Recent demonstrations of magnetization switching induced by in-plane current in heavy metal/ferromagnetic heterostructures (HMFHs) have drawn great attention to spin torques arising from large spin-orbit coupling (SOC). Given the intrinsic strong SOC, topological insulators (TIs) are expected to be promising candidates for exploring spin-orbit torque (SOT)-related physics. Here we demonstrate experimentally the magnetization switching through giant SOT induced by an in-plane current in a chromium-doped TI bilayer heterostructure. The critical current density required for switching is below 8.9 × 10(4) A cm(-2) at 1.9 K. Moreover, the SOT is calibrated by measuring the effective spin-orbit field using second-harmonic methods. The effective field to current ratio and the spin-Hall angle tangent are almost three orders of magnitude larger than those reported for HMFHs. The giant SOT and efficient current-induced magnetization switching exhibited by the bilayer heterostructure may lead to innovative spintronics applications such as ultralow power dissipation memory and logic devices.

Breaking of structural symmetries of nanomagnetic systems is of great interest for the development of ultralow-power spintronic devices. The structural asymmetry in various magnetic heterostructures has been engineered to reveal novel fundamental interactions between electric currents and magnetization, resulting in spin-orbit-torques (SOTs) on the magnetization [1][2][3][4][5][6] , which are both fundamentally important and technologically promising for device applications. Such SOTs have been used to realize current-induced magnetization switching [2][3][4]7 and domain-wall 3 motion [8][9][10] in recent experiments. Typical heterostructures exhibiting SOTs consist of a ferromagnet (F) with a heavy nonmagnetic metal (NM) having strong spin-orbit coupling on one side, and an insulator (I) on the other side (referred to as NM/F/I structures, shown schematically in Fig. 1a, which break mirror symmetry in the growth direction). In terms of device applications, the use of SOTs in NM/F/I structures allows for a significantly lower write current compared to regular spin-transfer-torque (STT) devices 4 . It can greatly improve energy efficiency and scalability [1][2][3][4][5]11 for new SOT-based devices such as magnetic random access memory (SOT-MRAM), going beyond state-of-the-art STT-MRAM.For practical applications, a critical requirement to achieve high-density SOT memory is the ability to perform SOT-induced switching without the use of external magnetic fields, in particular for perpendicularly-magnetized ferromagnets, which show better scalability and thermal stability as compared to the in-plane case 12 .However, there are currently no practical solutions that meet this requirement. In NM/F/I heterostructures studied so far, the form of the resultant current-induced SOT alone does not allow for deterministic switching of a perpendicular ferromagnet, requiring application of an additional external in-plane magnetic field to switch the perpendicular magnetization [2][3][4] . (This is a very general feature of SOT devices, which can be explained by symmetry-based arguments, as discussed below). In such experiments, the external field allows for each current direction to favor a particular orientation for the out-of-plane component of magnetization, thereby resulting in deterministic perpendicular switching. However, this external field is undesirable 4 from a practical point of view. For device applications, it also reduces the thermal stability of the perpendicular magnet by lowering the zero-current energy barrier between the stable perpendicular states, resulting in a shorter retention time if used for memory.This work provides a solution to eliminate the use of external magnetic fields, bringing SOT-based spintronic devices such as SOT-MRAM closer to practical application. We present a new NM/F/I structure, which provides a novel spin-orbit torque, resulting in zero-field current-induced switching of perpendicular magnetization. Our device consists of a stack of Ta/Co 20 Fe 60 B 20 /TaO x layers, but also has a...

Topological insulators display unique properties, such as the quantum spin Hall effect, because time-reversal symmetry allows charges and spins to propagate along the edge or surface of the topological insulator without scattering. However, the direct manipulation of these edge/surface states is difficult because they are significantly outnumbered by bulk carriers. Here, we report experimental evidence for the modulation of these surface states by using a gate voltage to control quantum oscillations in Bi(2)Te(3) nanoribbons. Surface conduction can be significantly enhanced by the gate voltage, with the mobility and Fermi velocity reaching values as high as ~5,800 cm(2) V(-1) s(-1) and ~3.7 × 10(5) m s(-1), respectively, with up to ~51% of the total conductance being due to the surface states. We also report the first observation of h/2e periodic oscillations, suggesting the presence of time-reversed paths with the same relative zero phase at the interference point. The high surface conduction and ability to manipulate the surface states demonstrated here could lead to new applications in nanoelectronics and spintronics.

We investigate the quantum anomalous Hall Effect (QAHE) and related chiral transport in the millimetersize (Cr 0.12 Bi 0.26 Sb 0.62 ) 2 Te 3 films. With high sample quality and robust magnetism at low temperatures, the quantized Hall conductance of e 2 /h is found to persist even when the film thickness is beyond the twodimensional (2D) hybridization limit. Meanwhile, the Chern insulator-featured chiral edge conduction is manifested by the non-local transport measurements. In contrast to the 2D hybridized thin film, an additional weakly field-dependent longitudinal resistance is observed in the 10 quintuple-layer film, suggesting the influence of the film thickness on the dissipative edge channel in the QAHE regime. The extension of QAHE into the three-dimensional thickness region addresses the universality of this quantum transport phenomenon and motivates the exploration of new QAHE phases with tunable Chern numbers.In addition, the observation of the scale-invariant dissipationless chiral propagation on a macroscopic scale makes a major stride towards ideal low-power interconnect applications.

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Electric-field manipulation of magnetic order has proved of both fundamental and technological importance in spintronic devices. So far, electric-field control of ferromagnetism, magnetization and magnetic anisotropy has been explored in various magnetic materials, but the efficient electric-field control of spin-orbit torque (SOT) still remains elusive. Here, we report the effective electric-field control of a giant SOT in a Cr-doped topological insulator (TI) thin film using a top-gate field-effect transistor structure. The SOT strength can be modulated by a factor of four within the accessible gate voltage range, and it shows strong correlation with the spin-polarized surface current in the film. Furthermore, we demonstrate the magnetization switching by scanning gate voltage with constant current and in-plane magnetic field applied in the film. The effective electric-field control of SOT and the giant spin-torque efficiency in Cr-doped TI may lead to the development of energy-efficient gate-controlled spin-torque devices compatible with modern field-effect semiconductor technologies.

Strong spin−orbit interaction and time-reversal symmetry in topological insulators enable the spin-momentum locking for the helical surface states. To date, however, there has been little report of direct electrical spin injection/ detection in topological insulator. In this Letter, we report the electrical detection of spin-polarized surface states conduction using a Co/Al 2 O 3 ferromagnetic tunneling contact in which the compound topological insulator (Bi 0.53 Sb 0.47 ) 2 Te 3 was used to achieve low bulk carrier density. Resistance (voltage) hysteresis with the amplitude up to about 10 Ω was observed when sweeping the magnetic field to change the relative orientation between the Co electrode magnetization and the spin polarization of surface states. The two resistance states were reversible by changing the electric current direction, affirming the spin-momentum locking in the topological surface states. Angle-dependent measurement was also performed to further confirm that the abrupt change in the voltage (resistance) was associated with the magnetization switching of the Co electrode. The spin voltage amplitude was quantitatively analyzed to yield an effective spin polarization of 1.02% for the surface states conduction in (Bi 0.53 Sb 0.47 ) 2 Te 3 . Our results show a direct evidence of spin polarization in the topological surface states conduction. It might open up great opportunities to explore energy-efficient spintronic devices based on topological insulators. KEYWORDS: Topological insulator, spin polarization, surface states, spin-momentum locking, spin detection S ince the discovery of two-dimensional (2D) and threedimensional (3D) topological insulators (TIs), 1−5 they have attracted extensive research interest for their exotic physical properties that could lead to dissipationless transport in the quantum spin Hall state. 6−9 Recent studies have shown a giant spin−orbit torque in TI originating from the strong spin− orbit interaction, 10,11 which enabled the current-induced magnetization switching through spin-transfer torque with a low current density. The unique feature of 3D TI, for instance, is that it has both insulating bulk and gapless Dirac surface states. 8,9 Ternary TI compounds, such as (Bi x Sb 1−x ) 2 Te 3 , have been widely investigated for their tunability to achieve low bulk carrier density and manifest topological surface states conduction. 12,13 The presence of surface states is supported by extensive angle-resolved photoemission spectroscopy (ARPES) measurements and transport studies, 14−20 such as Shubnikov-de Haas (SdH) and Aharonov Bohm (AB) quantum oscillations. Because of the strong spin−orbital interaction in TI, direct back scatterings from nonmagnetic impurities are prohibited by the time-reversal symmetry. 8,9 More importantly, the spin-momentum locking naturally leads to a currentinduced spin polarization in surface states; 21 the surface states conduction is spin-polarized once an electric current is passed through a TI film, and this spin polarization can be...

Introducing magnetic order in a topological insulator (TI) breaks time-reversal symmetry of the surface states and can thus yield a variety of interesting physics and promises for novel spintronic devices. To date, however, magnetic effects in TIs have been demonstrated only at temperatures far below those needed for practical applications. In this work, we study the magnetic properties of Bi2Se3 surface states (SS) in the proximity of a high Tc ferrimagnetic insulator (FMI), yttrium iron garnet (YIG or Y3Fe5O12). Proximity-induced butterfly and square-shaped magnetoresistance loops are observed by magneto-transport measurements with out-of-plane and in-plane fields, respectively, and can be correlated with the magnetization of the YIG substrate. More importantly, a magnetic signal from the Bi2Se3 up to 130 K is clearly observed by magneto-optical Kerr effect measurements. Our results demonstrate the proximity-induced TI magnetism at higher temperatures, an important step toward room-temperature application of TI-based spintronic devices.