Hybrid nanocomposites can offer a wide range of opportunities to control the light-matter interaction and electromagnetic energy flow at the nanoscale, leading to exotic optoelectronic devices. We study theoretically the dipole-dipole interaction in noble metal nanoparticles-graphene nanodisksquantum dots hybrid systems in the optical region of the electromagnetic spectrum. The quantum dot is assumed to be a three-level atom interacting with ultrashort control and probe pulses in a Λ configuration. The dynamics of the system are studied by numerically solving for the time evolution of the density matrix elements. We investigate the rate of energy exchange between surface plasmon resonances of the graphene nanodisks and excitons of the quantum dots in the presence of metal nanoparticles at steady state and for specific geometrical conditions of the system. Ultrafast population dynamics are obtained with a large energy exchange rate significantly depending on the size of metal nanoparticles. The power transfer can be controlled by varying the center-to-center distances between the components of the system, and their positions with respect to each other. We also find that the rate of energy transfer within the system is governed by the probe field Rabi frequency, enhanced by the dipole-dipole interaction.
Hybrid nanocomposites can provide a promising platform for integrated optics. Optical nonlinearity can significantly widen the range of applications of such structures. In the present paper, a theoretical investigation is carried out by solving the density matrix equations derived for a metal nanoparticles-graphene nanodisks-quantum dots hybrid system interacting with weak probe and strong control fields, in the steady state. We derive analytical expressions for linear and third-order nonlinear susceptibilities of the probe field. A giant self-Kerr nonlinear index of refraction is obtained in the optical region with relatively low light intensity. The optical absorption spectrum of the system demonstrates electromagnetically induced transparency and amplification without population inversion in the linear optical response arising from the negative real part of the polarizabilities for the plasmonic components at the energy of the localized surface plasmon resonance of the graphene nanodisks induced by the probe field. We find that the self-Kerr nonlinear optical properties of the system can be controlled by the geometrical features of the system, the size of metal nanoparticles and the strength of the control field. The controllable self-Kerr nonlinearities of hybrid nanocomposites can be employed in many interesting applications of modern integrated optics devices allowing for high nonlinearity with relatively low light intensity.
Active nanoplasmonics has recently led to the emergence of many promising applications. One of them is spaser (surface plasmons amplification by stimulated emission of radiation) that has been shown to generate coherent and intense fields of selected surface plasmon modes that are strongly localized in the nanoscale. We propose a novel nanospaser composed of metal nanoparticlesgraphene nanodisks hybrid plasmonic system as its resonator and a quantum dots cascade stack as its gain medium. We derive the plasmonic fields induced by pulsed excitation through the use of the effective medium theory. Based on the density matrix approach and by solving the Lindblad quantum master equation, we get ultrafast dynamics of the spaser associated with coherent amplified plasmonic fields. The intensity of the latter is significantly affected by the width of the metallic contact and the time duration of the laser pulse used to launch the surface plasmons. The proposed nanospaser operates in the mid-infrared region that has received much attention due to its wide biomedical, chemical and telecommunication applications.
We theoretically investigate the optical bistability in the metal nanoparticles-graphene nanodisks-quantum dots hybrid plasmonic system in the infrared regime of the electromagnetic radiation. The quantum dot is considered to be a three-level atomic-like system of Λ type interacting with probe and control fields. By using the standard model of the optical bistability where a nonlinear medium is situated in an optical ring cavity, we numerically solve the equation of motion for the density matrix elements that describe the dynamics of the system in steady-state conditions along with the boundary conditions of the cavity to analyze the optical bistability of the system. The effect of the geometrical features of the system and the parameters of the interacting fields including the strength and detuning of the fields on the optical bistability behavior are investigated. Our proposed hybrid plasmonic system shows an ultralow-threshold controllable optical bistability, providing a promising platform for optical bistable devices at the terahertz, such as all-optical switches and biosensors.
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