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The aerosols harboring microorganisms and viruses released from the wastewater system into the air have greatly threatened the health and safety of human beings. The wastewater systems, including toilet and wastewater treatment plant (WWTP), are the major locations of epidemic infections due to the extensive sources of aerosols, as well as multifarious germs and microorganisms. Viruses and microorganisms may transport from both toilet and hospital into municipal pipes and subsequently into WWTP, which accounts for the main source of bioaerosols dispersed in the air of the wastewater system. This review aims to elaborate the generation, transmission, and diffusion processes of bioaerosols at toilet and WWTP. Moreover, the main factors affecting bioaerosol transmission and the corresponding prevention strategies for the airborne and inhaled bioaerosols are also discussed. Collectively, this review highlights the importance of managing bioaerosol occurrence in the wastewater system, which has aroused increasing concern from the public.

Metal-phenol coordination is a widely used method to prepare nanofiltration membrane. However, the facile, controllable and scaled fabrication remains a great challenge. Herein, a novel strategy was developed to fabricate a loose nanofiltration membrane via integrating blending and interfacial coordination strategy. Specifically, iron acetylacetonate was firstly blended in Polyether sulfone (PES) substrate via non-solvent induced phase separation (NIPS), and then the loose selective layer was formed on the membrane surface with tannic acid (TA) crosslinking reaction with Fe3+. The surface properties, morphologies, permeability and selectivity of the membranes were carefully investigated. The introduction of TA improved the surface hydrophilicity and negative charge. Moreover, the thickness of top layer increased about from ~30 nm to 119 nm with the increase of TA assembly time. Under the optimum preparation condition, the membrane with assembly 3 h (PES/Fe-TA3h) showed pure water flux of 175.8 L·m−2·h−1, dye rejections of 97.7%, 97.1% and 95.0% for Congo red (CR), Methyl blue (MB) and Eriochrome Black T (EBT), along with a salt penetration rate of 93.8%, 95.1%, 97.4% and 98.1% for Na2SO4, MgSO4, NaCl and MgCl2 at 0.2 MPa, respectively. Both static adhesion tests and dynamic fouling experiments implied that the TA modified membranes showed significantly reduced adsorption and high FRR for the dye solutions separation. The PES/Fe-TA3h membrane exhibited high FRR of 90.3%, 87.5% and 81.6% for CR, EBT and MB in the fouling test, stable CR rejection (>97.2%) and NaCl permeation (>94.6%) in 24 h continuous filtration test. The combination of blending and interfacial coordination assembly method could be expected to be a universal way to fabricate the loose nanofiltration membrane for effective fractionation of dyes and salts in the saline textile wastewater.

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The effective separation of dyes and inorganic salts is highly desirable for recycling inorganic salts and water resource in printing and dyeing wastewater treatment. In this work, tannic acid (TA) and polyethyleneimine (PEI) were grafted on the PES/Fe ultrafiltration membrane via the coordination assembly and Michael addition strategy to fabricated a loose nanofiltration membrane (LNM). The effect of PEI concentration on membrane morphologies and properties was systematically investigated. The membrane surface becomes more hydrophilic and transforms into positive charge after the PEI grafting. The optimized PES/Fe-TA-PEI membrane possesses high pure water flux (124.6 L·m−2·h−1) and excellent dye rejections (98.5%, 99.8%, 98.4%, and 86.4% for Congo red, Eriochrome black T, Alcian blue 8GX, and Bromophenol blue, respectively) under 2 bar operation pressure. Meanwhile, the LNM showed a high Alcian blue 8GX rejection (>98.4%) and low NaCl rejection (<5.3%) for the dye/salt mixed solutions separation. Moreover, the PES/Fe-TA-PEI LNM exhibited good antifouling performance and long-term performance stability. These results reveal that such LNM shows great potential for effective fractionation of dyes and salts and recycling of textile wastewater.

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