The quality of rainwater from a tile and a galvanized-iron type roof catchments were analysed over a period of 5 months. Examination of staggered I litre samples collected during a rainfall event showed that the concentration of various pollutants were high in the first litre but decreased in subsequent samples with few exceptions. Faecal coliform and total coliform counts ranged from 8-13 (tile roof) and 4-8 (iron roof) to 41-75 (tile roof) and 25-63 (iron roof) colonies per 100 ml, respectively. However, no faecal coliforms were detected in the fourth and fifth litre samples from both roofs. The pH of rainwater collected from the open was acidic but increased slightly after falling on the roofs. The average zinc concentrations in the run-off from the galvanized-iron roof was about 5-fold higher compared to the tile roof, indicating leaching action but was well below the WHO limits for drinking water quality. Lead concentrations remained consistently high in all samples collected and exceeded the WHO guidelines by a factor of 3.5. For the roof area studied, a "foul flush" volume of 51. would be the minimum to safeguard against microbiological contamination but the high metals content in the water indicate the need for some form of treatment. Rainfall intensity and the number of dry days preceeding a rainfall event significantly affects the quality of runoff water from the catchment systems.

Four anoxic sediment cores were collected from Chini Lake, Malaysia in order to investigate the variability of polycyclic aromatic hydrocarbon (PAH) and perylene concentrations. The study also determined significant differences of perylene concentrations in different sediment layers. Total PAH concentrations ranged from 248 to 8098 ng g−1 in the samples. Diagnostic PAH ratios such as methylphenanthrenes/phenanthrene (MP/P), phenanthrene/anthracene (P/A) and fluoranthene/(fluoranthene + pyrene) (Fl/(Fl + Py) revealed a dominance of pyrogenic influences and partial petrogenic inputs to the top sediment layers. Perylene concentrations were high in the top layers (<12 cm) and increased with increasing depth. There is a significant positive correlation (r = 0.705, p = 0.01) between perylene concentrations and TOC. Analysis of variance (ANOVA) and LSD revealed significant differences (p < 0.05) in TOC-normalized perylene concentrations between the upper (<12 cm) and bottom layers (>12 cm). The average perylene concentrations accounted for 26-50% (0-12 cm) and 50-77% (12-36 cm) of pentacyclic-aromatic hydrocarbon isomers (PAI) present whereas it made up 10-34% (0-12 cm) and 46-66% (12-36 cm) of the total PAH. The average pyrene concentrations decreased with increasing depth and accounted for 62% (0-3 cm), 20-23% (3-12 cm) and 3-1.4% (12-36 cm) of perylene present. The results of hierarchical cluster analysis based on these ratios suggested different input sources for the top and bottom layers. It is concluded that the activity of termites on woody plants produced perylene which is supplied to the lake by runoff from the heavy and frequent rains in this Asian tropical climate. In addition, there was also in situ formation of perylene in the bottom layers due to diagenetic processes.

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The numbers of salmonellas in raw sewage entering a treatment plant varied hourly and diurnally; their peak concentration preceded the peak influent waste water flow into the plant by about 2 hours. Salmonellas were detected in all raw influent samples collected from 2 sewage works and the mean population level at the daily peak period was 3000 organisms/1. On average. 70–80% of the salmonellas were removed during primary sedimentation when upwards of 74–84% of solids were removed. Biological treatment and secondary sedimentation removed a further 70–100% of the pathogen. Compared with the activated sludge process the trickling filters were less efficient in removing salmonellas and they were adversely affected by increased loading following rainfall. Considering the whole treatment process, the Guildford works with its activated sludge treatment removed an average of 99–83% salmonellas while the Woking works with its trickling filter plant removed an average of 93–04% of the organisms. The large variance in the numbers of salmonellas in the final effluent from the trickling filters suggest that greater emphasis should be placed on the actual quality of the effluent rather than on percentage removal efficiencies.

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Salmonella destruction efficiencies of 99% were obtained after 10 h aeration at 15°C in a laboratory model of the activated sludge process. This study demonstrated that, in a batch process, the removal of salmonellas occurred in three phases. (i) By 4 h, 90% of the original inoculum had disappeared from the activated sludge, probably due mainly to predation by ciliated protozoa. The remaining 10% was distributed between the liquid phase (approximately 90%) and the sludge floc (approximately 10%). (ii) During the next 2 h this situation was inverted so that, by 6 h, more than 80% of the remaining salmonellas were then adsorbed to floc, leaving less than 20% in liquid suspension. (iii) From 6 h onwards there was a much slower decline of the remaining salmonellas attached to floc. The addition of dioctyl sodium sulphosuccinate after 4 h, inactivated the ciliated protozoa populations and completely eliminated the continued reduction of salmonellas from activated sludge observed previously.

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