High-resolution powder neutron diffraction has been used to study
the crystal structure of the Mg11B2 superconductor (Tc = 39.2 K) prepared at high pressure in the temperature range 2 to
293 K. The experimental data provide clear evidence of
temperature-independent phase inhomogeneity, which was modelled by
coexisting Mg1+δB2 phases. Precise structural
information for temperatures near Tc also reveals extremely small
volume and c-axis discontinuities, consistent with the existence
of a specific heat anomaly at Tc.
Polarized and unpolarized neutron triple-axis spectrometry was used to study the dynamical magnetic susceptibility χ ′′ (q, ω) as a function of energy (¯ hω) and wave vector (q) in a wide temperature range for the bilayer superconductor YBa2Cu3O6+x with oxygen concentrations, x, of 0.45, 0.5, 0.6, 0.7, 0.8, 0.93, and 0.95. The most prominent features in the magnetic spectra include a spin gap in the superconducting state, a pseudogap in the normal state, the much-discussed resonance, and incommensurate spin fluctuations below the resonance. We establish the doping dependence of the spin gap in the superconducting state, the resonance energy, and the incommensurability of the spin fluctuations. The magnitude of the spin gap (Esg) up to the optimal doping is proportional to the superconducting transition temperature Tc with Esg/kBTc = 3.8. The resonance, which exists exclusively below Tc for highly doped YBa2Cu3O6+x with x = 0.93 and 0.95, appears above Tc for underdoped compounds with x ≤ 0.8. The resonance energy (Er) also scales with kBTc, but saturates at Er ≈ 40 meV for x close to 0.93. The incommensurate spin fluctuations at energies below the resonance have structures similar to that of the single-layer superconducting La2−xSrxCuO4. However, there are also important differences. While the incommensurability (δ) of the spin fluctuations in La2−xSrxCuO4 is proportional to Tc for the entire hole-doping range up to the optimal value, the incommensurability in YBa2Cu3O6+x increases with Tc for low oxygen doping and saturates to δ = 0.1 for x ≥ 0.6. In addition, the incommensurability decreases with increasing energy close to the resonance. Finally, the incommensurate spin fluctuations appear above Tc in underdoped compounds with x ≤ 0.6 but for highly doped materials they are only observed below Tc. We discuss in detail the procedure used for separating the magnetic scattering from phonon and other spurious effects. In the comparison of our experimental results with various microscopic theoretical models, particular emphasis was made to address the similarities and differences in the spin fluctuations of the two most studied superconductors. Finally, we briefly mention recent magnetic field dependent studies of the spin fluctuations and discuss their relevance in understanding the microscopic origin of the resonance.
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