Switching a polymer Electrically switchable metasurfaces and plasmonic materials will enable the development of active nanophotonic technology. Karst et al . show that a metallic polymer can be used for electrical switching of plasmonic nanoantenna resonances. The plasmonic resonance can be completely switched ON and OFF with switching speeds up to 30 hertz (video rate), low switching voltages of ±1 volt (complementary metal-oxide semiconductor compatible), and a switching contrast of 100%. The results could have applications in nanophotonic devices such as those used in augmented and virtual reality imaging applications. —ISO
Switchable metasurfaces can actively control the functionality of integrated metadevices with high efficiency and on ultra-small length scales. Such metadevices include active lenses, dynamic diffractive optical elements, or switchable holograms. Especially, for applications in emerging technologies such as AR (augmented reality) and VR (virtual reality) devices, sophisticated metaoptics with unique functionalities are crucially important. In particular, metaoptics which can be switched electrically on or off will allow to change the routing, focusing, or functionality in general of miniaturized optical components on demand. Here, we demonstrate metalenses-on-demand made from metallic polymer plasmonic nanoantennas which are electrically switchable at CMOS (complementary metal-oxide-semiconductor) compatible voltages of ±1 V. The nanoantennas exhibit plasmonic resonances which can be reversibly switched ON and OFF via the applied voltage, utilizing the optical metal-to-insulator transition of the metallic polymer. Ultimately, we realize an electro-active non-volatile multi-functional metaobjective composed of two metalenses, whose unique optical states can be set on demand. Overall, our work opens up the possibility for a new level of electro-optical elements for ultra-compact photonic integration.
We introduce an extremely simple and highly stable system for stimulated Raman scattering (SRS) microscopy. An 8-W, 450-fs Yb:KGW bulk oscillator with 41 MHz repetition rate pumps an optical parametric amplifier, which is seeded by a cw tunable external cavity diode laser. The output radiation is frequency doubled in a long PPLN crystal and generates 1.5-ps long narrowband pump pulses that are tunable between 760 and 820 nm with >50 mW average power. Part of the oscillator output is sent through an etalon and creates Stokes pulses with 100 mW average power and 1.7 ps duration. We demonstrate SRS microscopy at a 30-μs pixel dwell time with high chemical contrast, signal-to-noise ratio in excess of 45 and no need for balanced detection, thanks to the favorable noise properties of the bulk solid-state system. Cw seeding intrinsically ensures low spectral drift. We discuss its application to chemical contrast microscopy of freshly prepared plant tissue sections at different vibrational bands.
We present an electrically switchable, compact metasurface device based on the metallic polymer PEDOT:PSS in combination with a gel polymer electrolyte. Applying square-wave voltages, we can reversibly switch the PEDOT:PSS from dielectric to metallic. Using this concept, we demonstrate a compact, standalone, and CMOS compatible metadevice. It allows for electrically controlled ON and OFF switching of plasmonic resonances in the 2–3 µm wavelength range, as well as electrically controlled beam switching at angles up to 10°. Furthermore, switching frequencies of up to 10 Hz, with oxidation times as fast as 42 ms and reduction times of 57 ms, are demonstrated. Our work provides the basis towards solid state switchable metasurfaces, ultimately leading to submicrometer-pixel spatial light modulators and hence switchable holographic devices.
In multiphoton 3D direct laser writing and stimulated Raman scattering applications, rapid and arbitrary pulse modulation with an extremely high contrast ratio would be very beneficial. Here, we demonstrate a femtosecond fiber-feedback optical parametric oscillator (FFOPO) system in combination with pulse picking in the pump beam. This allows tunable signal output at variable burst rates from DC all the way up to 5 MHz. Furthermore, arbitrary pulse sequences can be generated. The rapid signal buildup dynamics provide individual full-power pulses with only two prepulses. This is possible without the requirement for additional injection seeding. Hereby, the intrinsically high intra-cavity losses of the FFOPO system are found to beneficial, as they enable rapid off-switching of the output as signal ring-down is efficiently suppressed. Possible applications are the reduction of the average power while maintaining a high peak power level, as well as tunable arbitrary pulse sequence generation.
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