Reclamation and reuse of wastewater are increasingly viewed as a pragmatic tool for water conservation. Greywater, which includes water from baths, washing machines, dishwashers, and kitchen sinks, is a dilute wastewater stream, making it an attractive stream for extraction of non-potable water. However, most previous studies primarily focused on passively aerated biological and physicochemical treatment processes for greywater treatment. Here, we investigated an integrated process of a microbial electrochemical cell (MEC) followed by granular activated carbon (GAC) biofilter for greywater treatment. The integrated system could achieve 99.3% removal of total chemical oxygen demand (TCOD) and 98.7% removal of the anionic surfactants (linear alkylbenzene sulphonates) from synthetic greywater at a total hydraulic residence time (HRT) of 25 h (1 day for MEC and 1 h for GAC biofilter). For one-day HRT, the maximum peak volumetric current density from MEC was 0.65 A/m3, which was comparable to that achieved at four-day HRT (0.66 A/m3). The adsorption by GAC was identified as a key mechanism for the removal of organics and surfactants. In addition, recirculation of liquid within the GAC biofilter was identified as a critical factor in achieving high-rate treatment. Although results indicated that GAC biofilter could be a standalone process for greywater, MEC can provide an opportunity for potential energy recovery from greywater. However, further studies should focus on developing high-rate MECs with higher energy recovery potential for practical operation.
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