In this study, NiCoFe2O4 nanoparticles were prepared and used as a reactive catalyst for the synthesis of trisubstituted imidazoles. The multicomponent reactions of aromatic aldehydes, benzil and ammonium acetate were carried out under solvent-free and conventional heating conditions. In this reaction, some imidazole derivatives with high purity, short reaction times and high yields were obtained. The prepared nanocatalyst was characterized by FT-IR, XRD, EDX, VSM and SEM techniques. Moreover, the organic products were identified by melting point, FT-IR and 1H NMR analyzes.

In this research, it was presented a simple and easy method for the preparation of graphene oxide (GO) supported ZnO nanoparticles with low cost, available precursor and their application as nanocatalyst for synthesis of l,4-dihydropyirimidinones. When GO combines with metal oxide nanoparticles such as ZnO shows very good properties. There is a wide range of chemical methods for the attachment of various functional groups. In this protocol, the GO was synthesized through Hummer's method. The structure and morphology properties of ZnO NPs@rGO nanocomposite were investigated by Fouriertransform infrared spectroscopy, X-ray diffraction, scanning electron microscopy, and energy-dispersive X-ray spectroscope techniques. Also, the organic compounds were identified by melting point, FT-IR, and proton nuclear magnetic resonance analyses.

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