Natural gas demand has dramatically increased due to the emerging growth of the world economy and industry. Presently, CO2 and H2S content in gas fields accounts for up to 90% and 15%, respectively. Apart from fulfilling the market demand, CO2 and H2S removal from natural gas is critical due to their corrosive natures, the low heating value of natural gas and the greenhouse gas effect. To date, several gas fields have remained unexplored due to limited technologies to monetize the highly sour natural gas. A variety of conventional technologies have been implemented to purify natural gas such as absorption, adsorption and membrane and cryogenic separation. The application of these technologies in natural gas upgrading are also presented. Among these commercial technologies, cryogenic technology has advanced rapidly in gas separation and proven ideally suitable for bulk CO2 removal due to its independence from absorbents or adsorbents, which require a larger footprint, weight and energy. Present work comprehensively reviews the mechanisms and potential of the advanced nonconventional cryogenic separation technologies for processing of natural gas streams with high CO2 and H2S content. Moreover, the prospects of emerging cryogenic technologies for future commercialization exploitation are highlighted.
It is estimated that 40% of natural gas reservoirs in the world are contaminated with acid gases (such as hydrogen sulfide and carbon dioxide), which hinder exploitation activities. The demand for natural gas will increase by 30% from 2020 to 2050, with the rise of industrial activities and the lifting of travel restrictions. The long-term production of these high acid-gas fields requires mitigation plans, which include carbon capture, utilization, and a storage process to reduce carbon emissions. Absorption is one the most established technologies for CO2 capture, yet it suffers from extensive energy regeneration and footprint requirements in offshore operations. Therefore, the aims of this paper are to review and analyze the recent developments in conventional and emerging solvent regeneration technologies, which include a conventional packed-bed column, membrane contactor, microwave heating, flash drum, rotating packed bed, and ultrasonic irradiation process. The conventional packed column and flash drum are less complex, with minimum maintenance requirements, but suffer from a large footprint. Even though the rotating packed-bed column and microwave heating demonstrate a higher solvent flexibility and process stability, both technologies require regular maintenance and high regeneration energy. Membrane contactor and ultrasonic irradiation absorption systems are compact, but restricted by various operational issues.
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