A new technique is described for the isochoric heating (i.e., heating at constant volume) of matter to high energy-density plasma states (>10(5) J/g) on a picosecond time scale (10(-12)sec). An intense, collimated, ultrashort-pulse beam of protons--generated by a high-intensity laser pulse--is used to isochorically heat a solid density material to a temperature of several eV. The duration of heating is shorter than the time scale for significant hydrodynamic expansion to occur; hence the material is heated to a solid density warm dense plasma state. Using spherically shaped laser targets, a focused proton beam is produced and used to heat a smaller volume to over 20 eV. The technique described of ultrafast proton heating provides a unique method for creating isochorically heated high-energy density plasma states.

Fusion fast ignition (FI) initiated by a laser-driven particle beam promises a path to high-yield and high-gain for inertial fusion energy. FI can readily leverage the proven capability of inertial confinement fusion (ICF) drivers, such as the National Ignition Facility, to assemble DT fusion fuel at the relevant high densities. FI provides a truly alternate route to ignition, independent of the difficulties with achieving the ignition hot spot in conventional ICF. FI by laser-driven ion beams provides attractive alternatives that sidestep the present difficulties with laser-driven electron-beam FI, while leveraging the extensive recent progress in generating ion beams with high-power density on existing laser facilities. Whichever the ion species, the ignition requirements are similar: delivering a power density ≈1022 W cm−3 (∼10 kJ in ≈20 ps within a volume of linear dimension ≈20 µm), to the DT fuel compressed to ∼400 g cm−3 with areal density ∼2 g cm−2. High-current, laser-driven beams of many ion species are promising candidates to deliver such high-power densities. The reason is that high energy, high-power laser drivers can deliver high-power fluxes that can efficiently make ion beams that are born neutralized in ∼fs–ps timescales, making them immune to the charge and current limits of conventional beams. In summary, we find that there are many possible paths to success with FI based on laser-driven ion beams. Although many ion species could be used for ignition, we concentrate here on either protons or C ions, which are technologically convenient species. We review the work to date on FI design studies with those species. We also review the tremendous recent progress in discovering, characterizing and developing many ion-acceleration mechanisms relevant to FI. We also summarize key recent technological advances and methods underwriting that progress. Based on the design studies and on the increased understanding of the physics of laser-driven ion acceleration, we provide laser and ion-generation laser-target design points based on several distinct ion-acceleration mechanisms.

High-harmonic generation is a universal response of matter to strong femtosecond laser fields, coherently upconverting light to much shorter wavelengths. Optimizing the conversion of laser light into soft x-rays typically demands a trade-off between two competing factors. Because of reduced quantum diffusion of the radiating electron wave function, the emission from each species is highest when a short-wavelength ultraviolet driving laser is used. However, phase matching--the constructive addition of x-ray waves from a large number of atoms--favors longer-wavelength mid-infrared lasers. We identified a regime of high-harmonic generation driven by 40-cycle ultraviolet lasers in waveguides that can generate bright beams in the soft x-ray region of the spectrum, up to photon energies of 280 electron volts. Surprisingly, the high ultraviolet refractive indices of both neutral atoms and ions enabled effective phase matching, even in a multiply ionized plasma. We observed harmonics with very narrow linewidths, while calculations show that the x-rays emerge as nearly time-bandwidth-limited pulse trains of ~100 attoseconds.

The charge state distributions of Fe, Na, and F are determined in a photoionized laboratory plasma using high resolution x-ray spectroscopy. Independent measurements of the density and radiation flux indicate unprecedented values for the ionization parameter xi=20-25 erg cm s(-1) under near steady-state conditions. Line opacities are well fitted by a curve-of-growth analysis which includes the effects of velocity gradients in a one-dimensional expanding plasma. First comparisons of the measured charge state distributions with x-ray photoionization models show reasonable agreement.

We make direct observations of localized light absorption in a single nanostructure irradiated by a strong femtosecond laser field, by developing and applying a technique that we refer to as plasma explosion imaging. By imaging the photoion momentum distribution resulting from plasma formation in a laser-irradiated nanostructure, we map the spatial location of the highly localized plasma and thereby image the nanoscale light absorption. Our method probes individual, isolated nanoparticles in vacuum, which allows us to observe how small variations in the composition, shape, and orientation of the nanostructures lead to vastly different light absorption. Here, we study four different nanoparticle samples with overall dimensions of ∼100 nm and find that each sample exhibits distinct light absorption mechanisms despite their similar size. Specifically, we observe subwavelength focusing in single NaCl crystals, symmetric absorption in TiO2 aggregates, surface enhancement in dielectric particles containing a single gold nanoparticle, and interparticle hot spots in dielectric particles containing multiple smaller gold nanoparticles. These observations demonstrate how plasma explosion imaging directly reveals the diverse ways in which nanoparticles respond to strong laser fields, a process that is notoriously challenging to model because of the rapid evolution of materials properties that takes place on the femtosecond time scale as a solid nanostructure is transformed into a dense plasma.