We report on polarized Raman scattering of single crystals of Nd 1−x Sr x MnO 3 (x = 0.3, 0.5). Raman spectra of Nd 0.7 Sr 0.3 MnO 3 show a significant change through the metal-insulator transition. In the ferromagnetic metallic phase phonon modes grow in intensity and number while the electronic continuum becomes more pronounced. We suggest that these effects are due to the strong competition between the localization and the delocalization of carriers which is the origin of the largest colossal magnetoresistance effect ever reported for the manganites. Raman spectra of Nd 0.5 Sr 0.5 MnO 3 , upon cooling through the charge-ordering temperature T C O = 148 K, exhibit several new lines which undergo a substantial hardening. This hardening is interpreted as a freezing of the Jahn-Teller distortions with a gradual decrease of a fraction of the ferromagnetic phase in the CE-type charge/orbital ordered state.
A tricritical point is observed in the Nd1−xSrxMnO3 (NSMO) (x=0.3, 0.33, and 0.4) manganites at x=0.33 which separates the first-order transition in NSMO-0.3 and second order transition in NSMO-0.4. The ferromagnetic transition of these compounds is further investigated by measuring magnetocaloric effect (MCE) and by applying a theoretical model based on Landau theory of phase transitions. Results indicate that the contributions to the free energy from the presence of correlated clusters are strongly influencing the MCE by coupling with the order parameter around the Curie temperature.
Abstract. We experimentally and computationally study the effect of an additional transverse magnetic field (TMF) on the Hanle resonance for a Fg = 2 → Fe = 3 transition of 87 Rb D2 line for magnetic field scans perpendicular to the propagation direction of the optical field. It is shown that with a π-polarized light, no resonance signal is observed in absence of the TMF. When the TMF is applied, two peaks are observed on either side of zero scanning magnetic field in the transmission spectrum. The separation between the two peaks is linearly proportional to magnitude of the TMF, which can be used for magnetometry. We applied this technique to measure magnetic field from 0.1 to 0.5 G with a pure Rb vapor cell and from 10 to 30 mG with a Rb cell containing buffer gas. These observations are attributed to the population redistribution among the ground state sublevels due to the TMF.
55 Mn nuclear magnetic resonance ͑NMR͒ in Nd 1Ϫx Sr x MnO 3 (0.1рxр0.5) manganites provides local evidence of the magnetic inhomogeneities arising from the electronic structure changes below T C . The temperature dependences of magnetization, resistivity, and NMR spectra were compared in samples in the ferromagnetic insulating, ferromagnetic metallic, and charge-ordered phases. Spin-spin relaxation enhancement around 15 K is attributed to a critical slowing down of the Nd sublattice.
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