The measurements of residual dipolar couplings in elastomer system is desirable, because they reflect the hindrance to molecular motions by the cross-linking, topological constraints and the external factors like mechanical stress. Dipolar-encoded longitudinal magnetization nuclear magnetic resonance (NMR) decay curves, double-quantum and triple-quantum NMR buildup intensities for measuring the residual dipolar couplings, and the associated dynamic order parameters are introduced. It is shown that in the short excitation time regime the effective dipolar network is simplified. In the limit of this model based on localized dipolar couplings, the spin response to two-dimensional pulse sequences used to record multiple-quantum (MQ) NMR coherences was evaluated for longitudinal magnetization, double-, and triple-quantum coherences of methylene, and methyl protons in synthetic 1,4-cis-polyisoprene. The dynamic order parameters can be evaluated from this NMR response using a classical scale-invariant polymer model. These dynamic order parameters were measured for a cross-link series of synthetic polyisoprene and correlated with the cross-link density. The decay rates of the Hahn-echo amplitudes reflecting residual dipolar couplings as well as effects of molecular motion are also measured for the same cross-link series. The contribution of molecular motions to the transverse relaxation can be separated from the residual dipolar couplings using a train of magic echoes. The sensitivity of these transverse relaxation rates to the cross-link density is compared to that of residual dipolar couplings. The NMR time scale is shorter for the dipolar-encoded longitudinal magnetization and MQ experiments as compared to transverse relaxation experiments leading to an increased sensitivity to cross-link density of the former approaches.
Circular permalloy elements were fabricated by a combination of electron beam lithography, thermal evaporation and liftoff technique on electron transparent membrane substrates. The magnetic properties have been studied by Lorentz transmission electron microscopy. In situ magnetizing experiments have been carried out to obtain information about the nucleation and propagation of magnetic domains within the permalloy nanodisks and to determine the nucleation and saturation fields. The diameter of the patterned elements has been varied between 180 and 950 nm, the height was 15 nm. The experiments showed that the vortex configuration is the most favorable state in zero field conditions of all investigated permalloy nanodisks.
Magnetic vortices play an important role in the switching behavior of micron- and submicron-sized ferromagnetic elements. We have prepared submicron permalloy elements by a combination of electron-beam lithography and liftoff technique on electron transparent membrane substrates. The magnetization reversal mechanism and the remanent magnetization configuration were observed by means of Lorentz transmission electron microscopy. In remanence, the investigated structures form a vortex configuration. In situ magnetizing experiments showed the possibility of adjusting the sense of magnetization rotation by introducing a slight geometric asymmetry to the otherwise circular nanostructures.
We report on the study of terahertz radiation-induced MIRO-like oscillations of magnetoresistivity in GaAs heterostructures. Our experiments provide an answer on two most intriguing questions-effect of radiation helicity and the role of the edges-yielding crucial information for an understanding of the MIRO (microwave-induced resistance oscillations) origin. Moreover, we demonstrate that the range of materials exhibiting radiation-induced magneto-oscillations can be largely extended by using high-frequency radiation. DOI: 10.1103/PhysRevB.94.081301 One of the most interesting phenomena recently observed in two-dimensional electron systems (2DES) is microwave (MW) -induced resistance oscillations (MIRO) and associated zero resistance states (ZRS) [1][2][3][4][5][6][7], reviewed, e.g., in [8]. Like Shubnikov-de Haas oscillations (SdH), MIRO are periodic on a 1/B scale, but occur at lower magnetic fields and show much weaker temperature dependence. Phenomenologically, they are very similar to Weiss oscillations [9], which reflect the commensurability between the cyclotron orbit radius and the period of a periodic potential. MIRO by contrast, reflect the commensurability between the MW photon energy 2π f and the cyclotron energy ω c . In extremely clean samples the minima of the MIRO develop into ZRS [3][4][5], which are explained [10] in terms of an instability of the system and formation of current domains, occurring when the conductivity becomes negative under MW irradiation (see also [8,11,12]).In spite of numerous experiments and significant advances in their theoretical understanding, there is still no commonly accepted microscopic description of the effect [13,14] and the ongoing MIRO investigations remain challenging [15][16][17][18][19][20][21]. Consequently, new materials have been studied [22][23][24][25] and new theoretical models have been put forward [26][27][28][29][30]. To the most pressing issues which need to be clarified experimentally and which might help to differentiate between the different models belong the MIRO polarization dependence [7,8,31] and the "bulk" or "edge" nature of the effect.So far the majority of experimental work has been done in the MW regime (1-350 GHz) and there are only a few reports on MIRO excited at terahertz (THz) frequencies [32][33][34]. Here we report on the observation of pronounced MIRO-like oscillations induced by THz radiation. We exploit the specific advantages of THz laser radiation not present in the MW regime, i.e., the possibility to focus it onto a spot smaller than the sample's size and easy control of the radiation's polarization. The most important features clearly detected on a large variety of samples are (i) a very weak dependence of the oscillations' amplitude on the photon helicity and (ii) the bulk nature of the effect. Furthermore, our study shows that the MIRO oscillations can be excited at THz frequencies even in the samples with low mobility, whereas in the MW range ultrahigh mobility samples are crucially needed for this type of experimen...
We investigate both experimentally and by means of micromagnetic calculations magnetic states preceding vortex formation in permalloy nanodisks. In experiment, we used micro-Hall sensors fabricated from GaAs/AlGaAs heterojunction material to measure stray field hysteresis loops of individual disks. Micromagnetic calculations involving different micromagnetic codes allowed us to interpret the experimental results. Both calculations and experiments suggest that vortex formation can be reached via different precursor states.
Lattice symmetry and magnetization reversal in micron-size antidot arrays in Permalloy filmWe have investigated the magnetic properties of flat permalloy cylinders by Lorentz transmission electron microscopy and micromagnetic simulations. The magnetization patterns during in situ magnetizing experiments have been imaged and they revealed that the magnetization reversal of the cylindrically shaped dots investigated is determined by the formation and annihilation of magnetic vortices. Furthermore, the experiments and micromagnetic simulations showed a dependence of the vortex annihilation field not only on the aspect ratio but also on the absolute thickness of the cylinders. The diameter of the cylindrical dots was varied between 150 and 1000 nm, and the thicknesses were 3, 5.5, 8.3, 15, and 20 nm, respectively. The formation of inhomogeneous magnetization patterns prior to vortex evolution was observed and by a comparison of the experimental to simulated Fresnel images these patterns can be identified as S-and C-like states.
A high pulsed magnetic field measurement system based on the use of CMR-B-scalar sensors was developed for the investigations of the electrodynamic processes in electromagnetic launchers. The system consists of four independent modules (channels) which are controlled by a personal computer. Each channel is equipped with a CMR-B-scalar sensor connected to the measurement device-B-scalar meter. The system is able to measure the magnitude of pulsed magnetic fields from 0.3 T to 20 T in the range from DC up to 20 kHz independently of the magnetic field direction. The measurement equipment circuit is electrically separated from the ground and shielded against low and high frequency electromagnetic noise. The B-scalar meters can be operated in the presence of ambient pulsed magnetic fields with amplitudes up to 0.2 T and frequencies higher than 1 kHz. The recorded signals can be transmitted to a personal computer in a distance of 25 m by means of a fiber optic link. The system was tested using the electromagnetic railgun RAFIRA installed at the French-German Research Institute of Saint-Louis, France.
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