Nanostructured metasurfaces demonstrate extraordinary capabilities to control light at the subwavelength scale, emerging as key optical components to physical realization of multitasked devices. Progress in multitasked metasurfaces has been witnessed in making a single metasurface multitasked by mainly resorting to extra spatial freedom, for example, interleaved subarrays, different angles. However, it imposes a challenge of suppressing the cross-talk among multiwavelength without the help of extra spatial freedom. Here, we introduce an entirely novel strategy of multitasked metasurfaces with noninterleaved single-size Si nanobrick arrays and minimalist spatial freedom demonstrating massive information on 6-bit encoded color holograms. The interference between electric dipole and magnetic dipole in individual Si nanobricks with in-plane orientation enables manipulating six bases of incident photons simultaneously to reconstructed 6-bit wavelength-and spin-dependent multicolor images. Those massively reconstructed images can be distinguished by pattern recognition. It opens an alternative route for integrated optics, data encoding, security encryption, and information engineering.
Metasurfaces hold great potentials for advanced holographic display with extraordinary information capacity and pixel sizes in an ultrathin flat profile. Dual-polarization channel to encode two independent phase profiles or spatially multiplexed metaholography by interleaved metasurfaces are captivated popular solutions to projecting multiplexed and vectorial images. However, the intrinsic limit of orthogonal polarization-channels, their crosstalk due to coupling between meta-atoms, and interleaving-induced degradation of efficiency and reconstructed image quality set great barriers for sophisticated meta-holography from being widely adopted. Here we report a non-interleaved TiO2 metasurface holography, and three distinct phase profiles are encoded into three orthogonal polarization bases with almost zero crosstalk. The corresponding three independently constructed intensity profiles are therefore assigned to trichromatic (RGB) beams, resulting in high-quality and high-efficiency vectorial meta-holography in the whole visible regime. Our strategy presents an unconventionally advanced holographic scheme by synergizing trichromatic colors and tri-polarization channels, simply realized with a minimalist non-interleaved metasurface. Our work unlocks the metasurface's potentials on massive information storage, polarization optics, polarimetric imaging, holographic data encryption, etc.Keywords: tri-polarization-channel metasurface; trichromatic vectorial holography; polarization conversion; non-interleaved metasurface; dielectric nanostructures. IntroductionSubwavelength metal or dielectric meta-units arranging in a two-dimensional plane form a metasurface, which can almost arbitrarily manipulate the wavefront such as amplitude, phase and polarization 1-3 . The complementary metal oxide semiconductor (CMOS) compatible fabrication process enables various metasurfaces components in the optical range that are more compact and perform better than conventional refractive optics, such as abnormal reflector/refractor 1, 4-6 , color filter 7, 8 , metalens 3, 9-11 , metahologram 12-14 , quantum metasurfaces 15-17 and multifunctional metasurfaces 18-21 .Multichannel metasurface-based devices have been extensively studied. One important application is to reconstruct full-color images. The crosstalk among different wavelengths is taken care of mainly by two approaches: optimized phase retrieval algorithm and judiciously optimized meta-atoms. The first approach enables a single phase profile to generate a color image by introducing position information in the phase retrieval processes to suppress the crosstalk among different operational wavelengths in the observation region [22][23][24] . However, unwanted images will be induced in other regions. On the other hand, the second approach is to provide wavelength-dependent phase profiles via carefully tailored meta-atoms 14,[25][26][27][28][29] , which can support wavelengthdependent responses. The meta-atom subarrays specifically designed for each given wavelength can be interleaved...
Monolayer two-dimensional transition-metal dichalcogenides (2D TMDCs) exhibit promising characteristics in miniaturized nonlinear optical frequency converters, due to their inversion asymmetry and large second-order nonlinear susceptibility. However, these materials usually have very short light interaction lengths with the pump laser because they are atomically thin, such that second-harmonic generation (SHG) is generally inefficient. In this paper, we fabricate a judiciously structured 150 nm-thick planar surface consisting of monolayer tungsten diselenide and sub-20 nm-wide gold trenches on flexible substrates, reporting ∼7000-fold SHG enhancement without peak broadening or background in the spectra as compared to WSe on as-grown sapphire substrates. Our proof-of-concept experiment yields effective second-order nonlinear susceptibility of 2.1 × 10 pm/V. Three orders of magnitude enhancement is maintained with pump wavelength ranging from 800 to 900 nm, breaking the limitation of narrow pump wavelength range for cavity-enhanced SHG. In addition, SHG amplitude can be dynamically controlled via selective excitation of the lateral gap plasmon by rotating the laser polarization. Such a fully open, flat, and ultrathin profile enables a great variety of functional samples with high SHG from one patterned silicon substrate, favoring scalable production of nonlinear converters. The surface accessibility also enables integration with other optical components for information processing in an ultrathin and flexible form.
Metasurfaces as artificially nanostructured interfaces hold significant potential for multi-functionality, which may play a pivotal role in the next-generation compact nano-devices. The majority of multi-tasked metasurfaces encode or encrypt multi-information either into the carefully tailored metasurfaces or in pre-set complex incident beam arrays. Here, we propose and demonstrate a multi-momentum transformation metasurface (i.e., meta-transformer), by fully synergizing intrinsic properties of light, e.g., orbital angular momentum (OAM) and linear momentum (LM), with a fixed phase profile imparted by a metasurface. The OAM meta-transformer reconstructs different topologically charged beams into on-axis distinct patterns in the same plane. The LM meta-transformer converts red, green and blue illuminations to the on-axis images of “R”, “G” and “B” as well as vivid color holograms, respectively. Thanks to the infinite states of light-metasurface phase combinations, such ultra-compact meta-transformer has potential in information storage, nanophotonics, optical integration and optical encryption.
Understanding the unique characteristics of plexcitons, hybridized states resulting from the strong coupling between plasmons and excitons, is vital for both fundamental studies and practical applications in nano-optics. However, the research of plexcitons from the perspective of chiral optics has been rarely reported. Here, we experimentally investigate the optical chirality of plexcitonic systems consisting of composite metal nanoparticles and chiral J-aggregates in the strong coupling regime. Mode splitting and anticrossing behavior are observed in both the circular dichroism (CD) and extinction spectra of the hybrid nanosystems. A large mode splitting (at zero detuning) of up to 136 meV/214 meV in CD/extinction measurements confirms that the systems attain the strong coupling regime. This phenomenon indicates that the formation of plexcitons modifies not only the extinction but also the optical chirality of the hybrid systems. We develop a quasistatic theory to elucidate the chiral optical responses of hybrid systems. Furthermore, we propose and justify a criterion of strong plasmon–exciton interaction: the mode splitting in the CD spectra (at zero detuning) is larger than half of that in the extinction spectra. Our findings give a chiral perspective on the study of strong plasmon–exciton coupling and have potential applications in the chiral optical field.
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