In the realization of ultrasmall semiconductor lasers, cavity-QED effects are used to enhance spontaneous emission and enable the lasing threshold to be crossed with gain contributions from only a few solid-state emitters. Operation in this regime fosters correlation effects that leave their fingerprint especially in the emission dynamics of nanolasers. Using time-resolved photon-correlation spectroscopy, we show that in a quantum-dot photonic-crystal nanolaser emitting in the telecom band, second-order coherence associated with lasing is established on a different timescale than the emission itself. By combining measurements with a microscopic semiconductor laser theory, we attribute the origin to carrier-photon correlations that give rise to non-Markovian effects in the emission dynamics that are not captured by laser rate-equation theories. Our results have direct implications with respect to the modulation response, repetition rate, noise characteristics, and coherence properties of nanolasers for device applications.
We provide experimental and theoretical insight into single-emitter lasing effects in a quantum dot (QD)-microlaser under controlled variation of background gain provided by off-resonant discrete gain centers. For that purpose, we apply an advanced two-color excitation concept where the background gain contribution of off-resonant QDs can be continuously tuned by precisely balancing the relative excitation power of two lasers emitting at different wavelengths. In this way, by selectively exciting a single resonant QD and off-resonant QDs, we identify distinct single-QD signatures in the lasing characteristics and distinguish between gain contributions of a single resonant emitter and a countable number of off-resonant background emitters to the optical output of the microlaser. Our work addresses the important question whether single-QD lasing is feasible in experimentally accessible systems and shows that, for the investigated microlaser, the single-QD gain needs to be supported by the background gain contribution of off-resonant QDs to reach the transition to lasing. Interestingly, while a single QD cannot drive the investigated micropillar into lasing, its relative contribution to the emission can be as high as 70% and it dominates the statistics of emitted photons in the intermediate excitation regime below threshold.
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