Abstract. In this paper we describe and summarize the main achievements of the European Aerosol Cloud Climate and Air Quality Interactions project (EUCAARI). EUCAARI started on 1 January 2007 and ended on 31 December 2010 leaving a rich legacy including: (a) a comprehensive database with a year of observations of the physical, chemical and optical properties of aerosol particles over Europe, (b) comprehensive aerosol measurements in four developing countries, (c) a database of airborne measurements of aerosols and clouds over Europe during May 2008, (d) comprehensive modeling tools to study aerosol processes fron nano to global scale and their effects on climate and air quality. In addition a new Pan-European aerosol emissions inventory was developed and evaluated, a new cluster spectrometer was built and tested in the field and several new aerosol parameterizations and computations modules for chemical transport and global climate models were developed and evaluated. These achievements and related studies have substantially improved our understanding and reduced the uncertainties of aerosol radiative forcing and air quality-climate interactions. The EUCAARI results can be utilized in European and global environmental policy to assess the aerosol impacts and the corresponding abatement strategies.

This article is published with the permission of the Controller of HMSO and the Queen's Printer for Scotland.The predictive quality of an ensemble model of cirrus ice crystals to model passive and active measurements of ice cloud, from the ultraviolet (UV) to the microwave, is tested. The ensemble model predicts m ∝ D 2 , where D is the maximum dimension of the ice crystal, and m is its mass. This predicted m-D relationship is applied to a moment estimation parametrization of the particle size distribution (PSD), to estimate the PSD shape, given ice water content (IWC) and in-cloud temperature. The same microphysics is applied across the electromagnetic spectrum to model UV, infrared, microwave and radar observations. The short-wave measurements consist of airborne UV backscatter lidar (light detection and ranging) estimates of the volume extinction coefficient, total solar optical depth, and spacebased multi-directional spherical albedo retrievals, at 0.865 µm, between the scattering angles 85 • and 125 • . The airborne long-wave measurements consist of high-resolution interferometer upwelling brightness temperatures, obtained between the wavelengths of about 3.45 µm and 4.1 µm, and 8.0 µm to 12.0 µm. The low-frequency measurements consist of ground-based Chilbolton 35 GHz radar reflectivity measurements and spacebased upwelling 190 GHz brightness temperature measurements. The predictive quality of the ensemble model is demonstrated to be generally within the experimental uncertainty of the lidar backscatter estimates of the volume extinction coefficient and total solar optical depth. The ensemble model prediction of the high-resolution brightness temperature measurements is generally within ±2 K and ±1 K at solar and infrared wavelengths, respectively. The 35 GHz radar reflectivity and 190 GHz brightness temperatures are generally simulated to within ±2 dBZ e , and ±2 K, respectively. The directional spherical albedo observations suggest that the scattering phase function of the most randomized ensemble model gives the best fit to the measurements (generally within ±3%). This article demonstrates that the ensemble model, assuming the same microphysics, is physically consistent across the electromagnetic spectrum.

In this paper we describe and summarize the main achievements of the European Aerosol Cloud Climate and Air Quality Interactions project (EUCAARI). EUCAARI started on 1 January 2007 and ended on 31 December 2010 leaving a rich legacy including: (a) a comprehensive database with a year of observations of the physical, chemical and optical properties of aerosol particles over Europe, (b) the first comprehensive aerosol measurements in four developing countries, (c) a database of airborne measurements of aerosols and clouds over Europe during May 2008, (d) comprehensive modeling tools to study aerosol processes fron nano to global scale and their effects on climate and air quality. In addition a new Pan-European aerosol emissions inventory was developed and evaluated, a new cluster spectrometer was built and tested in the field and several new aerosol parameterizations and computations modules for chemical transport and global climate models were developed and evaluated. This work enabled EUCAARI to improve our understanding of aerosol radiative forcing and air quality-climate interactions. The EUCAARI results can be utilized in European and global environmental policy to assess the aerosol impacts and the corresponding abatement strategies

Abstract. This is the first paper to investigate the relationship between the scattering phase function of cirrus and the relative humidity with respect to ice (RHi), using space-based solar radiometric angle-dependent measurements. The relationship between RHi, and the complexity of ice crystals has been previously studied using data from aircraft field campaigns and laboratory cloud chambers. However, to the best of our knowledge, there have been no studies to date that explore this relationship, through the use of remotely sensed space-based angle-dependent solar radiometric measurements. In this paper, a case study of semi-transparent cirrus is used to explore the possibility of such a relationship. Moreover, for the first time, RHi fields predicted by a high-resolution numerical weather prediction (NWP) model are combined with satellite retrievals of ice crystal complexity. The NWP model was initialised at midnight, on the 25 January 2010, and the mid-latitude RHi field was extracted from the NWP model at 13:00 UTC. At about the same time, there was a Polarization and Anisotropy of Reflectance for Atmospheric science coupled with Observations from a Lidar (PARASOL) overpass, and the PARASOL swath covered the NWP model predicted RHi field. The cirrus case was located over Scotland, and over the North Sea. From the satellite channel based at 0.865 μm, the directionally averaged and directional spherical albedos were retrieved between the scattering angles of about 80° and 130°. An ensemble model of cirrus ice crystals is used to predict phase functions that vary between phase functions that exhibit optical features (called pristine), to featureless phase functions. For each of the PARASOL pixels, the phase function that best minimised differences between the spherical albedos was selected. This paper reports a positive correlation between the scattering phase function and RHi. That is, the pristine and completely featureless phase functions are found to be correlated with RHi < 100%, and RHi> 100%, respectively. Moreover, it is demonstrated that the NWP model prediction of the vertical profile of RHi is in good agreement with independent aircraft-based physical retrievals of RHi. Furthermore, the NWP model prediction of the cirrus cloud-top height and its vertical extent is also found to be in good agreement with aircraft-based lidar measurements.