Metasurfaces of gold (Au) nanoparticles on a SiO2-Si substrate were fabricated for the enhancement of second harmonic generation (SHG) using electron beam lithography and lift-off. Triangular Au nanoprisms which are non-centro-symmetric and support second-order nonlinearity were examined for SHG. The thickness of the SiO2 spacer is shown to be an effective parameter to tune for maximising SHG. Electrical field enhancement at the fundamental wavelength was shown to define the SHG intensity. Numerical modeling of light enhancement was verified by experimental measurements of SHG and reflectivity spectra at the normal incidence. At the plasmonic resonance, SHG is enhanced up to ∼3.5 × 103 times for the optimised conditions.
The fabrication of ultra-violet (UV) second-harmonic generation (SHG) (UV-SHG) devices requires GaN quasi-phase matching (GaN-QPM) crystals with periodically arranged polar GaN. For fabricating GaN-QPM crystals, the double polarity selective area growth (DP-SAG) using carbon mask technique is employed. However, the growth of narrow (2–4 [Formula: see text]m) pitch pattern GaN-QPM crystals, which is necessary for UV-SHG devices, has not been reported using this technique. Herein, we report the successful fabrication of 4 [Formula: see text]m pitch pattern GaN-QPM. We fabricated a thick GaN-QPM crystal at the optimized V/III ratio. Through optical characterization, we observed SHG generation from the GaN-QPM crystal fabricated using DP-SAG.
Metasurfaces of gold (Au) nanoparticles on a SiO2-Si substrate were fabricated for the enhancement of second harmonic generation (SHG) using electron beam lithography and lift-off. Triangular Au nanoprisms which are non-centro-symmetric and support the second- order non-linearity were examined for SHG. The thickness of the SiO2 spacer is shown to be an efficient parameter to spectrally tune to maximise SHG. Electrical field enhancement at the fundamental wavelength was shown to define the intensity of the second harmonics. Numerical modeling of light enhancement was verified by experimental measurements of SHG and reflectivity spectra at the normal incidence. At the plasmonic resonance, SHG is enhanced up to ∼3.5×103 times for the optimised conditions.
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