Oscillatory clusters are sets of domains in which nearly all elements in a given domain oscillate with the same amplitude and phase. They play an important role in understanding coupled neuron systems. In the simplest case, a system consists of two clusters that oscillate in antiphase and can each occupy multiple fixed spatial domains. Examples of cluster behaviour in extended chemical systems are rare, but have been shown to resemble standing waves, except that they lack a characteristic wavelength. Here we report the observation of so-called 'localized clusters'--periodic antiphase oscillations in one part of the medium, while the remainder appears uniform--in the Belousov-Zhabotinsky reaction-diffusion system with photochemical global feedback. We also observe standing clusters with fixed spatial domains that oscillate periodically in time and occupy the entire medium, and irregular clusters with no periodicity in either space or time, with standing clusters transforming into irregular clusters and then into localized clusters as the strength of the global negative feedback is gradually increased. By incorporating the effects of global feedback into a model of the reaction, we are able to simulate successfully the experimental data.
We study pattern formation arising from the interaction of the stationary Turing and wave ͑oscillatory Turing͒ instabilities. Interaction and competition between these symmetry-breaking modes lead to the emergence of a large variety of spatiotemporal patterns, including modulated Turing structures, modulated standing waves, and combinations of Turing structures and spiral waves. Spatial resonances are obtained near codimension-two Turing-wave bifurcations. Far from bifurcation lines, we obtain inwardly propagating spiral waves with Turing spots at their tips. We demonstrate that the coexistence of Turing spots and traveling waves is a result of interaction between Turing and oscillatory modes, while the inwardly propagating waves ͑antispirals͒ do not require this interaction; they can arise from the wave instability combined with a negative group velocity.
Spatial resonances leading to superlattice hexagonal patterns, known as "black-eyes," and superposition patterns combining stripes and/or spots are studied in a reaction-diffusion model of two interacting Turing modes with different wavelengths. A three-phase oscillatory interlacing hexagonal lattice pattern is also found, and its appearance is attributed to resonance between a Turing mode and its subharmonic.
A model reaction-diffusion system with two coupled layers yields oscillatory Turing patterns when oscillation occurs in one layer and the other supports stationary Turing structures. Patterns include "twinkling eyes," where oscillating Turing spots are arranged as a hexagonal lattice, and localized spiral or concentric waves within spot-like or stripe-like Turing structures. A new approach to generating the short-wave instability is proposed.
Oscillatory cluster patterns are studied numerically in a reaction-diffusion model of the photosensitive Belousov-Zhabotinsky reaction supplemented with a global negative feedback. In one- and two-dimensional systems, families of cluster patterns arise for intermediate values of the feedback strength. These patterns consist of spatial domains of phase-shifted oscillations. The phase of the oscillations is nearly constant for all points within a domain. Two-phase clusters display antiphase oscillations; three-phase clusters contain three sets of domains with a phase shift equal to one-third of the period of the local oscillation. Border (nodal) lines between domains for two-phase clusters become stationary after a transient period, while borders drift in the case of three-phase clusters. We study the evolving border movement of the clusters, which, in most cases, leads to phase balance, i.e., equal areas of the different phase domains. Border curling of three-phase clusters results in formation of spiral clusters-a combination of a fast oscillating cluster with a slow spiraling movement of the domain border. At higher feedback coefficient, irregular cluster patterns arise, consisting of domains that change their shape and position in an irregular manner. Localized irregular and regular clusters arise for parameters close to the boundary between the oscillatory region and the reduced steady state region of the phase space.
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