The framework of relativistic energy density functionals is extended to include correlations related to restoration of broken symmetries and fluctuations of collective variables. A new implementation is developed for the solution of the eigenvalue problem of a five-dimensional collective Hamiltonian for quadrupole vibrational and rotational degrees of freedom, with parameters determined by constrained self-consistent relativistic mean-field calculations for triaxial shapes. The model is tested in a series of illustrative calculations of potential energy surfaces and the resulting collective excitation spectra and transition probabilities of the chain of even-even gadolinium isotopes.

The article reviews the general version of the Bohr collective model for the description of quadrupole collective states, including a detailed discussion of the model's kinematics. The quadrupole coordinates, momenta and angular momenta are defined and the structure of the isotropic tensor fields as functions of the tensor variables is investigated. After a comprehensive discussion of the quadrupole kinematics, the general form of the classical and quantum Bohr Hamiltonian is presented. The electric and magnetic multipole moment operators acting in the collective space are constructed and the collective sum rules are given. A discussion of the tensor structure of the collective wavefunctions and a review of various methods of solving the Bohr Hamiltonian eigenvalue equation are also presented. Next, the methods of derivation of the classical and quantum Bohr Hamiltonian from the microscopic many-body theory are recalled. Finally, the microscopic approach to the Bohr Hamiltonian is applied to interpret collective properties of 12 heavy even-even nuclei in the Hf-Hg region. Calculated energy levels and E2 transition probabilities are compared with experimental data.

The Coulomb excitation experiment to study electromagnetic properties of the heaviest stable Mo isotope, 100 Mo, was performed using a 76 MeV 32 S beam from the Warsaw cyclotron U-200P. Magnitudes and relative signs of 26 E1, E2, E3, and M1 matrix elements coupling nine low-lying states in 100 Mo were determined using the least-squares code GOSIA. Diagonal matrix elements (related to the spectroscopic quadrupole moments) of the 2 + 1 , 2 + 2 , and 2 + 3 states as well as the 4 + 1 state were extracted. The resulting set of reduced E2 matrix elements was complete and precise enough to obtain, using the quadrupole sum rules approach, quadrupole deformation parameters of 100 Mo in its two lowest 0 + states: ground and excited. The overall deformation of the 0 + 1 and 0 + 2 states in 100 Mo is of similar magnitude, in both cases larger compared to what was found for the neighboring isotopes 96 Mo and 98 Mo. At the same time, the asymetry parameters obtained for both states strongly differ, indicating a triaxial shape of the 100 Mo nucleus in the ground state and a prolate shape in the excited 0 + state. Low-energy quadrupole excitations of the 100 Mo nucleus were studied in the frame of the general quadrupole collective Bohr Hamiltonian model (GBH). The potential energy and inertial functions were calculated using the adiabatic time-dependent Hartree-Fock-Bogoliubov (ATDHFB) method starting from two possible variants of the Skyrme effective interaction: SIII and Sly4. The overall quadrupole deformation parameters resulting from the GBH calculations with the SLy4 variant of the Skyrme interaction are slightly closer to the experimentally obtained values than those obtained using SIII.

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