Brillouin spectroscopy has been widely used for the investigation of acoustic properties of condensed matters in the hypersonic region. A high-pressure Brillouin spectrometer was set up by combining a diamond anvil cell and a tandem multi-pass Fabry-Perot interferometer. It was successfully applied to liquid ethanol, and the pressure dependence of the sound velocity, the refractive index and other acoustic properties were derived based on the measurements. The detailed optical setup and experimental procedure are described.
Well-established microfabrication techniques are employed to demonstrate a new architecture of metal grids made of metal nanowire networks for flexible and transparent conductive electrode applications.
Acoustic properties of antiferroelectric (AFE) PbZr 0.72 Sn 0.28 O 3 single crystals were investigated in a wide temperature range by Brillouin light scattering spectroscopy. The Brillouin frequency shift of the longitudinal acoustic (LA) mode exhibited three abrupt changes corresponding to the successive phase transitions between the paraelectric, intermediate, antiferroelectric (AFE2) and antiferroelectric (AFE1) phases upon cooling. The change in the LA mode frequency and the damping maximum of PbZr 0.72 Sn 0.28 O 3 were much higher than those of pure PbZrO 3 . This was attributed to enhanced polarization fluctuations caused by increased ferroelectric distortions due to Sn substitution and the proximity to the tricritical point on the phase diagram of PbZr 1-x Sn x O 3 .
Green electronics based on biodegradable polymers have received considerable attention as a solution to electronic waste (e-waste). Herein, we describe an efficient approach to constructing green conductive fibers, comprising poly(3,4-ethylenedioxythiophene) (PEDOT) and regenerated cellulose (RC), via a wet-spinning process and vapor-phase polymerization (VPP). Eco-friendly RC fibers were prepared as a support layer by wet spinning, and the conductive PEDOT layers were coated onto the surface of the RC fibers by the oxidation of EDOT monomers. We demonstrated that the vapor-phase-polymerized PEDOT/RC composite fibers (PEDOT/RC-VPP) exhibited approximately 17 times higher electrical conductivity (198.2 ± 7.3 S/cm), compared with that of the solution-phase-polymerized PEDOT/RC composite fibers (PEDOT/RC-SPP, 11.6 ± 0.6 S/cm). Importantly, PEDOT/RC-VPP exhibited a high tensile strength of 181 MPa, good flexibility, and long-standing electrical stability under ambient air conditions. Moreover, the obtained PEDOT/RC-VPP under 50% strain turned on a green light-emitting diode (LED), indicating the flexibility and stability of green conductive fibers. This strategy can be easily integrated into various electronic textiles for the development of next-generation wearable green electronics.
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