Gaseous fuels for heavy-duty internal combustion engines provide inherent advantages for reducing CO2, particulate matter (PM), and NOX emissions. Pilot-ignited direct-injected NG (PIDING) combustion uses a small pilot injection of diesel to ignite a late-cycle main direct injection of NG, resulting in significant reduction of unburned CH4 emissions relative to port-injected NG. Previous works have identified NG premixing as a critical parameter establishing indicated efficiency and emissions performance. To this end, a recent experimental investigation using a metal engine identified six general regimes of PIDING heat release and emissions behavior arising from variation of NG stratification through control of relative injection timing (RIT) of the NG with respect to the pilot diesel. The objective of the current work is to provide comprehensive description of in-cylinder fuel mixing of direct injected gaseous fuel and its impacts on combustion and pollutant formation processes for stratified PIDING combustion. In-cylinder imaging of OH*-chemiluminescence (OH*-CL) and PM (700 nm), and measurement of local concentration of fuel is considered for 11 different [Formula: see text], representing 5 regimes of stratified PIDING combustion (performed with [Formula: see text] MPa and [Formula: see text]). The magnitude and cyclic variability of premixed fuel concentration near the bowl wall provides direct experimental validation of thermodynamic metrics ([Formula: see text], [Formula: see text], [Formula: see text]) that describe the fuel-air mixture state of all 5 regimes of PIDING combustion. The local fuel concentration develops non-monotonically and is a function of RIT. High indicated efficiency and low CH4 emissions previously observed for stratified-premixed PIDING combustion in previous (non-optical) investigations are due to: (i) very rapid reaction zone growth ([Formula: see text] m/s) and (ii) more distributed early reaction zones when overlapping pilot and NG injections cause partial pilot quenching. These results connect and extend the findings of previous investigations and guide the future strategic implementation of NG stratification for improved combustion and emissions performance.
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