In the present work, we report on the in situ magnetic force microscopy (MFM) study of the magnetization reversal in two-dimensional arrays of ferromagnetic Ni80Fe20 and Co55Fe45 nanowires (NW) with different diameters (40, 50, 70 and 100 nm) deposited inside low porosity (P < 1%) nanoporous polycarbonate membranes. In such arrays, the nanowires are sufficiently isolated from each other so that long range dipolar interactions can be neglected. The MFM experiments performed for different magnetization states at the same spot of the samples are analysed to determine the switching field distribution (SFD). The magnetization curves obtained from the MFM images are relatively square shaped. The SFD widths are narrower compared to those obtained for high density arrays. The weak broadening of the curves may be ascribed to the NW intrinsic SFD. The influence of diameter and composition of the ferromagnetic NW is also investigated.
The magnetic properties of arrays of nanowires (NWs) and nanotubes (NTs), 150 nm in diameter, electrodeposited inside nanoporous polycarbonate membranes are investigated. The comparison of the nanoscopic magnetic force microscopy (MFM) imaging and the macroscopic behavior as measured by alternating gradient force magnetometry (AGFM) is made. It is shown that MFM is a complementary technique that provides an understanding of the magnetization reversal characteristics at the microscopic scale of individual nanostructures. The local hysteresis loops have been extracted by MFM measurements. The influence of the shape of such elongated nanostructures on the dipolar coupling and consequently on the squareness of the hysteresis curves is demonstrated. It is shown that the nanowires exhibit stronger magnetic interactions than nanotubes. The non-uniformity of the magnetization states is also revealed by combining the MFM and AGFM measurements.
First-order reversal curve diagrams, or FORC diagrams, have been studied to determine if the widths of their distributions along the interaction and coercivity axes can be related to the mean-field magnetization dependent interaction field (MDIF). Arrays of nanowires with diameters ranging from 18 up to 100 nm and packing fractions varying from 0.4 to 12% have been analyzed. The mean-field MDIF has been measured using the remanence curves and used as a measuring scale on the FORC diagrams. Based on these measurements, the full width of the interaction field distribution and the full width at half maximum (FWHM) of the FORC distribution profile along the interaction field direction are shown to be proportional to the MDIF, and the relation between them is found. Moreover, by interpreting the full width of the coercive field distribution in terms of the dipolar induced shearing, a simple relation is found between the width of this distribution and the MDIF. Furthermore, we show that the width of the FORC distribution along the coercive field axis is equal to the width of the switching field distribution obtained by the derivation of the DC remanence curve. This was further verified with the switching field distribution determined using in-field magnetic force microscopy (MFM) for very low density nanowires. The results are further supported by the good agreement found between the experiments and the values calculated using the mean-field model, which provides analytical expressions for both FORC distributions.
The fundamental properties of 2D arrays of magnetic nanowires and nanotubes (NWs and NTs) have been well described theoretically, but real systems are subject to certain flaws and imperfections which strongly affect the mechanism and dynamics of magnetization reversal. Therefore, before exploiting the vast potential of magnetic NWs and NTs, there is a need to investigate the materials parameters as well as the field dependent magnetic properties in real systems. Amongst the various issues at stake for a comprehensive understanding of these arrays is the influence of long-range dipolar interactions because these interactions strongly influence the magnetization reversal and thus the switching field distributions (SFD) which plays a significant role for information storage. Particularly, the width of the SFD is important since smaller values of this parameter leads to less recording errors and it is also a measure of the quality of the recording media. Consequently, the understanding a
scite is a Brooklyn-based organization that helps researchers better discover and understand research articles through Smart Citations–citations that display the context of the citation and describe whether the article provides supporting or contrasting evidence. scite is used by students and researchers from around the world and is funded in part by the National Science Foundation and the National Institute on Drug Abuse of the National Institutes of Health.