Inelastic neutron scattering is used to investigate the collective magnetic excitations of the high-temperature superconductor-parent antiferromagnet La2CuO4. We find that while the lower energy excitations are well described by spin-wave theory, including one- and two-magnon scattering processes, the high-energy spin waves are strongly damped near the (1/2, 0) position in reciprocal space and merge into a momentum dependent continuum. This anomalous damping indicates the decay of spin waves into other excitations, possibly unbound spinon pairs.
We report the discovery of ferroelectricity below 4.5 K in highly underdoped La 2 CuO 4+x accompanied by slow charge dynamics which develop below T~40 K. An anisotropic magnetoelectric response has also been observed, indicating considerable spin-charge coupling in this lightly doped "parent" high temperature copper-oxide superconductor. The ferroelectric state is proposed to develop from polar nanoregions, in which spatial inversion symmetry is locally broken due to non-stoichiometric carrier doping.
We use inelastic neutron scattering with spin polarization analysis to study the magnetic excitations in the normal and superconducting states of YBa 2 Cu 3 O 6.9 . Polarization analysis allows us to determine the spin polarization of the magnetic excitations and to separate them from phonon scattering. In the normal state, we find unambiguous evidence of magnetic excitations over the 10-60 meV range of the experiment with little polarization dependence to the excitations. In the superconducting state, the magnetic response is enhanced near the "resonance energy" and above. At lower energies, 10 E 30 meV, the local susceptibility becomes anisotropic, with the excitations polarized along the c axis being suppressed. We find evidence for a new diffuse anisotropic response polarized perpendicular to the c axis which may carry significant spectral weight.
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