The textile industry has been considered as one of the polluting industries, producing a large amount of textile waste and CO2 emissions each year. Recycling of waste fabric has attracted more research interest in recent years. Herein, renewable polydopamine (PDA)-functionalized cellulose aerogels (CAs) have been designed by a feasible and green way for clean water generation. With the polymerization of PDA on the surface, which possesses excellent photothermal conversion performance and water purification ability, the resulting CA could achieve a high light absorption of 96.5% with the evaporation rate of 2.74 kg m–2 h–1 under 1 sun. Meanwhile, the solar steam generator with the increasing height can absorb energy from adjacent ambient air to strengthen the vapor generation. The features of renewable CAs can achieve efficient water evaporation, which combined with their low material cost and recycling, offer promise in reducing not only energy consumption but also the environmental footprint of cotton textiles.

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Solar steam generation has been considered a promising approach for using renewable solar energy to produce clean water from seawater and wastewater. It shows great potential for alleviating water shortages. However, salt accumulation and system longevity are challenges which impede the widespread use of evaporators. This paper reports a stable Janus evaporator with thickness controllable hydrophilic and hydrophobic layers based on cellulose composite aerogels, which were extracted from waste cotton fabric by a two-step freeze-drying process. The obtained glutaraldehyde cross-linked carbon nanotubes/cellulose Janus aerogel exhibited an attractive solar steam generation rate of 1.81 kg·m–2·h–1 and a light-to-vapor efficiency of up to 92.5% in 1 sun illumination. Moreover, the Janus solar steam generator could pledge stable and sustainable solar-driven water evaporation performance within a 10 h test, showing a high salt-resistant property in simulated seawater. In addition, the developed solar evaporator also had a good purification effect on dye wastewater. These findings suggest its potential ability for seawater desalination and wastewater purification.

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