We present a study of electric, thermal and thermoelectric response in noncollinear antiferromagnet Mn3Sn, which hosts a large Anomalous Hall Effect (AHE). Berry curvature generates off-diagonal thermal(Righi-Leduc) and thermoelectric(Nernst) signals, which are detectable at room temperature and invertible with a small magnetic field. The thermal and electrical Hall conductivities respect the Wiedemann-Franz law, implying that the transverse currents induced by Berry curvature are carried by Fermi surface quasi-particles. In contrast to conventional ferromagnets, the anomalous Lorenz number remains close to the Sommerfeld number over the whole temperature range of study, excluding any contribution by inelastic scattering and pointing to Berry curvature as the unique source of AHE. The anomalous off-diagonal thermo-electric and Hall conductivities are strongly temperature-dependent and their ratio is close to kB/e.The ordinary Hall effect, the transverse electric field generated by a longitudinal charge current in presence of a magnetic field, is caused by the Lorentz force exerted by magnetic field on charge carriers. In ferromagnetic solids, there is an additional component to this response (known as extraordinary or anomalous), thought to arise as a result of a sizeable magnetization. During the past decade, a clear link between the Anomalous Hall Effect (AHE) and the Berry curvature of Bloch waves has been established [1,2]. Charged carriers of entropy are also affected by the Lorenz force. Therefore, one expects a transverse component to thermal conductivity called the Righi-Leduc (or the thermal Hall) effect [3] in presence of magnetic field. This is also the case of thermoelectric conductance, which acquires an off-diagonal component, α ij , intimately linked to the Nernst coefficient, directly measurable by experiment [4]. When the Berry curvature replaces the magnetic field, counterparts of the AHE appear in the thermal and thermoelectric response of ferromagnets [5][6][7][8]. They can be an additional source of information regarding the fundamental mechanism leading to the generation of dissipationless transverse currents. Recently, following a proposition by Chen, Niu and Macdonald[9], Nakasutji et al. and Nayak et al. found a large AHE in Mn 3 Sn [10] and Mn 3 Ge [11,12], which are noncollinear antiferromagnets at room temperature. Several recent theoretical studies were devoted to this issue [13][14][15].In this letter, we present a study of Anomalous Righi-Leduc and Nernst effects (ANE) in Mn 3 Sn in order to quantify the amplitude of these coefficients compared to their Hall counterpart.We detect a large Anomalous Righi-Leduc conductivity and find that its magnitude corresponds to what is expected according to the Wiedemann-Franz (WF) Law over an extended temperature window. The result confirms a theoretical prediction by Haldane[16] with important consequences for the debate regarding the two alternative formulations of anomalous Hall effect [16][17][18]. AHE can be formulated as a property of th...
Intrinsic anomalous Nernst effect (ANE), like its Hall counterpart, is generated by Berry curvature of electrons in solids. Little is known about its response to disorder. In contrast, the link between the amplitude of the ordinary Nernst coefficient (ONE) and the mean-free-path is extensively documented. Here, by studying Co3Sn2S2, a topological half-metallic semimetal hosting sizable and recognizable ordinary and anomalous Nernst responses, we demonstrate an anti-correlation between the amplitude of ANE and carrier mobility. We argue that the observation, paradoxically, establishes the intrinsic origin of the ANE in this system. We conclude that various intrinsic off-diagonal coefficients are set by the way the Berry curvature is averaged on a grid involving the mean-free-path, the Fermi wavelength and the de Broglie thermal length.
The Wiedemann-Franz (WF) law links the ratio of electronic charge and heat conductivity to fundamental constants. It has been tested in numerous solids, but the extent of its relevance to the anomalous transverse transport, which represents the topological nature of the wave function, remains an open question. Here we present a study of anomalous transverse response in the noncollinear antiferromagnet Mn3Ge extended from room temperature down to sub-Kelvin temperature and find that the anomalous Lorenz ratio remains close to the Sommerfeld value up to 100 K, but not above. The finite-temperature violation of the WF correlation is caused by a mismatch between the thermal and electrical summations of the Berry curvature, rather than the inelastic scattering as observed in ordinary metals. This interpretation is backed by our theoretical calculations, which reveals a competition between the temperature and the Berry curvature distribution. The accuracy of the experiment is supported by the verification of the Bridgman relation between the anomalous Ettingshausen and Nernst effects. Our results identify the anomalous Lorenz ratio as an extremely sensitive probe of Berry spectrum near the chemical potential. arXiv:1812.04339v3 [cond-mat.str-el]
Magnetic domain walls are topological solitons whose internal structure is set by competing energies which sculpt them. In common ferromagnets, domain walls are known to be of either Bloch or Néel types. Little is established in the case of Mn 3 Sn, a triangular antiferromagnet with a large room-temperature anomalous Hall effect, where domain nucleation is triggered by a well-defined threshold magnetic field. Here, we show that the domain walls of this system generate an additional contribution to the Hall conductivity tensor and a transverse magnetization. The former is an electric field lying in the same plane with the magnetic field and electric current and therefore a planar Hall effect. We demonstrate that in-plane rotation of spins inside the domain wall would explain both observations and the clockwise or anticlockwise chirality of the walls depends on the history of the field orientation and can be controlled.
Mn 3 X (X= Sn, Ge) are noncollinear antiferromagnets hosting a large anomalous Hall effect (AHE). Weyl nodes in the electronic dispersions are believed to cause this AHE, but their locus in the momentum space is yet to be pinned down. We present a detailed study of the Hall conductivity tensor and magnetization in Mn 3 Sn crystals and find that in the presence of a moderate magnetic field, spin texture sets the orientation of the k-space Berry curvature with no detectable inplane anisotropy due to the Z 6 symmetry of the underlying lattice. We quantify the energy cost of domain nucleation and show that the multidomain regime is restricted to a narrow field window. Comparing the field dependence of AHE and magnetization, we find that there is a distinct component in the AHE which does not scale with magnetization when the domain walls are erected. This socalled 'topological' Hall effect provides indirect evidence for a non-coplanar spin components and real-space Berry curvature in domain walls.
Magnetic Weyl semimetals (WSMs) bearing long-time pursuing are still very rare. We herein identified magnetic exchange induced Weyl state in EuCd 2 Sb 2 , a semimetal in type IV magnetic space group, via performing high magnetic field
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