Green hydrogen technology has recently gained in popularity due to the current economic and ecological trends that aim to remove the fossil fuels share in the energy mix. Among various alternatives, biogas reforming is an attractive choice for hydrogen production. To meet the authorities’ requirements, reforming biogas-enriched natural gas and sole biogas is tempting. Highly effective process conditions of biogas reforming are yet to be designed. The current state of the art lacks proper optimization of the process conditions. The optimization should aim to allow for maximization of the process effectiveness and limitation of the phenomena having an adverse influence on the process itself. One of the issues that should be addressed in optimization is the uniformity of temperature inside a reactor. Here we show an optimization design study that aims to unify temperature distribution by novel arrangements of catalysts segments in the model biogas reforming reactor. The acquired numerical results confirm the possibility of the enhancement of reaction effectiveness, coming from improving the thermal conditions. The used amount of catalytic material is remarkably reduced as a side effect of the presented optimization. To ensure an unhindered perception of the reaction improvement, the authors proposed a ratio of the hydrogen output and the amount of used catalyst as a measure.
Recent trends in hydrogen production include using renewable energy sources, e.g., biogas as feedstocks for steam reforming. Crucial to the field is minimizing existing reforming reactors for their applications to fuel cell systems. Here, we present a novel design of a steam reforming reactor for an efficient biogas conversion to hydrogen. The design includes a radial division of the catalytic insert into individual segments and substituting parts of the catalytic material with metallic foam. The segment configuration is optimized using a genetic algorithm to maximize the efficiency of the reactor. Changes in the catalytic insert design influence the thermal conditions inside the reactor, leading to moderation of the reaction rate. This article presents a promising approach to producing hydrogen from renewable sources via steam reforming. A significant enhancement in the reforming process effectiveness is achieved with a notable decrease in the amount of the catalyst used. The final results demonstrate the capability for acquiring a similar level of biogas conversion with a 41% reduction of the catalytic material applied.
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