Spontaneous and field-induced linear birefringence is measured at low temperatures on singledomained single crystals of weakly doped SrTi0,:Ca (x=0.002 and 0.007) in order to investigate polar ordering processes near to T,-4 and 18 K, respectively. In agreement with direct polarization measurements the size of mesoscopic polar nanodomains is determined within the framework of a nonlinear polarization optical response model. Quasi-first-order Raman scattering of soft and hard polar modes, TO,, TO, and TO,, is observed on local precursor nanodomains above T,. Below T, the change of the global symmetry from D,, to C,, is reflected by selection rules imposed on first-order Raman lines in various scattering geometries.
The interaction between surface acoustic waves (SAWs) and spin waves (SWs) in a piezoelectric/magnetic thin film heterostructure yields potential for the realization of novel microwave devices and applications in magnonics. In the present work, we investigate the SAW-SW interaction in a Pt/Co(2 nm)/Ru(0.85 nm)/Co(4 nm)/Pt synthetic antiferromagnet (SAF) composed of two ferromagnetic layers with different thicknesses separated by a thin nonmagnetic Ru spacer layer. Because of the combined presence of interfacial Dzyaloshinskii-Moriya interaction (iDMI) and interlayer dipolar coupling fields, the optical SW mode shows a large nondegenerate dispersion relation for oppositely propagating SWs. Due to SAW-SW interaction, we observe nonreciprocal SAW transmission in the piezoelectric/SAF hybrid device. The equilibrium magnetization directions of both Co layers are manipulated by an external magnetic field to set a ferromagnetic, canted, or antiferromagnetic configuration. This has a strong impact on the SW dispersion, its nonreciprocity, and SAW-SW interaction. The experimental results are in agreement with a phenomenological SAW-SW interaction model, which considers the interlayer exchange coupling, iDMI, and interlayer dipolar coupling fields of the SWs.
We study the interaction of surface acoustic waves (SAWs) with spin waves (SWs) in a Co 40 Fe 40 B 20 /Au/Ni 81 Fe 19 system composed of two ferromagnetic layers separated by a nonmagnetic Au spacer layer. Because of interlayer magnetic dipolar coupling between the two ferromagnetic layers, a symmetric and an antisymmetric SW mode form, which both show a highly nondegenerate dispersion relation for oppositely propagating SWs. Due to magnetoacoustic SAW-SW interaction, we observe highly nonreciprocal SAW transmission in the piezoelectric-ferromagnetic hybrid device. We experimentally and theoretically characterize the magnetoacoustic wave propagation as a function of frequency, wave vector, and external magnetic field magnitude and orientation. Additionally, we demonstrate that the nonreciprocal SW dispersion of a coupled magnetic bilayer is highly tuneable and not limited to ultrathin magnetic films, in contrast to the nonreciprocity induced by the interfacial Dzyaloshinskii-Moriya interaction. Therefore, magnetoacoustic coupling in ferromagnetic multilayers provides a promising route towards building efficient acoustic isolators.
We study the interaction of Rayleigh and shear horizontal surface acoustic waves (SAWs) with spin waves in thin Ni films on a piezoelectric LiTaO 3 substrate, which supports both SAW modes simultaneously. Because Rayleigh and shear horizontal modes induce different strain components in the Ni thin films, the symmetries of the magnetoelastic driving fields, of the magnetoelastic response, and of the transmission nonreciprocity differ for both SAW modes. Our experimental findings are well explained by a theoretical model based on a modified Landau-Lifshitz-Gilbert approach. We show that the symmetries of the magnetoelastic response driven by Rayleigh and shear horizontal SAWs complement each other, which makes it possible to excite spin waves for any relative orientation of magnetization and SAW propagation direction and, moreover, can be utilized to characterize surface strain components of unknown acoustic wave modes.
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