Abstract-The mixed method approaches have recently risen to prominence. The reason that more researchers are opting for these types of research is that both qualitative and quantitative data are simultaneously collected, analyzed and interpreted. In this article the main research instruments (questionnaire, interview and classroom observation) usually used in the mixed method designs are presented and elaborated on. It is believed that using different types of procedures for collecting data and obtaining that information through different sources (learners, teachers, program staff, etc.) can augment the validity and reliability of the data and their interpretation. Therefore, the various ways of boosting the validity and reliability of the data and instruments are delineated at length. Finally, an outline of reporting the findings in the mixed method approaches is sketched out. It is believed that this article can be useful and beneficial to the researchers in general and postgraduate students in particular who want to start or are involved in the process of conducting research.
A key question concerning the three-body fragmentation of polyatomic molecules is the distinction of sequential and concerted mechanisms, i.e., the stepwise or simultaneous cleavage of bonds. Using laser-driven fragmentation of OCS into O^{+}+C^{+}+S^{+} and employing coincidence momentum imaging, we demonstrate a novel method that enables the clear separation of sequential and concerted breakup. The separation is accomplished by analyzing the three-body fragmentation in the native frame associated with each step and taking advantage of the rotation of the intermediate molecular fragment, CO^{2+} or CS^{2+}, before its unimolecular dissociation. This native-frame method works for any projectile (electrons, ions, or photons), provides details on each step of the sequential breakup, and enables the retrieval of the relevant spectra for sequential and concerted breakup separately. Specifically, this allows the determination of the branching ratio of all these processes in OCS^{3+} breakup. Moreover, we find that the first step of sequential breakup is tightly aligned along the laser polarization and identify the likely electronic states of the intermediate dication that undergo unimolecular dissociation in the second step. Finally, the separated concerted breakup spectra show clearly that the central carbon atom is preferentially ejected perpendicular to the laser field.
The dissociation of an H + 2 molecular-ion beam by linearly polarized, carrier-envelope-phase-tagged 5 fs pulses at 4×10 14 W/cm 2 with a central wavelength of 730 nm was studied using a coincidence 3D momentum imaging technique. Carrier-envelope-phase-dependent asymmetries in the emission direction of H + fragments relative to the laser polarization were observed. These asymmetries are caused by interference of odd and even photon number pathways, where net-zero photon and 1-photon interference predominantly contributes at H + +H kinetic energy releases of 0.2 -0.45 eV, and net-2-photon and 1-photon interference contributes at 1.65 -1.9 eV. These measurements of the benchmark H + 2 molecule offer the distinct advantage that they can be quantitatively compared with ab initio theory to confirm our understanding of strong-field coherent control via the carrier-envelope phase. PACS numbers: XXXOne ultimate goal of ultrafast, strong-field laser science is to coherently control chemical reactions [1][2][3]. A prerequisite to achieving this goal is to understand the control mechanisms and reaction pathways. To this end, tailoring the electric field waveform of few-cycle laser pulses to control reactions and uncover the underlying physics has become a powerful tool [4][5][6]. It has been applied to the dissociative ionization of H 2 and its isotopologues [7][8][9][10][11][12] and has recently been extended to more complex diatomic molecules, such as CO [13][14][15], and to small polyatomic molecules [16,17].Conceptually, one of the most basic features of a fewcycle laser pulse to control is the carrier-envelope phase (CEP). When the laser's electric field is written as E(t) = E 0 (t) cos(ωt + φ), E 0 (t) is an envelope function, ω is the carrier angular frequency, and φ is the CEP. In fact, all of the few-cycle waveform experiments cited above used the CEP as the control parameter.For example, Kling et al. used 5 fs, 1.2×10 14 W/cm 2 pulses with stabilized CEP to dissociatively ionize D 2 and found asymmetries in the emission direction of D + ions for kinetic energy releases (KER) above 6 eV [7,8]. The diminished dissociation signal in a circularly polarized laser field indicated that recollision played a role. Recollision entails a tunnel-ionized electron undergoing a collision with its parent ion after acceleration by the oscillating laser field [18,19]. The energy exchange between the laser-driven electron and the parent ion can promote the D + 2 to the 2pσ u excited state. Coupling of the 2pσ u and 1sσ g states [20] on the trailing edge of the laser pulse during the dissociation of D + 2 was suggested as the explanation for the CEP-dependent asymmetry [7,8].Another example comes from Kremer et al. who exposed an H 2 target to 6 fs, 4.4×10 14 W/cm 2 CEPstabilized laser pulses and observed asymmetries for KER values between 0.4 and 3 eV [9] -energies they attributed to bond softening (BS) [21] and not electron recollision, which has higher KER. They proposed that the initial ionization of H 2 generates a coherent wav...
We present kinematically complete measurements of the photo double ionization of ethylene (double CC bond) and acetylene (triple CC bond) hydrocarbons just above the double ionization threshold. We discuss the results in terms of the coincident kinetic energy of the photo electrons and the nuclear kinetic energy release of the recoiling ions. We have incorporated quantum chemistry calculations to interpret which of the electronic states of the dication have been populated and trace the various subsequent fragmentation channels. We suggest pathways that involve the electronic ground and excited states of the precursor ethylene dication and explore the strong influence of the conical intersections between the different electronic states. The nondissociative ionization yield is small in ethylene and high in acetylene when compared with the dissociative ionization channels.The reason for such a striking difference is explained in part on the basis of a propensity rule which influences the population of states in the photo double ionization of a centrosymmetric closed shell molecule by favoring singlet ungerade and triplet gerade final states. This propensity rule and the calculated potential energy surfaces clarify a picture of the dynamics leading to the observed dication dissociation products.
Shaping ultrafast laser pulses using adaptive feedback can manipulate dynamics in molecular systems, but extracting information from the optimized pulse remains difficult. Experimental time constraints often limit feedback to a single observable, complicating efforts to decipher the underlying mechanisms and parameterize the search process. Here we show, using two strong-field examples, that by rapidly inverting velocity map images of ions to recover the three-dimensional photofragment momentum distribution and incorporating that feedback into the control loop, the specificity of the control objective is markedly increased. First, the complex angular distribution of fragment ions from the no þis controlled via a barrier-suppression mechanism, a result that is validated by model calculations. Collectively, these experiments comprise a significant advance towards the fundamental goal of actively guiding population to a specified quantum state of a molecule.
This paper reports on research findings on leaner-centered approach compared to teacher-centered approach in teaching English grammar as a foreign language in Iranian high school context. It shows the need for grammar instruction in English language classes when roughly all education efforts are bottom-up explicit approach. One could compare and contrast these two learning approaches and try to evaluate the effectiveness of them. To this end, a cohort of 60 male homogeneous students at a junior high school in Tabriz, Iran participated in this study. All participants were native speakers of Azerbaijani and Persian aged around 16. There were two classes, including 30 students in each group (class) who were assigned to the control and experimental group. The experimental group received a treatment in passive-active voice, followed by a grammar pre-and post-test. All the tests consisted of multiple-choice, cloze, and fill-in-blanks, which were administered to study the homogeneity in their grammar knowledge over one month, and the results were compared. Two groups were observed, namely the control group (group A) or teacher-centered and the experimental group (group B) or student-centered. This experimental study also comprised classroom observations and teacher interview. When the students are given the opportunity to merge input in what they learn and how they learn, academic achievements and comprehension occur. The results support the implementation of teacher-centered process for the purpose of developing grammar knowledge of Iranian EFL learners. English classes cannot fulfill the learners' needs on communication. The findings suggest the need for explicit teaching of grammar rules and their use through communicative tasks.
In a recent Letter, Manschwetus et al. [Phys. Rev. Lett. 102, 113002 (2009)] reported evidence of electron recapture during strong-field fragmentation of H 2 -explained using a frustrated tunneling ionization model. Unusually, the signature of this process was detection of excited H * atoms. We report here an extensive study of this process in D 2 . Our measurements encompass a study of the pulse duration, intensity, ellipticity, and angular distribution dependence of D * formation. While we find that the mechanism suggested by Manschwetus et al. is consistent with our experimental data, our theoretical work shows that electron recollision excitation cannot be completely ruled out as an alternative mechanism for D * production.
Laser-induced dissociation of O + 2 is studied in the strong-field limit using two independent methods, namely a crossed laser-ion-beam coincidence 3D momentum imaging method and a supersonic gas jet velocity map imaging technique (790 and 395 nm, 8-40 fs, ∼10 15 W/cm 2 ). The measured kinetic energy release spectra from dissociation of O + 2 and dissociative ionization of O 2 reveal vibrational structure which persists over a wide range of laser intensities. The vibrational structure is similar for O + 2 produced incoherently in an ion source and coherently by laser pulses. By evaluation of the potential energy curves, we assign the spectral energy peaks to dissociation of the v = 10-15 vibrational states of the metastable a 4 u state via the dissociation pathway |a 4 u → |f 4 g − 1ω -a mechanism equivalent to bond softening in H + 2 .
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