In 1933, Meissner and Ochsenfeld reported the expulsion of magnetic flux-the diamagnetic Meissner effect-from the interior of superconducting lead. This discovery was crucial in formulating the BardeenCooper-Schrieffer (BCS) theory of superconductivity. In exotic superconducting systems BCS theory does not strictly apply. A classical example is a superconductor-magnet hybrid system where magnetic ordering breaks time-reversal symmetry of the superconducting condensate and results in the stabilization of an odd-frequency superconducting state. It has been predicted that under appropriate conditions, odd-frequency superconductivity should manifest in the Meissner state as fluctuations in the sign of the magnetic susceptibility, meaning that the superconductivity can either repel (diamagnetic) or attract (paramagnetic) external magnetic flux. Here, we report local probe measurements of faint magnetic fields in a Au=Ho=Nb trilayer system using low-energy muons, where antiferromagnetic Ho (4.5 nm) breaks time-reversal symmetry of the proximity-induced pair correlations in Au. From depth-resolved measurements below the superconducting transition of Nb, we observe a local enhancement of the magnetic field in Au that exceeds the externally applied field, thus proving the existence of an intrinsic paramagnetic Meissner effect arising from an odd-frequency superconducting state.
We use calorimetry to identify pressure-driven isothermal entropy changes in ceramic samples of the prototypical ferroelectric BaTiO3. Near the structural phase transitions at ∼400 K (cubic-tetragonal) and ∼280 K (tetragonal-orthorhombic), the inverse barocaloric response differs in sign and magnitude from the corresponding conventional electrocaloric response. The differences in sign arise due to the decrease in unit-cell volume on heating through the transitions, whereas the differences in magnitude arise due to the large volumetric thermal expansion on either side of the transitions.
Scanning tunneling spectroscopy measurements performed on La 0.7 Ca 0.3 Mn 3 O (LCMO) films epitaxially grown on Pr 1.85 Ce 0.15 CuO 4 (PCCO) reveal localized penetration of superconductivity into the LCMO up to distances much larger than is possible for Cooper pairs in a singlet spin state to exist. This long-range proximity effect is manifested in the tunneling spectra as gaps and, less abundantly, as zero-bias conductance peaks (ZBCPs). Since ZBCPs were not found on the bare PCCO films, their appearance is attributed to an anisotropic (p wave or d wave) triplet-pairing superconductor order parameter induced in the LCMO.
Long-ranged superconductor proximity effects recently found in superconductorferromagnetic (S-F) systems are generally attributed to the formation of triplet-pairing correlations due to various forms of magnetic inhomogeneities at the S-F interface. In order to investigate this conjecture within a single F layer coupled to a superconductor, we performed scanning tunneling spectroscopy on bilayers of La2/3Ca1/3MnO3 (LCMO) ferromagnetic thin-films grown on high temperature superconducting films of YBa2Cu3O7- (YBCO) or Pr1.85Ca0.15CuO4 (PCCO) under various magnetic fields. We find a strong correlation between the magnitude of superconductor-related spectral features measured on the LCMO layer and the degree of magnetic inhomogeneity controlled by the external magnetic field. This corroborates theoretical predictions regarding the role played by magnetic inhomogeneities in inducing triplet-pairing at S-F interfaces.
Conventional spin-singlet Cooper pairs convert into spin-triplet pairs in ferromagnetic Josephson junctions in which the superconductor/ferromagnet interfaces (S/F) are magnetically inhomogeneous. Although much of the theoretical work describing this triplet proximity effect has considered ideal junctions with magnetic domain walls (DW) at the interfaces, in practice it is not easily possible to isolate a DW and propagate a supercurrent through it. The rare-earth magnet Gd can form a field-tuneable in-plane Bloch DW if grown between non-co-linearly aligned ferromagnets. Here we report supercurrents through magnetic Ni-Gd-Ni nanopillars: by field annealing at room temperature, we are able to modify the low temperature DW-state in Gd and this result has a striking effect on the junction supercurrent at 4.2 K. We argue that this result can only be explained in terms of the interconversion of triplet and singlet pairs, the efficiency of which depends on the magnetic helicity of the structure.
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