All-optical-fiber Fabry-Perot interferometers (FPIs) with microcavities of different shapes were investigated. It was found that the size and shape of the cavity plays an important role on the performance of these interferometers. To corroborate the analysis, FPIs with spheroidal cavities were fabricated by splicing a photonic crystal fiber (PCF) with large voids and a conventional single mode fiber (SMF), using an ad hoc splicing program. It was found that the strain sensitivity of FPIs with spheroidal cavities can be controlled through the dimensions of the spheroid. For example, a FPI whose cavity had a size of ~10x60 μm exhibited strain sensitivity of ~10.3 pm/με and fringe contrast of ~38 dB. Such strain sensitivity is ~10 times larger than that of the popular fiber Bragg gratings (~1.2 pm/με) and higher than that of most low-finesse FPIs. The thermal sensitivity of our FPIs is extremely low (~1pm/°C) due to the air cavities. Thus, a number of temperature-independent ultra-sensitive microscopic sensors can be devised with the interferometers here proposed since many parameters can be converted to strain. To this end, simple vibration sensors are demonstrated.
We demonstrate the digital electric field induced switching of plasmonic nanorods between "1" and "0" orthogonal aligned states using an electro-optic fluid fiber component. We show by digitally switching the nanorods, that thermal rotational diffusion of the nanorods can be circumvented, demonstrating an approach to achieve submicrosecond switching times. We also show, from an initial unaligned state, that the nanorods can be aligned into the applied electric field direction in 110 nanoseconds. The high-speed digital switching of plasmonic nanorods integrated into an all-fiber optical component may provide opportunities for remote sensing and signaling applications.In general, the permanent or induced dipole moment and resulting polarizability of a molecule is too small to couple to external electric fields to overcome disordering thermal forces, preventing alignment. If anisotropic molecules are condensed into a liquid crystal phase, then the additional van der Waal forces from the nearneighbor interactions increases the polarizability to enable alignment of the molecules and control the optical properties. The electric field induced alignment of anisotropic molecules in liquid crystal phases has enabled disruptive technologies such as smart phones and flat screen displays. 1,2The switching time of these materials depends on the sum of their on-and off -times. The on-time needed to align the molecules into the direction of the applied electric field is predominately set by the magnitude of the field applied, τ on ≈ γ/εE 2 , where γ is the viscosity, ε is the dielectric permittivity and E is the electric field. The off -time is related to the thermal rotational diffusion of the liquid crystal molecules and typically is the limiting factor to determine the overall switching time. In the case of liquid crystals, the near-neighbor interactions create strong electrohydrodynamic coupling, leading to a slow characteristic off -time, τ of f ≈ γd 2 /K ≈ ms, where d is the cell thickness and K is the elastic constant of the liquid crystal. This well-known limitation has constrained potential electro-optic applications for decades.A recent elegant approach avoided re-alignment of the molecules altogether by rapidly electrically inducing a change in the refractive index of the molecules in a liquid crystal phase.3 The response time of this system was 10 s of nanoseconds, yet the change in the optical properties was small and cannot be maintained for long times before a) Electronic mail: walter.margulis@ri.se b) Electronic mail: jake.fontana@nrl.navy.mil the usual electric field induced alignment of the molecules occurs.The electric field induced alignment of plasmonic nanorods is a paradigm to anisotropic molecules in liquid crystal phases.4 A key advantage of plasmonic nanorods is that the polarizibility of a single nanorod in a dilute suspension is adequately large to couple to an external electric field, enabling alignment and the ability to tune the optical properties at visible and near infrared wavelengths.4,5 A sig...
The capability to dynamically control the nonlinear refractive index of plasmonic suspensions may enable innovative nonlinear sensing and signaling nanotechnologies. Here, we experimentally determine the effective nonlinear refractive index for gold nanorods suspended in an index matching oil aligned using electric fields, demonstrating an approach to modulate the nonlinear optical properties of the suspension. The nonlinear optical experiments were carried out using a Hartmann-Shack wavefront aberrometer in a collimated beam configuration with a high repetition rate femtosecond laser. The suspensions were probed at 800 nm, overlapping with the long-axis absorption peak of the nanorods. We find that the effective nonlinear refractive index of the gold nanorods suspension depends linearly on the orientational order parameter, S, which can be understood by a thermally induced nonlinear response. We also show the magnitude of the nonlinear response can be varied by ∼ 60%.
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