[1] During the Stratosphere-Troposphere Analyses of Regional Transport (START) experiment in December 2005, the behavior of the extratropical tropopause was examined under a variety of dynamical conditions. Using in situ measurements of ozone and water vapor, on board the new NSF/NCAR research aircraft Gulfstream V, and data from large-scale meteorological analyses, we address issues of the tropopause definitions and sharpness. Comparisons of the data from two flights show that the sharpness of chemical transitions across the tropopause varies with the sharpness of the static stability change across the tropopause. Using tracer correlations, air masses of mixed stratospheric and tropospheric characteristics are identified. The mixed air mass does not form a uniform mixing layer near the tropopause, but rather shows strong spatial variation. A depth of mixed air ($5 km in vertical distribution) is found on the cyclonic side of the polar jet, where the thermal gradient is weak and significant separation occurs between the thermal and the dynamical tropopause. Away from the jet or on the anticyclonic side of the jet, where the stability gradient is strong, the chemical transition across the tropopause was much more abrupt and shows minimum mixing. In both cases (either significant or minimal mixing), the thermal tropopause is shown to be approximately at the center of the mixing layer, and the altitude relative to the thermal tropopause is found to be an effective coordinate for locating the chemical transition. To further understand the role of the thermal and dynamical tropopause as a chemical transport boundary, tracer correlations are used to examine the chemical characteristics, and the trajectory calculations are used to infer the fate of the air mass between the thermal and dynamic tropopauses in the region of significant separation. The tracer correlation analysis shows that the air mass in this region is a mixture of stratospheric and tropospheric air but predominantly of tropospheric characteristics. Trajectory model calculations show that a significant fraction of the air parcels in this region ended in the mid to lower troposphere, which suggest the irreversible nature of the observed stratospheric intrusion.
The Fronts and Atlantic Storm-Track Experiment (FASTEX) provided an opportunity for testing targetedobserving procedures in a real-time framework during January and February 1997. This study describes the use of singular vectors (SVs) for objective targeting during FASTEX, and the evaluation of the impact obtained from targeted dropsonde data, satellite wind data, and other observations on 1-2 day forecast skill in intensive observation periods (IOPs) 17 and 18.In IOP17, targeted dropsondes improve a 42 h forecast of L41 (Low 41; cyclones were numbered in sequence throughout FASTEX) in terms of sea-level pressure, but the forecast skill is degraded in the upper troposphere. It is suggested that the degraded forecast may be caused by an incomplete survey of the SV target area, that improved the analysis in one region, but made the analysis less accurate in an adjacent part of the target area where no dropsonde data were provided. In a series of experiments, the best 42 h forecast of L41 is obtained by the addition of a few radiosonde profiles provided specially for FASTEX at off-times, that provide observational data in the most sensitive part of the SV target area. The analysis differences introduced by the radiosonde profiles are much smaller in magnitude than those from the dropsonde data, but have a larger forecast impact, because they occur in an area that has larger error growth rates in this forecast.In a series of experiments for IOP18, the best 24 h forecast of L44 is obtained using a combination of targeted-dropsonde data and satellite wind data. Both data types can also be used separately to improve this forecast. The assimilation of satellite wind data and ship-based soundings in areas of weak initial-condition sensitivity ('null' areas) is shown to have minimal impact on the forecast error. The target areas identified by SVs in these two IOPs occur in strongly baroclinic regions, tending to favour the right-entrance and left-exit regions of the upper-level jet, but with greatest sensitivity near 600 hPa.
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