We demonstrate a method to create arbitrary terahertz (THz) polarization profiles by exploiting the magnetic field-dependent emission process of a spintronic source. As a proof-of-concept, we show that by applying a specific magnetic field pattern to the source, it is possible to generate a quadrupole-like THz polarization profile. Experimental measurements of the electric field at the focus of the THz beam revealed a polarity flip in the transverse profile of the quadrupole-like mode with a resulting strong, on-axis longitudinal component of 17.7 kV cm−1. This represents an order of magnitude increase in the longitudinal component for the quadrupole-like profile compared to a linear polarization, showing an example of how the magnetic field patterning of a spintronic source can be exploited to obtain desirable THz polarization properties. This unique ability to generate any desired THz polarization profile opens up possibilities for schemes such as rotatable polarization spectroscopy and for efficient mode coupling in various waveguide designs. Furthermore, the strong longitudinal fields that can be generated have applications in areas including intra-subband spectroscopy of semiconductors, non-diffraction limited THz imaging, and particle-beam acceleration.

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The effective mass, sheet carrier concentration, and mobility of electrons within a two-dimensional electron gas in an AlGaN/GaN heterostructure were determined using a laboratory-based terahertz cyclotron resonance spectrometer. The ability to perform terahertz cyclotron resonance spectroscopy with magnetic fields of up to 31 T was enabled by combining a high-field pulsed magnet with a modified asynchronous optical sampling terahertz detection scheme. This scheme allowed around 100 transmitted terahertz waveforms to be recorded over the 14 ms magnetic field pulse duration. The sheet density and mobility were measured to be 8.0 × 1012 cm−2 and 9000 cm2 V−1 s−1 at 77 K. The in-plane electron effective mass at the band edge was determined to be 0.228 ± 0.002m0.

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Periodically-poled lithium niobate (PPLN) sources consisting of custom-built stacks of large-area wafers provide a unique opportunity to systematically study the multi-cycle terahertz (THz) generation mechanism as they are assembled layer-by-layer. Here we investigate and optimize the THz emission from PPLN wafer stacks as a function of wafer number, pump fluence, pulse duration and chirp, wafer separation, and pump focusing. Using 135 µm-thick, 2"-diameter wafers we generate high-energy, narrowband THz pulses with central frequencies up to 0.39 THz, directly suitable for THz-driven particle acceleration applications. We explore the multi-cycle pulse build-up with increasing wafer numbers using electro-optic sampling measurements, achieving THz conversion efficiencies up to 0.17%, while demonstrating unique control over the pulse length and bandwidth these sources offer. Guided by simulations, observed frequency-dependence on both stack-mounting and pump focusing conditions have been attributed to inter-wafer etalon and Gouy phase-shifts respectively, revealing subtle features that are critical to the understanding and performance of PPLN wafer-stack sources for optimal narrowband THz generation.

We have developed dielectric-lined rectangular waveguide structures for terahertz (THz)-driven ultrafast deflection of 100 keV electron beams. The structures were designed to achieve THz phase velocity matching with co-propagating electron bunches.The phase-matching capability was experimentally confirmed through time-frequency analysis of the broadband coherent THz transmission measured by electro-optic sampling. The analysis determined both the frequency dependent propagation constants in the electron interaction region, and the propagation characteristics of the integrated THz tapered coupler.

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We explore the terahertz (THz) emission from CoFeB/Pt spintronic structures in the below-magnetic-saturation regime and reveal an orientation dependence in the emission, arising from in-plane uniaxial magnetic anisotropy (UMA) in the ferromagnetic layer. Maximizing the UMA during the film deposition process and aligning the applied magnetic field with the easy axis of the structure allow the THz emission to reach saturation under weaker applied fields. In addition, the THz emission amplitude remains at saturation levels when the applied field is removed. The development of CoFeB/Pt spintronic structures that can emit broadband THz pulses without the need for an applied magnetic field is beneficial to THz magneto-optical spectroscopy and facilitates the production of large-area spintronic emitters. Furthermore, by aligning the applied field along the hard axis of the structure, the linear polarization plane of the emitted THz radiation can be manipulated by changing the magnitude of the applied field. We, therefore, demonstrate THz polarization control without the need for mechanical rotation of external magnets.