All-dielectric optical metasurfaces are a workhorse in nano-optics, because of both their ability to manipulate light in different degrees of freedom and their excellent performance at light frequency conversion. Here, we demonstrate first-time generation of photon pairs via spontaneous parametric-down conversion in lithium niobate quantum optical metasurfaces with electric and magnetic Mie-like resonances at various wavelengths. By engineering the quantum optical metasurface, we tailor the photon-pair spectrum in a controlled way. Within a narrow bandwidth around the resonance, the rate of pair production is enhanced up to 2 orders of magnitude, compared to an unpatterned film of the same thickness and material. These results enable flat-optics sources of entangled photons—a new promising platform for quantum optics experiments.

Lithium niobate is an excellent and widely used material for nonlinear frequency conversion due to its strong optical nonlinearity and broad transparency region. Here, we report the fabrication and experimental investigation of resonant nonlinear metasurfaces for second-harmonic generation based on thin-film lithium niobate. In the fabricated metasurfaces, we observe pronounced Mie-type resonances leading to enhanced second-harmonic generation in the direction normal to the metasurface. We find the largest second-harmonic generation efficiency for the resonance dominated by the electric contributions because its specific field distribution enables the most efficient usage of the largest element of the lithium niobate nonlinear susceptibility tensor. This is confirmed by polarization-resolved second-harmonic measurements, where we study contributions from different elements of the nonlinear susceptibility tensor to the total second-harmonic signal. Our work facilitates establishing lithium niobate as a material for resonant nanophotonics.

We present our experimental results on electric field poling of X-cut thin-film lithium niobate with poling periods of 1–4 µm. We used polarization contrast microscopy combined with digital image processing to study the impact of the experimental parameters of the poling process such as electric field strength, poling pulse duration, and layout of metal electrodes on the domain growth and quality of resulting poling patterns. High-quality results with excellent homogeneity of the domain pattern on large areas [i.e., 16 µm along the domain ( z axis) and millimeter long domain gratings along the y axis with a period down to 1 µm] allow for the integration of numerous devices and structures.

In this work, we present a systematic experimental study of surface electric field poling for creating periodically poled lithium niobate. We want to control the homogeneity and the duty cycle of the periodic structures as well as domain shape and size in general. The created domain patterns are analyzed by selective etching with subsequent scanning electron microscopy. We investigate theoretically and experimentally how the shape of electrodes influences the poling results. Furthermore, the influence of the temporal waveform and magnitude of the applied poling voltage pulse is studied. Our results enable to identify optimal experimental parameters for high-quality surface poling.

We demonstrate resonant metasurfaces with spatially engineered nonlinearity based on periodically poled lithium niobate. Such spatial control of the nonlinearity unlocks additional degrees of freedom for controlling the properties of second-harmonic radiation from metasurfaces.

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Sources of spectrally engineered photonic states are a key resource in several quantum technologies. Of particular importance are the so-called factorizable biphoton states, which possess no spectral entanglement and hence, are ideal for heralded generation of high-purity single photons. An essential prerequisite for generating these states through nonlinear frequency conversion is the control over the group indices of the photonic modes of the source. Here, we show that thin-film lithium niobate on insulator (LNOI) is an excellent platform for this purpose. We design and fabricate periodically poled ridge waveguides in LNOI to demonstrate group index engineering of its guided photonic modes and harness this control to experimentally realize on-chip group index matched type-II sum-frequency generation (SFG). Also, we numerically study the role of the top cladding layer in tuning the dispersion properties of the ridge waveguide structures and reveal a distinctive difference between the air and silica-clad designs which are currently among the two most common device cladding configurations in LNOI. We expect that these results will be relevant for various classical and quantum applications where dispersion control is crucial in tailoring the nonlinear response of the LNOI-based devices.

Sources of spectrally engineered photonic states are a key resource in several quantum technologies. Of particular importance are the so-called factorizable biphoton states which possess no spectral entanglement and hence, are ideal for heralded generation of high-purity single photons. An essential prerequisite for generating these states through nonlinear frequency conversion is the control over the group indices of the photonic modes of the source. Here, we show that thin-film lithium niobate on insulator (LNOI) is an excellent platform for this purpose. We design and fabricate periodically poled ridge waveguides in LNOI to demonstrate group index engineering of its guided photonic modes and harness this control to experimentally realize on-chip group index matched type-II sum-frequency generation (SFG) and photon-pair creation through spontaneous parametric down-conversion (SPDC). Also, we numerically study the role of the top cladding layer in tuning the dispersion properties of the ridge waveguide structures and reveal a distinctive difference between the air and silica-clad designs which are currently among the two most common device cladding configurations in LNOI. We expect that these results will be relevant for various classical and quantum applications where dispersion control is crucial in tailoring the nonlinear response of the LNOIbased devices.