The complex refractive indices of polymers have important applications in the analysis of their components and the study of radiation endothermic mechanisms. Since these materials have high transmittance in the visible to near-infrared ranges, it is difficult to accurately measure their complex refractive indices. At present, the data for complex refractive indices of polymers are seriously lacking, which greatly limits the applications of these materials in the field of thermal radiation. In this work, spectroscopic ellipsometry (SE) combined with the ray tracing method (RTM) is used to measure the complex refractive indices of five polymers, polydimethylsiloxane, poly(methyl methacrylate) (PMMA), polycarbonate, polystyrene, and polyethylene terephthalate, in the spectral range of 0.4–2 µm. The double optical pathlength transmission method (DOPTM) is used to measure the complex refractive indices of three polymers, PMMA, polyvinyl chloride, and polyetherimide, in the 0.4–2 µm range. The complex refractive index of PMMA measured by the DOPTM almost coincides with the data measured by SE combined with the RTM. The results show that the trends of the complex refractive indices spectra for the seven polymers in the 0.4–2 µm range are similar. This work makes up for the lack of complex refractive indices in the 0.4–2 µm range for these seven materials and points out the direction for accurate measurements of the complex refractive indices of polymers with weak absorption.
The many-body radiative heat transfer theory [P. Ben-Abdallah, S.-A. Biehs, and K. Joulain, Phys.Rev. Lett. 107, 114301 (2011)] only considered the contribution from the electric dipole moment. For metal particles, however, the magnetic dipole moment due to eddy current plays an important role, which can further couple with the electric dipole moment to introduce crossed terms. In this work, we develop coupled electric and magnetic dipole (CEMD) approach for the radiative heat transfer in a collection of objects in mutual interaction. Due to the coupled electric and magnetic interactions, four terms, namely the electric-electric, the electric-magnetic, the magnetic-electric and the magnetic-magnetic terms, contribute to the radiative heat flux and the local energy density. The CEMD is applied to study the radiative heat transfer between various dimers of nanoparticles. It is found that each of the four terms can dominate the radiative heat transfer depending on the position and composition of particles.Moreover, near-field many-body interactions are studied by CEMD considering both dielectric and metallic nanoparticles. The near-field radiative heat flux and local energy density can be greatly increased when the particles are in coupled resonances. Surface plasmon polariton and surface phonon polariton can be coupled to enhance the radiative heat flux.
We propose a wide-angle, polarization-independent and dual-band infrared perfect metamaterial absorber made of double L-shaped gold patches on a dielectric spacer and opaque gold ground layer. Numerical and experimental results demonstrate that the absorber has two near-unity absorption peaks, which are result from magnetic polariton modes generated at two different resonant wavelengths. In addition, the proposed structure also shows good absorption stability in a wide range of incident anglesθfor both TE and TM incidences at azimuthal angle φ = 0°. Moreover, we demonstrate that such structure has good absorption stability for a wide range of azimuthal angles due to the excitation of perpendicular magnetic polariton modes within the asymmetric double L-shaped structure. Such structure will assist in designing magnetic polaritons absorbing element for infrared spectroscopy and imaging.
We perform a comprehensive analysis of multi-band absorption by exciting magnetic polaritons in the infrared region. According to the independent properties of the magnetic polaritons, we propose a parallel inductance and capacitance(PLC) circuit model to explain and predict the multi-band resonant absorption peaks, which is fully validated by using the multi-sized structure with identical dielectric spacing layer and the multilayer structure with the same strip width. More importantly, we present the application of the PLC circuit model to preliminarily design a radiative cooling structure realized by merging several close peaks together. This omnidirectional and polarization insensitive structure is a good candidate for radiative cooling application.
Energy consumption of buildings during heating and cooling accounts for about 15% of global total energy consumption. Advanced dynamic switchable windows that enable independent control of solar heat will contribute to optimal energy efficiency in heating, cooling, and artificial lighting systems throughout buildings. Recently, energy‐efficient plasmonic electrochromic smart windows (PESWs) based on metal oxide nanocrystals (NCs) have been gaining increasing attention due to their effective and controllable regulation over the near‐infrared region of the solar spectrum without affecting the dynamic visible transmittance of the smart windows. Herein, the current state‐of‐the‐art results of colloidal metal oxide NCs for PESWs are highlighted, along with their design strategies and working principles. The recent research status of PESWs in typical colloidal metal oxide NCs is reviewed in detail, and the challenges and corresponding countermeasures in this field are discussed. Furthermore, an outlook into novel opportunities in PESW‐related academic research and how to accelerate the pace of real‐world applications is presented.
Near-field radiative heat transfer (RHT) between two bodies can significantly exceed the far-field limit set by Planck's law due to the evanescent wave tunneling, which typically can only occur when the two bodies are separated at subwavelength distances. We show that the RHT between two SiC nanoparticles with separation distances much larger than the thermal wavelength can still exceed the far-field limit when the particles are located within a subwavelength distance away from a SiC substrate. In this configuration, the localized surface phonon polariton (SPhP) of the particles couples to the propagating SPhP of the substrate which then provides a new channel for the near-field energy transport and enhances the RHT by orders of magnitude at large distances. The enhancement is also demonstrated to appear in a chain of closely spaced SiC nanoparticles located in the near field of a SiC substrate. The findings provide a new way for the long-distance transport of near-field energy.
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