Organic-inorganic perovskites are a class of solution-processed semiconductors holding promise for the realization of low-cost efficient solar cells and on-chip lasers. Despite the recent attention they have attracted, fundamental aspects of the photophysics underlying device operation still remain elusive. Here we use photoluminescence and transmission spectroscopy to show that photoexcitations give rise to a conducting plasma of unbound but Coulomb-correlated electron-hole pairs at all excitations of interest for light-energy conversion and stimulated optical amplification. The conductive nature of the photoexcited plasma has crucial consequences for perovskite-based devices: in solar cells, it ensures efficient charge separation and ambipolar transport while, concerning lasing, it provides a low threshold for light amplification and justifies a favourable outlook for the demonstration of an electrically driven laser. We find a significant trap density, whose cross-section for carrier capture is however low, yielding a minor impact on device performance.
Bose-Einstein condensates of sodium atoms, prepared in an optical dipole trap, were distilled into a second empty dipole trap adjacent to the first one. The distillation was driven by thermal atoms spilling over the potential barrier separating the two wells and then forming a new condensate. This process serves as a model system for metastability in condensates, provides a test for quantum kinetic theories of condensate formation, and also represents a novel technique for creating or replenishing condensates in new locations.PACS numbers: 03.75.Lm, 64.60.My The characteristic feature of Bose-Einstein condensation is the accumulation of a macroscopic number of particles in the lowest quantum state. Condensate fragmentation, the macroscopic occupation of two or more quantum states, is usually prevented by interactions [1], but may happen in spinor condensates [2,3]. However, multiple condensates may exist in metastable situations. Let's assume that an equilibrium condensate has formed in one quantum state, but now we modify the system allowing for one even lower state. How does the original condensate realize that it is in the wrong state and eventually migrate to the true ground state of the system? What determines the time scale for this equilibration process? This is the situation which we experimentally explore in this paper using a double-well potential.The process we study is relevant for at least four different questions.(1) The description of the formation of the condensate is a current theoretical frontier and requires finite-temperature quantum kinetic theories. There are still discrepancies between theoretical predictions and experimental results [4,5]. Our double-well system has the advantage of being an almost closed system (little evaporation) with well defined initial conditions and widely adjustable time scales (through the height of the barrier). (2) Spinor condensates show rich ground states and collective excitations due to the multi-component order parameter [2]. Several groups have observed longlived metastable configurations [6,7,8,9] and speculated about transport of atoms from one domain to another via the thermal cloud [6,8]. The double-well potential allows us to characterize such distillation processes in their simplest realization. (3) The incoherent transport observed here in a double well-potential imposes stringent limitations on future experiments aiming at the observation of coherent transport in Josephson junctions [10,11,12]. (4) Our observation of condensate growth in one potential well due to the addition of thermal atoms realizes the key ideas of proposals on how to achieve a continuous atom laser [13] which is different from the experiment where condensates were replenished with transported condensates [14]. The whole system has equilibrated. V denotes the height of the potential barrier between the two wells, which is measured with respect to the bottom of the left well, and ∆U the trap depth difference between the two wells.The scheme of the experiment is shown in Fig....
Cavity polaritons, the elementary optical excitations of semiconductor microcavities, may be understood as a superposition of excitons and cavity photons. Owing to their composite nature, these bosonic particles have a distinct optical response, at the same time very fast and highly nonlinear. Very efficient light amplification due to polariton-polariton parametric scattering has recently been reported in semiconductor microcavities at liquid-helium temperatures. Here we demonstrate polariton parametric amplification up to 120 K in GaAlAs-based microcavities and up to 220 K in CdTe-based microcavities. We show that the cut-off temperature for the amplification is ultimately determined by the binding energy of the exciton. A 5-micrometer-thick planar microcavity can amplify a weak light pulse more than 5,000 times. The effective gain coefficient of an equivalent homogeneous medium would be 107 cm-1. The subpicosecond duration and high efficiency of the amplification could be exploited for high-repetition all-optical microscopic switches and amplifiers. 105 polaritons occupy the same quantum state during the amplification, realizing a dynamical condensate of strongly interacting bosons which can be studied at high temperature.
We measure the relative phase of two Bose-Einstein condensates confined in a radio frequency induced double-well potential on an atom chip. We observe phase coherence between the separated condensates for times up to approximately 200 ms after splitting, a factor of 10 longer than the phase diffusion time expected for a coherent state for our experimental conditions. The enhanced coherence time is attributed to number squeezing of the initial state by a factor of 10. In addition, we demonstrate a rotationally sensitive (Sagnac) geometry for a guided atom interferometer by propagating the split condensates.
A trapped-atom interferometer was demonstrated using gaseous Bose-Einstein condensates coherently split by deforming an optical single-well potential into a double-well potential. The relative phase between the two condensates was determined from the spatial phase of the matter wave interference pattern formed upon releasing the condensates from the separated potential wells. Coherent phase evolution was observed for condensates held separated by 13 µm for up to 5 ms and was controlled by applying ac Stark shift potentials to either of the two separated condensates.PACS numbers: 03.75. Dg, 39.20.+q, 03.75.Lm Demonstrating atom interferometry with particles confined by magnetic [1,2,3,4] and optical [5] microtraps and waveguides would realize the matter wave analog of optical interferometry using fiber-optic devices. Current proposals for confined-atom interferometers rely on the merger and separation of two potential wells to coherently divide atomic wavepackets [6,7,8]. This type of division differs from previously demonstrated atomic beam splitters. To date, atomic beams and vapors have been coherently diffracted into different momentum states by mechanical [9,10] and optical [11] gratings, and Bose-Einstein condensates have been coherently delocalized over multiple sites in optical lattices [12,13,14,15,16,17]. Atom interferometers utilizing these beam splitting elements have been used to sense accelerations [12,18] and rotations [19,20], monitor quantum decoherence [21], characterize atomic and molecular properties [22], and measure fundamental constants [18,23].In this Letter, we demonstrate a trapped-atom interferometer with gaseous Bose-Einstein condensates confined in an optical double-well potential. Condensates were coherently split by deforming an initially single-well potential into two wells separated by 13 µm. The relative phase between the two condensates was determined from the spatial phase of the matter wave interference pattern formed upon releasing the atoms from the separated potential wells [17,24]. This recombination method avoids deleterious mean field effects [25,26] and detects applied phase shifts on a single realization of the experiment, unlike in-trap recombination schemes [6,7,8].The large separation between the split potential wells allowed the phase of each condensate to evolve independently and either condensate to be addressed individually. An ac Stark phase shift was applied to either condensate by temporarily turning off the optical fields generating its potential well. The spatial phase of the resulting matter wave interference pattern shifted linearly with the applied phase shift and was independent of the time of its application. This verified the phase sensitivity of the interferometer and the independent phase evolution of the separated condensates. The measured coherence time of the separated condensates was 5 ms.The present work demonstrates a trapped-atom interferometer with two interfering paths. This geometry has the flexibility to measure either highly localized...
Doubly quantized vortices were topologically imprinted in |F = 1 23 Na condensates, and their time evolution was observed using a tomographic imaging technique. The decay into two singly quantized vortices was characterized and attributed to dynamical instability. The time scale of the splitting process was found to be longer at higher atom density.PACS numbers: 03.75. Kk, 03.75.Lm, 67.90.+z Quantum fluids, like superfluid He, electrons in a superconductor or a Bose-Einstein condensate of atoms, are described by a macroscopic wavefunction. This requires the flow field to be irrotational, and gives rise to superfluidity and quantized circulation [1]. Atoms in a BoseEinstein condensate, for example, can only circulate with angular momentum equal to integer multiple ofh, in the form of a quantized vortex [2].Vortices are excited states of motion and therefore energetically unstable towards relaxation into the motional ground state, where the condensate is at rest. However, quantization constrains the decay: a vortex in BoseEinstein condensates cannot simply fade away or disappear, it is only allowed to move out of the condensate or annihilate with another vortex of opposite circulation. Vortex decay and metastability, due to inhibition of decay, have been a central issue in the study of superfluidity [3,4,5,6,7,8]. In almost pure Bose-Einstein condensates, vortices with lifetimes up to tens of seconds have been observed [9,10,11].Giving a Bose-Einstein condensate angular momentum per particle larger thanh can result in one multiplyquantized vortex with large circulation or, alternatively, in many singly-quantized vortices each with angular momentumh. The kinetic energy of atoms circulating around the vortex is proportional to the square of the angular momentum; therefore the kinetic energy associated with the presence of a multiply-quantized vortex is larger than the kinetic energy of a collection of singlyquantized vortices carrying the same angular momentum. A multiply-quantized vortex can decay coherently by splitting into singly-quantized vortices and transferring the kinetic energy to coherent excitation modes, a phenomenon called dynamical instability which is driven by atomic interactions [5,12,13,14], and not caused by dissipation in an external bath. Observations of arrays of singly-quantized vortices in rapidly rotating condensates [10,11] indirectly suggests that the dynamical instability leads to fast decay of multiply-quantized vortices. However, the existence of stable multiply-quantized vortices in trapped Bose-Einstein condensates has been predicted with a localized pinning potential [12] or in a quartic potential [15]. Stable doubly-quantized vortices were observed in superconductors in presence of pinning forces [16] and in superfluid 3 He-A which has a multicomponent order parameter [17]. Recently, formation of a multiply-quantized vortex in a Bose-Einstein condensate has been demonstrated using topological phases [18,19], and surprisingly long lifetime of a "giant" vortex core has been report...
Spin-polarized gaseous Bose-Einstein condensates were confined by a combination of gravitational and magnetic forces. The partially condensed atomic vapors were adiabatically decompressed by weakening the gravito-magnetic trap to a mean frequency of 1hertz, then evaporatively reduced in size to 2500 atoms. This lowered the peak condensate density to 5 x 10(10) atoms per cubic centimeter and cooled the entire cloud in all three dimensions to a kinetic temperature of 450 +/- 80 picokelvin. Such spin-polarized, dilute, and ultracold gases are important for spectroscopy, metrology, and atom optics.
We observed quantum reflection of ultracold atoms from the attractive potential of a solid surface. Extremely dilute Bose-Einstein condensates of 23Na, with peak density 10(11)-10(12) atoms/cm(3), confined in a weak gravitomagnetic trap were normally incident on a silicon surface. Reflection probabilities of up to 20% were observed for incident velocities of 1-8 mm/s. The velocity dependence agrees qualitatively with the prediction for quantum reflection from the attractive Casimir-Polder potential. Atoms confined in a harmonic trap divided in half by a solid surface exhibited extended lifetime due to quantum reflection from the surface, implying a reflection probability above 50%.
scite is a Brooklyn-based organization that helps researchers better discover and understand research articles through Smart Citations–citations that display the context of the citation and describe whether the article provides supporting or contrasting evidence. scite is used by students and researchers from around the world and is funded in part by the National Science Foundation and the National Institute on Drug Abuse of the National Institutes of Health.
hi@scite.ai
10624 S. Eastern Ave., Ste. A-614
Henderson, NV 89052, USA
Copyright © 2024 scite LLC. All rights reserved.
Made with 💙 for researchers
Part of the Research Solutions Family.