-dioctyl[1]benzothieno[3,2-b][1]benzothiophene (C8-BTBT) OTFT array is demonstrated via a simple spin-coating method, with mobility as high as 11 cm V s (average mobility: 7.22 cm V s ), on/off current ratio of over 10 , switching current of >1 mA, and a good yield ratio as high as 100%. The ultrathin thickness at ≈380 nm and the ultralight weight at ≈0.89 g m enable the free-standing OTFTs to imperceptibly adhere onto human skin, and even a damselfly wing without affecting its flying. More importantly, the OTFTs show good electrical characteristics and mechanical stability when conformed onto the curved surfaces and even folded in a book after 100 folding cycles. These results illustrate the broad application potential of this simply fabricated ultrathin OTFT in next-generation electronics such as foldable displays and wearable devices.
To achieve adhesive and conformable wearable electronics, improving stretchable transparent electrode (STE) becomes an indispensable bottleneck needed to be addressed. Here, we adopt a nonuniform Young’s modulus structure with silver nanowire (AgNW) and fabricate a STE layer. This layer possesses transparency of >88% over a wide spectrum range of 400–1000 nm, sheet resistance below 20 Ω sq−1, stretchability of up to 100%, enhanced mechanical robustness, low surface roughness, and good interfacial wettability for solution process. As a result of all these properties, the STE enables the fabrication of a highly efficient ultraflexible wearable device comprising of both organic photovoltaic (OPV) and organic photodetector (OPD) parts with high mechanical durability and conformability, for energy-harvesting and biomedical-sensing applications, respectively. This demonstrates the great potential of the integration of OPVs and OPDs, capable of harvesting energy independently for biomedical applications, paving the way to a future of independent conformable wearable OPV/OPDs for different applications.
Commercial applications of the skin-like electronic devices for healthcare, intelligent robotics and electronic communication, require large-scale high-density transistor array with high mechanical deformability and robustness that can be provided by...
A photolithographic stretchable transparent electrode comprising PEDOT:PSS and SWCNT was developed for an all-solution-processed transparent conformal organic transistor array.
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