The excitation of electrostatic waves in plasma by laser electromagnetic (EM) pulse is important as it provides a scheme by which the power from the laser EM field can be transferred into the plasma medium. The paper presents a fundamentally new ponderomotive pressure-driven mechanism of excitation of electrostatic waves in an overdense magnetized plasma by a finite laser pulse. Particle-in-cell simulations using the EPOCH-4.17.10 framework have been utilized for the study of a finite laser pulse interacting with a magnetized overdense plasma medium. The external magnetic field is chosen to be aligned parallel to the laser propagation direction. In this geometry, the EM wave propagation inside the plasma is identified as whistler or R and L waves. The group velocity of these waves being different, a clear spatial separation of the R and L pulses are visible. In addition, excitation of electrostatic perturbation associated with the EM pulses propagating inside the plasma is also observed. These electrostatic perturbations are important as they couple laser energy to the plasma medium. The excitation of electrostatic oscillations are understood here by a fundamentally new mechanism of charge separation created by the difference between the ponderomotive force (of the EM pulse) felt by the two plasma species, viz., the electrons and the ions in a magnetized plasma.

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The mechanism of harmonic generation in both O- and X-mode configurations for a magnetized plasma has been explored here in detail with the help of particle-in-cell simulations. A detailed characterization of both the reflected and transmitted electromagnetic radiation propagating in the bulk of the plasma has been carried out for this purpose. The efficiency of harmonic generation is shown to increase with the incident laser intensity. A dependency of harmonic efficiency has also been found on magnetic field strength. This work demonstrates that there is an optimum value of the magnetic field at which the efficiency of harmonic generation maximizes. The observations are in agreement with theoretical analysis. For the O-mode configuration, this is compelling as the harmonic generation provides for a mechanism by which laser energy can propagate inside an overdense plasma region.

We report the fabrication of low cost highly structured silver (Ag) capped aluminium (Al) nanorods (NRs) as surface enhanced Raman spectroscopy (SERS) substrate utilising the glancing angle deposition technique. The nano-capping of silver onto the Al NRs can concentrate the local electric field within the minimal volume that can serve as hotspots. The average size of the Ag nanocaps was 50 nm. The newly proposed nanoporous Ag capped Al NRs as SERS substrate could detect the Raman signal of rhodamine 6G (R6G) up to 10 −15 molar concentration. The significant enhancement in the Raman signal of 10 7 was achieved for Ag capped Al NRs considering R6G as a probe molecule. Using the developed SERS substrate, we recorded Raman spectra for Escherichia coli bacteria with its concentration varying from 10 8 colony forming units per ml (CFU ml −1 ) up to 10 2 CFU ml −1 . All the reported Raman spectra were acquired by a portable handheld Raman spectrometer. Hence, this newly proposed low cost, effective SERS substrate can be used commercially for the onsite detection of clinical pathogens. The 3D finite difference time domain simulation model was performed for Ag capped Al nanostructure to understand the generation of hotspots. The simulated results show excellent agreement with the experimental results. We fabricated uncapped Ag nanorods of similar dimensions and performed the experimental measurements and simulations for comparison. We found a significant enhancement in Ag capped Al NRs compared to the long Ag NRs. The description of the Raman signal enhancement has been elaborated.

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