No abstract

a b s t r a c tThe transient injection and subsequent auto-ignition of a methane jet issuing into a laminar coflow of hot exhaust gas from a lean premixed hydrogen air flame was studied using high-speed planar Rayleigh scattering, yielding two-dimensional measurements of mixture fraction, temperature and scalar dissipation rate with high spatio-temporal resolution. The temporal development of the mixing field between the transient fuel jet and the surrounding coflow prior to the occurrence of auto-ignition was examined at a sampling rate of 10 kHz. The impact of the transient jet development on numerical modeling of this test case is discussed. It was found that auto-ignition occurred after the jet transitioned from a transient state into the steady state, thus eliminating the need to model the complete transient fuel injection when the primary focus is on the onset of auto-ignition.Simultaneous high-speed OH * chemiluminescence from two viewing angles was applied to gain 3D-information of the ignition kernel location. This information allowed the selection and analysis of ignition events where the initial kernel formed inside the laser light sheet. Detailed analysis of the dynamics of a single ignition event, as well as statistical analysis of multiple ignition events based on a joint probability density approach, indicated that the ignition kernels occurred at very lean mixture fractions and at locations with low scalar dissipation rates.

In this manuscript we describe an experimental approach to simultaneously measure high-speed image sequences of the mixture fraction and temperature fields during pulsed, turbulent fuel injection into a high-temperature, co-flowing, and vitiated oxidizer stream. The quantitative mixture fraction and temperature measurements are determined from 10-kHz-rate planar Rayleigh scattering and a robust data processing methodology which is accurate from fuel injection to the onset of auto-ignition. In addition, the data processing is shown to yield accurate temperature measurements following ignition to observe the initial evolution of the "burning" temperature field. High-speed OH* chemiluminescence (CL) was used to determine the spatial location of the initial auto-ignition kernel. In order to ensure that the ignition kernel formed inside of the Rayleigh scattering laser light sheet, OH* CL was observed in two viewing planes, one near-parallel to the laser sheet and one perpendicular to the laser sheet. The highspeed laser measurements are enabled through the use of the unique high-energy pulse burst laser system (HEPBLS) which generates long-duration bursts of ultra-high pulse energies at 532 nm (> 1 Joule) suitable for planar Rayleigh scattering imaging. A particular focus of this study was to characterize the fidelity of the measurements both in the context of the precision and accuracy, which includes facility operating and boundary conditions and measurement signal-to-noise (SNR). The mixture fraction and temperature fields deduced from the high-speed planar Rayleigh scattering measurements exhibited SNR values greater than 100 at temperatures exceeding 1300 K. The accuracy of the measurements was determined by comparing the current mixture fraction results to that of "cold", isothermal, non-reacting jets. All profiles, when properly normalized exhibited self-similarity and collapsed upon one another. Finally, example mixture fraction, temperature, and OH* emission sequences are presented for a variety for fuel and vitiated oxidizer combinations. For all cases considered, auto-ignition occurred at the periphery of the fuel jet, under very "lean" conditions, where the local mixture fraction was less than the stoichiometric mixture fraction ( <  s). Furthermore, the ignition kernel formed in regions of low scalar dissipation rate, which agrees with previous results from direct numerical simulations.

This Letter presents results from a new master-oscillator, power-amplifier pulse-burst laser system demonstrating ultrahigh pulse energies greater than 2.0 J/pulse at 1064 nm with interpulse separations of 100 μs (10 kHz) for burst durations of 100 pulses. Each pulse generates peak powers exceeding 130 MW and an average power of approximately 20 kW is generated over a 100-pulse-burst. Pulse energies decrease by less than 10% over a 100 sequential pulses, demonstrating negligible "droop" over long-duration pulse trains. Second-harmonic generation of 532 nm with conversion efficiency greater than 50% is demonstrated for 100-pulse-burst durations.

Auto-ignition is a complex process which is extremely sensitive to boundary conditions such as local temperature, mixture or strain rate and occurs on very short timescales. Therefore, measurement techniques with high spatio-temporal resolution have to be applied to test cases with well-defined boundary conditions in order to generate high-quality validation data for numerical simulations. In the current paper, the auto-ignition of a transient propane jet-in-hot coflow was studied with high-speed OH* chemiluminescence imaging and high-speed Rayleigh scattering for the simultaneous determination of mixture fraction, mixture temperature and scalar dissipation rate immediately prior to the onset of auto-ignition. A variation of the coflow temperature showed a pronounced temperature dependence of the auto-ignition location and time, and the temperature sensitivity was higher than for a comparable methane test case from the literature. This is explained by the lower sensitivity of propane ignition delay times to the local strain rate in comparison to methane. The Rayleigh measurements however showed that the formation mechanism of auto-ignition kernels is similar for propane and methane. Ignition kernels were found to form upstream of bulges of the inflowing jet at locations with locally low scalar dissipation rate.